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- ItemDaytime ozone loss term in the mesopause region(Katlenburg, Lindau : Copernicus, 2017-5-23) Kulikov, Mikhail Y.; Belikovich, Mikhail V.; Grygalashvyly, Mykhaylo; Sonnemann, Gerd R.; Ermakova, Tatiana S.; Nechaev, Anton A.; Feigin, Alexander M.For the retrieval of atomic oxygen via ozone observations in the extended mesopause region under sunlight conditions, two assumptions are used: first, the photochemical equilibrium of ozone and, second, that the ozone losses are dominated by ozone's dissociation from solar UV radiation, silently ignoring the O3 destruction by atomic hydrogen. We verify both by 3-D modeling. We found that ozone approaches photochemical equilibrium at 75–100 km for daytime conditions. Hence, the first assumption is valid. However, the reaction of ozone with atomic hydrogen was found to be an important loss process and should not be omitted in retrieving atomic oxygen.
- ItemThe revised method for retrieving daytime distributions of atomic oxygen and odd-hydrogens in the mesopause region from satellite observations(Heidelberg : Springer, 2022) Kulikov, Mikhail Y.; Belikovich, Mikhail V.; Grygalashvyly, Mykhaylo; Sonnemann, Gerd R.; Feigin, Alexander M.Atomic oxygen (O) and atomic hydrogen (H) in the mesopause region are critical species, governing chemistry, airglow, and energy budget. However, they cannot be directly measured by satellite remote sensing techniques and so inference techniques, by airglow observations, are used. In this work, we retrieved daytime O and H distributions at ~ 77 km–100 km from the data of observations by the SABER (Sounding of the Atmosphere using Broadband Emission Radiometry) instrument at the TIMED (Thermosphere Ionosphere Mesosphere Energetics and Dynamics) satellite in 2003–2015. The retrieval approach considered the reaction H + O3 → O2 + OH in the ozone balance equation. Moreover, we revised all quenching and spontaneous emission coefficients according to latest published data. We then calculated daytime distributions of OH and HO2 at these altitudes with the use of their conditions of photochemical equilibrium.