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- ItemPhotoelectron holography in strong optical and dc electric fields(Bristol : Institute of Physics Publishing, 2014) Stodolna, A.; Huismans, Y.; Rouzée, A.; Lépine, F.; Vrakking, M.J.J.The application of velocity map imaging for the detection of photoelectrons resulting from atomic or molecular ionization allows the observation of interferometric, and in some cases holographic structures that contain detailed information on the target from which the photoelecrons are extracted. In this contribution we present three recent examples of the use of photoelectron velocity map imaging in experiments where atoms are exposed to strong optical and dc electric fields. We discuss (i) observations of the nodal structure of Stark states of hydrogen measured in a dc electric field, (ii) mid-infrared strong-field ionization of metastable Xe atoms and (iii) the reconstruction of helium electronic wavepackets in an attosecond pump-probe experiment. In each case, the interference between direct and indirect electron pathways, reminiscent of the reference and signal waves in holography, is seen to play an important role.
- ItemMapping the dissociative ionization dynamics of molecular nitrogen with attosecond resolution(Bristol : IOP Publ., 2015) Klinker, M.; Trabattoni, A.; González-Vázquez, J.; Liu, C.; Sansone, G.; Linguerri, R.; Hochlaf, M..; Klei, J.; Vrakking, M.J.J.; Martin, F.; Nisoli, M.; Calegari, F.We wish to understand the processes underlying the ionization dynamics of N2 as experimentally induced and studied by recording the kinetic energy release (KER) in a XUV-pump/IR-probe setup. To this end a theoretical model was developed describing the ionization process using Dyson Orbitals and, subsequently, the dissociation process using a large set of diabatic potential energy surfaces (PES) on which to propagate. From said set of PES, a small subset is extracted allowing for the identification of one and two photon processes chiefly responsible for the experimentally observed features.
- ItemStrong field ionization of small hydrocarbon chains with full 3D momentum analysis(Bristol : IOP Publ., 2015) Schulz, Claus Peter; Birkner, Sascha; Furch, Federico J.; Anderson, Alexandria; Mikosch, Jochen; Schell, Felix; Vrakking, Marc J. J.Strong field ionization of small hydrocarbon chains is studied in a kinematic complete experiment using a reaction microscope. By coincidence detection of ions and electrons different ionization continua populated during the ionization process are identified. In addition, photoelectron momentum distributions from laser-aligned molecules allow to characterize the electron wavepackets emerging from different Dyson orbitals.