CC BY 4.0 UnportedSchneider, MichaelPfau, BastianGünther, Christian M.von Korff Schmising, ClemensWeder, DavidGeilhufe, JanPerron, JonathanCapotondi, FlavioPedersoli, EmanueleManfredda, MicheleHennecke, MartinVodungbo, BorisLüning, JanEisebitt, Stefan2021-12-072021-12-072020https://oa.tib.eu/renate/handle/123456789/7650https://doi.org/10.34657/6697We systematically study the fluence dependence of the resonant scattering cross-section from magnetic domains in Co/Pd-based multilayers. Samples are probed with single extreme ultraviolet (XUV) pulses of femtosecond duration tuned to the Co M3,2 absorption resonances using the FERMI@Elettra free-electron laser. We report quantitative data over 3 orders of magnitude in fluence, covering 16  mJ/cm2/pulse to 10 000  mJ/cm2/pulse with pulse lengths of 70 fs and 120 fs. A progressive quenching of the diffraction cross-section with fluence is observed. Compression of the same pulse energy into a shorter pulse—implying an increased XUV peak electric field—results in a reduced quenching of the resonant diffraction at the Co M3,2 edge. We conclude that the quenching effect observed for resonant scattering involving the short-lived Co 3p core vacancies is noncoherent in nature. This finding is in contrast to previous reports investigating resonant scattering involving the longer-lived Co 2p states, where stimulated emission has been found to be important. A phenomenological model based on XUV-induced ultrafast demagnetization is able to reproduce our entire set of experimental data and is found to be consistent with independent magneto-optical measurements of the demagnetization dynamics on the same samples.enghttps://creativecommons.org/licenses/by/4.0/550530Ultrafast magnetization dynamicsMagnetic multilayersX-ray magnetic circular dichroismArticle