2011, Gademann, G., Kelkensberg, F., Siu, W.K., Johnsson, P., Gaarde, M.B., Schafer, K.J., Vrakking, M.J.J.

We show that high harmonic generation driven by an intense nearinfrared (IR) laser can be temporally controlled when an attosecond pulse train (APT) is used to ionize the generation medium, thereby replacing tunnel ionization as the first step in the well-known three-step model. New harmonics are formed when the ionization occurs at a well-defined time within the optical cycle of the IR field. The use of APT-created electron wave packets affords new avenues for the study and application of harmonic generation. In the present experiment, this makes it possible to study harmonic generation at IR intensities where tunnel ionization does not give a measurable signal.

2010, Mauritsson, J., Remetter, T., Swoboda, M., Klünder, K., L'Huillier, A., Schafer, K.J., Ghafur, O., Kelkensberg, F., Siu, W., Johnsson, P., Vrakking, M.J.J., Znakovskaya, I., Uphues, T., Zherebtsov, S., Kling, M.F., Lépine, F., Benedetti, E., Ferrari, F., Sansone, G., Nisoli, M.

We present an interferometric pump-probe technique for the characterization of attosecond electron wave packets (WPs) that uses a free WP as a reference to measure a bound WP. We demonstrate our method by exciting helium atoms using an attosecond pulse (AP) with a bandwidth centered near the ionization threshold, thus creating both a bound and a free WP simultaneously. After a variable delay, the bound WP is ionized by a few-cycle infrared laser precisely synchronized to the original AP. By measuring the delay-dependent photoelectron spectrum we obtain an interferogram that contains both quantum beats as well as multipath interference. Analysis of the interferogram allows us to determine the bound WP components with a spectral resolution much better than the inverse of the AP duration. © 2010 The American Physical Society.