Molecular dynamics investigated by temporally two-dimensional coherent Raman spectroscopy

dc.bibliographicCitation.firstPage35eng
dc.bibliographicCitation.issue1-4eng
dc.bibliographicCitation.volume19eng
dc.contributor.authorLau, A.
dc.contributor.authorPfeiffer, M.
dc.contributor.authorKozich, V.
dc.contributor.authorKummrow, A.
dc.date.accessioned2020-08-07T13:48:32Z
dc.date.available2020-08-07T13:48:32Z
dc.date.issued1999
dc.description.abstractA six-wave set-up is described to determine molecular dynamics in the condensed phase. Applying two independent time delays between excitation and probe pulses additional information on the dynamics should be obtainable. We show experimentally that such investigations can be carried out with noisy light having intensity fluctuations in the femtosecond region. As first result we found a fast relaxation time in neat nitrobenzene of 100 fs, becoming even faster in mixtures with low viscosity liquids. Switching on a Raman resonance yields a longer relaxation time, which could be explained by an additional contribution by that vibration.eng
dc.description.versionpublishedVersioneng
dc.identifier.urihttps://doi.org/10.34657/4034
dc.identifier.urihttps://oa.tib.eu/renate/handle/123456789/5405
dc.language.isoengeng
dc.publisherRoutledge : Taylor and Francis Inc.eng
dc.relation.doihttps://doi.org/10.1155/1999/41281
dc.relation.ispartofseriesLaser Chemistry 19 (1999), Nr. 1-4eng
dc.relation.issn0278-6273
dc.rights.licenseCC BY 3.0 Unportedeng
dc.rights.urihttps://creativecommons.org/licenses/by/3.0/eng
dc.subjectFifth order nonlinearityeng
dc.subjectKerr effecteng
dc.subjectNonlinear spectroscopyeng
dc.subjectRamaneng
dc.subject.ddc530eng
dc.titleMolecular dynamics investigated by temporally two-dimensional coherent Raman spectroscopyeng
dc.typearticleeng
dc.typeTexteng
dcterms.bibliographicCitation.journalTitleLaser Chemistryeng
tib.accessRightsopenAccesseng
wgl.contributorMBIeng
wgl.subjectPhysikeng
wgl.typeZeitschriftenartikeleng
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