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- ItemCharging of mesospheric aerosol particles: The role of photodetachment and photoionization from meteoric smoke and ice particles(Göttingen : Copernicus, 2009) Rapp, M.Time constants for photodetachment, photoemission, and electron capture are considered for two classes of mesospheric aerosol particles, i.e., meteor smoke particles (MSPs) and pure water ice particles. Assuming that MSPs consist of metal oxides like Fe2O3 or SiO, we find that during daytime conditions photodetachment by solar photons is up to 4 orders of magnitude faster than electron attachment such that MSPs cannot be negatively charged in the presence of sunlight. Rather, even photoemission can compete with electron capture unless the electron density becomes very large (≫1000 cm-3) such that MSPs should either be positively charged or neutral in the case of large electron densities. For pure water ice particles, however, both photodetachment and photoemission are negligible due to the wavelength characteristics of its absorption cross section and because the flux of solar photons has already dropped significantly at such short wavelengths. This means that water ice particles should normally be negatively charged. Hence, our results can readily explain the repeated observation of the coexistence of positive and negative aerosol particles in the polar summer mesopause, i.e., small MSPs should be positively charged and ice particles should be negatively charged. These results have further important implications for our understanding of the nucleation of mesospheric ice particles as well as for the interpretation of incoherent scatter radar observations of MSPs. © 2009 Author(s).
- ItemInfluence of tides and gravity waves on layering processes in the polar summer mesopause region(Göttingen : Copernicus, 2008) Hoffmann, P.; Rapp, M.; Fiedler, J.; Latteck, R.Polar Mesosphere Summer Echoes (PMSE) have been studied at Andenes (69° N, 16° E), Norway, using VHF radar observations since 1994. One remarkable feature of these observations is the fact that {during 50% of the time,} the radar echoes occur in the form of two or more distinct layers. In the case of multiple PMSE layers, statistical analysis shows that the lower layer occurs at a mean height of ∼83.4 km, which is almost identical to the mean height of noctilucent clouds (NLC) derived from observation with the ALOMAR Rayleigh/Mie/Raman lidar at the same site. To investigate the layering processes microphysical model simulations under the influence of tidal and gravity waves were performed. In the presence of long period gravity waves, these model investigations predict an enhanced formation of multiple PMSE layer structures, where the lower layer is a consequence of the occurrence of the largest particles at the bottom of the ice cloud. This explains the coincidence of the lowermost PMSE layers and NLC. During periods with enhanced amplitudes of the semidiurnal tide, the observed NLC and PMSE show pronounced tidal structures comparable to the results of corresponding microphysical simulations. At periods with short period gravity waves there is a tendency for a decreasing occurrence of NLC and for variable weak PMSE structures.
- ItemLong-term behavior of the concentration of the minor constituents in the mesosphere-a model study(Göttingen : Copernicus, 2009) Grygalashvyly, M.; Sonnemann, G.R.; Hartogh, P.We investigate the influence the rising concentrations of methane, nitrous oxide and carbon dioxide which have occurred since the pre-industrial era, have had on the chemistry of the mesosphere. For this investigation we use our global 3-D-model COMMA-IAP which was designed for the exploration of the MLT-region and in particular the extended mesopause region. Assumptions and approximations for the trends in the Lyman-flux (needed for the water vapor dissociation rate), methane and the water vapor mixing ratio at the hygropause are necessary to accomplish this study. To approximate the solar Lyman-α flux back to the pre-industrial time, we derived a quadratic fit using the sunspot number record which extends back to 1749 and is the only solar proxy available for the Lyman-α flux prior to 1947. We assume that methane increases with a constant growth rate from the pre-industrial era to the present. An unsolved problem for the model calculations consists of how the water vapor mixing ratio at the hygropause should be specified during this period. We assume that the hygropause was dryer during pre-industrial times than the present. As a consequence of methane oxidation, the model simulation indicates that the middle atmosphere has become more humid as a result of the rising methane concentration, but with some dependence on height and with a small time delay of few years. The solar influence on the water vapor mixing ratio is insignificant below about 80 km in summer high latitudes, but becomes increasingly more important above this altitude. The enhanced water vapor concentration increasesthe hydrogen radical concentration and reduces the mesospheric ozone. A second region of stronger ozone decrease is located in the vicinity of the stratopause. Increases in CO2 concentration enhance slightly the concentration of CO in the mesosphere. However, its influence upon the chemistry is small and its main effect is connected with a cooling of the upper atmosphere. The long-term behavior of water vapor is discussed in particular with respect to its impact on the NLC region.
- ItemOn the efficiency of rocket-borne particle detection in the mesosphere(München : European Geopyhsical Union, 2007) Hedin, J.; Gumbel, J.; Rapp, M.Meteoric smoke particles have been proposed as a key player in the formation and evolution of mesospheric phenomena. Despite their apparent importance still very little is known about these particles. Important questions concern the smoke number density and size distribution as a function of altitude as well as the fraction of charged particles. Sounding rockets are used to measure smoke in situ, but aerodynamics has remained a major challenge. Basically, the small smoke particles tend to follow the gas flow around the payload rather than reaching the detector if aerodynamics is not considered carefully in the detector design. So far only indirect evidence for the existence of meteoric smoke has been available from measurements of heavy charge carriers. Quantitative ways are needed that relate these measured particle population to the atmospheric particle population. This requires in particular knowledge about the size-dependent, altitude-dependent and charge-dependent detection efficiency for a given instrument. In this paper, we investigate the aerodynamics for a typical electrostatic detector design. We first quantify the flow field of the background gas, then introduce particles in the flow field and determine their trajectories around the payload structure. We use two different models to trace particles in the flow field, a Continuous motion model and a Brownian motion model. Brownian motion is shown to be of basic importance for the smallest particles. Detection efficiencies are determined for three detector designs, including two with ventilation holes to allow airflow through the detector. Results from this investigation show that rocket-borne smoke detection with conventional detectors is largely limited to altitudes above 75 km. The flow through a ventilated detector has to be relatively large in order to significantly improve the detection efficiency.
- ItemSeasonal variations in the horizontal wind structure from 0-100 km above Rothera station, Antarctica (67° S, 68° W)(München : European Geopyhsical Union, 2005) Hibbins, R.E.; Shanklin, J.D.; Espy, P.J.; Jarvis, M.J.; Riggin, D.M.; Fritts, D.C.; Lübken, F.-J.A medium frequency spaced-antenna radar has been operating at Rothera station, Antarctica (67° S, 68° W) for two periods, between 1997-1998 and since 2002, measuring winds in the mesosphere and lower thermosphere. In this paper monthly mean winds are derived and presented along with three years of radiosonde balloon data for comparison with the HWM-93 model atmosphere and other high latitude southern hemisphere sites. The observed meridional winds are slightly more northwards than those predicted by the model above 80 km in the winter months and below 80 km in summer. In addition, the altitude of the summer time zero crossing of the zonal winds above the westward jet is overestimated by the model by up to 8 km. These data are then merged with the wind climatology obtained from falling sphere measurements made during the PORTA campaign at Rothera in early 1998 and the HWM-93 model atmosphere to generate a complete zonal wind climatology between 0 and 100 km as a benchmark for future studies at Rothera. A westwards (eastwards) maximum of 44 ms-1 at 67 km altitude occurs in mid December (62 ms-1 at 37 km in mid July). The 0 ms-1 wind contour reaches a maximum altitude of 90 km in mid November and a minimum altitude of 18 km in January extending into mid March at 75 km and early October at 76 km.
- ItemValidation of the Atmospheric Chemistry Experiment (ACE) version 2.2 temperature using ground-based and space-borne measurements(München : European Geopyhsical Union, 2008) Sica, R.J.; Izawa, M.R.M.; Walker, K.A.; Boone, C.; Petelina, S.V.; Argall, P.S.; Bernath, P.; Burns, G.B.; Catoire, V.; Collins, R.L.; Daffer, W.H.; De Clercq, C.; Fan, Z.Y.; Firanski, B.J.; French, W.J.R.; Gerard, P.; Gerding, M.; Granville, J.; Innis, J.L.; Keckhut, P.; Kerzenmacher, T.; Klekociuk, A.R.; Kyrö, E.; Lambert, J.C.; Llewellyn, E.J.; Manney, G.L.; McDermid, I.S.; Mizutani, K.; Murayama, Y.; Piccolo, C.; Raspollini, P.; Ridolfi, M.; Robert, C.; Steinbrecht, W.; Strawbridge, K.B.; Strong, K.; Stübi, R.; Thurairajah, B.An ensemble of space-borne and ground-based instruments has been used to evaluate the quality of the version 2.2 temperature retrievals from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS). The agreement of ACE-FTS temperatures with other sensors is typically better than 2 K in the stratosphere and upper troposphere and 5 K in the lower mesosphere. There is evidence of a systematic high bias (roughly 3–6 K) in the ACE-FTS temperatures in the mesosphere, and a possible systematic low bias (roughly 2 K) in ACE-FTS temperatures near 23 km. Some ACE-FTS temperature profiles exhibit unphysical oscillations, a problem fixed in preliminary comparisons with temperatures derived using the next version of the ACE-FTS retrieval software. Though these relatively large oscillations in temperature can be on the order of 10 K in the mesosphere, retrieved volume mixing ratio profiles typically vary by less than a percent or so. Statistical comparisons suggest these oscillations occur in about 10% of the retrieved profiles. Analysis from a set of coincident lidar measurements suggests that the random error in ACE-FTS version 2.2 temperatures has a lower limit of about ±2 K.
- ItemSmall scale density variations of electrons and charged particles in the vicinity of polar mesosphere summer echoes(München : European Geopyhsical Union, 2003) Rapp, M.; Lübken, F.-J.; Blix, T.A.We present small scale variations of electron number densities and particle charge number densities measured in situ in the presence of polar mesosphere summer echoes. It turns out that the small scale fluctuations of electrons and negatively charged particles show a strong anticorrelation down to the smallest scales observed. Comparing these small scale structures with the simultaneously measured radar signal to noise profile, we find that the radar profile is well described by the power spectral density of both electrons and charged particles at the radar half wavelength (=the Bragg scale). Finally, we consider the shape of the power spectra of the observed plasma fluctuations and find that both charged particles and electrons show spectra that can be explained in terms of either neutral air turbulence acting on the distribution of a low diffusivity tracer or the fossil remnants of a formerly active turbulent region. All these results are consistent with the theoretical ideas by Rapp and Lübken (2003) suggesting that PMSE can be explained by a combination of active and fossil neutral air turbulence acting on the large and heavy charged aerosol particles which are subsequently mirrored in the electron number density distribution that becomes visible to a VHF radar when small scale fluctuations are present.
- ItemThe thermal and dynamical state of the atmosphere during polar mesosphere winter echoes(München : European Geopyhsical Union, 2006) Lübken, F.-J.; Strelnikov, B.; Rapp, M.; Singer, W.; Latteck, R.; Brattli, A.; Hoppe, U.-P.; Friedrich, M.In January 2005, a total of 18 rockets were launched from the Andøya Rocket Range in Northern Norway (69° N) into strong VHF radar echoes called "Polar Mesosphere Winter Echoes" (PMWE). The echoes were observed in the lower and middle mesosphere during large solar proton fluxes. In general, PMWE occur much more seldom compared to their summer counterparts PMSE (typical occurrence rates at 69° N are 1–3% vs. 80%, respectively). Our in-situ measurements by falling sphere, chaff, and instrumented payloads provide detailed information about the thermal and dynamical state of the atmosphere and therefore allow an unprecedented study of the background atmosphere during PMWE. There are a number of independent observations indicating that neutral air turbulence has caused PMWE. Ion density fluctuations show a turbulence spectrum within PMWE and no fluctuations outside. Temperature lapse rates close to the adiabatic gradient are observed in the vicinity of PMWE indicating persistent turbulent mixing. The spectral broadening of radar echoes is consistent with turbulent velocity fluctuations. Turbulence also explains the mean occurrence height of PMWE (~68–75 km): viscosity increases rapidly with altitude and destroys any small scale fluctuations in the upper mesosphere, whereas electron densities are usually too low in the lower mesosphere to cause significant backscatter. The seasonal variation of echoes in the lower mesosphere is in agreement with a turbulence climatology derived from earlier sounding rocket flights. We have performed model calculations to study the radar backscatter from plasma fluctuations caused by neutral air turbulence. We find that volume reflectivities observed during PMWE are in quantitative agreement with theory. Apart from turbulence the most crucial requirement for PMWE is a sufficiently large number of electrons, for example produced by solar proton events. We have studied the sensitivity of the radar echo strength on various parameters, most important electron number density and turbulence intensity. Our observational and theoretical considerations do not provide any evidence that charged aerosol particles are needed to explain PMWE, in contrast to the summer echoes which owe their existence to charged ice particles.