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search.filters.applied.f.access: openAccess × Start date: 2017 × DDC: 600 × WGL Institute: MBI ×

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Now showing 1 - 10 of 28
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    Transient spin injection efficiencies at ferromagnet/metal interfaces
    (Weinheim : Wiley-VCH, 2022-10-19) Elliott, Peter; Eschenlohr, Andrea; Chen, Jinghao; Shallcross, Sam; Bovensiepen, Uwe; Dewhurst, John Kay; Sharma, Sangeeta
    Spin injection across interfaces driven by ultrashort optical pulses on femtosecond timescales constitutes a new way to design spintronics applications. Targeted utilization of this phenomenon requires knowledge of the efficiency of non-equilibrium spin injection. From a quantitative comparison of ab initio time-dependent density functional theory and interface-sensitive, time-resolved non-linear optical experiment, the spin injection efficiency (SIE) at the Co/Cu(001) interface is determined, and its microscopic origin, i.e., the influence of spin-orbit coupling and the interface electronic structure, is discussed. Moreover, we theoretically predict that the SIE at ferromagnetic–metal interfaces can be optimized through laser pulse and materials parameters, namely the fluence, pulse duration, and substrate material.
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    Generation of millijoule few-cycle pulses at 5 μm by indirect spectral shaping of the idler in an optical parametric chirped pulse amplifier
    (Washington, DC : Soc., 2018) Bock, Martin; Grafenstein, Lorenz von; Griebner, Uwe; Elsaesser, Thomas
    Spectral pulse shaping in a high-intensity midwave-infrared (MWIR) optical parametric chirped pulse amplifier (OPCPA) operating at 1 kHz repetition rate is reported. We successfully apply a MWIR spatial light modulator (SLM) for the generation of ultrashort idler pulses at 5 μm wavelength. Only bulk optics and active phase control of the 3.5 μm signal pulses via the SLM are employed for generating compressed idler pulses with a duration of 80 fs. The 80-fs pulse duration corresponds to less than five optical cycles at the central wavelength of 5.0 μm. The pulse energy amounts to 1.0 mJ, which translates into a peak power of 10 GW. The generated pulse parameters represent record values for high-intensity MWIR OPCPAs.
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    Element-specific magnetization dynamics of complex magnetic systems probed by ultrafast magneto-optical spectroscopy
    (Basel : MDPI, 2020) Korff Schmising, Clemens von; Willems, Felix; Sharma, Sangeeta; Yao, Kelvin; Borchert, Martin; Hennecke, Martin; Schick, Daniel; Radu, Ilie; Strüber, Christian; Engel, Dieter W.; Shokeen, Vishal; Buck, Jens; Bagschik, Kai; Viefhaus, Jens; Hartmann, Gregor; Manschwetus, Bastian; Grunewald, Soeren; Düsterer, Stefan; Jal, Emmanuelle; Vodungbo, Boris; Lüning, Jan; Eisebitt, Stefan
    The vision to manipulate and control magnetism with light is driven on the one hand by fundamental questions of direct and indirect photon-spin interactions, and on the other hand by the necessity to cope with ever growing data volumes, requiring radically new approaches on how to write, read and process information. Here, we present two complementary experimental geometries to access the element-specific magnetization dynamics of complex magnetic systems via ultrafast magneto-optical spectroscopy in the extreme ultraviolet spectral range. First, we employ linearly polarized radiation of a free electron laser facility to demonstrate decoupled dynamics of the two sublattices of an FeGd alloy, a prerequisite for all-optical magnetization switching. Second, we use circularly polarized radiation generated in a laboratory-based high harmonic generation setup to show optical inter-site spin transfer in a CoPt alloy, a mechanism which only very recently has been predicted to mediate ultrafast metamagnetic phase transitions. © 2020 by the authors. Licensee MDPI, Basel, Switzerland.
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    Ultrashort vortex pulses with controlled spectral gouy rotation
    (Basel : MDPI, 2020) Liebmann, Max; Treffer, Alexander; Bock, Martin; Wallrabe, Ulrike; Grunwald, Ruediger
    Recently, the spatio-spectral propagation dynamic of ultrashort-pulsed vortex beams was demonstrated by 2D mapping of spectral moments. The rotation of characteristic anomalies, so-called "spectral eyes", was explained by wavelength-dependent Gouy phase shift. Controlling of this spectral rotation is essential for specific applications, e.g., communication and processing. Here, we report on advanced concepts for spectral rotational control and related first-proof-of-principle experiments. The speed of rotation of spectral eyes during propagation is shown to be essentially determined by angular and spectral parameters. The performance of fixed diffractive optical elements (DOE) and programmable liquid-crystal-on silicon spatial light modulators (LCoS-SLMs) that act as spiral phase gratings (SPG) or spiral phase plates (SPP) is compared. The approach is extended to radially chirped SPGs inducing axially variable angular velocity. The generation of time-dependent orbital angular momentum (self-torque) by superimposing multiple vortex pulses is proposed. © 2020 by the authors.
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    Application of Matched-Filter Concepts to Unbiased Selection of Data in Pump-Probe Experiments with Free Electron Lasers
    (Basel : MDPI, 2017-06-16) Callegari, Carlo; Takanashi, Tsukasa; Fukuzawa, Hironobu; Motomura, Koji; Iablonskyi, Denys; Kumagai, Yoshiaki; Mondal, Subhendu; Tachibana, Tetsuya; Nagaya, Kiyonobu; Nishiyama, Toshiyuki; Matsunami, Kenji; Johnsson, Per; Piseri, Paolo; Sansone, Giuseppe; Dubrouil, Antoine; Reduzzi, Maurizio; Carpeggiani, Paolo; Vozzi, Caterina; Devetta, Michele; Faccialà, Davide; Calegari, Francesca; Castrovilli, Mattea; Coreno, Marcello; Alagia, Michele; Schütte, Bernd; Berrah, Nora; Plekan, Oksana; Finetti, Paola; Ferrari, Eugenio; Prince, Kevin; Ueda, Kiyoshi
    Pump-probe experiments are commonly used at Free Electron Lasers (FEL) to elucidate the femtosecond dynamics of atoms, molecules, clusters, liquids and solids. Maximizing the signal-to-noise ratio of the measurements is often a primary need of the experiment, and the aggregation of repeated, rapid, scans of the pump-probe delay is preferable to a single long-lasting scan. The limited availability of beamtime makes it impractical to repeat measurements indiscriminately, and the large, rapid flow of single-shot data that need to be processed and aggregated into a dataset, makes it difficult to assess the quality of a measurement in real time. In post-analysis it is then necessary to devise unbiased criteria to select or reject datasets, and to assign the weight with which they enter the analysis. One such case was the measurement of the lifetime of Intermolecular Coulombic Decay in the weakly-bound neon dimer. We report on the method we used to accomplish this goal for the pump-probe delay scans that constitute the core of the measurement; namely we report on the use of simple auto- and cross-correlation techniques based on the general concept of “matched filter”. We are able to unambiguously assess the signal-to-noise ratio (SNR) of each scan, which then becomes the weight with which a scan enters the average of multiple scans. We also observe a clear gap in the values of SNR, and we discard all the scans below a SNR of 0.45. We are able to generate an average delay scan profile, suitable for further analysis: in our previous work we used it for comparison with theory. Here we argue that the method is sufficiently simple and devoid of human action to be applicable not only in post-analysis, but also for the real-time assessment of the quality of a dataset.
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    Monitoring of evolving laser induced periodic surface structures
    (Basel : MDPI, 2019) Lübcke, Andrea; Pápa, Zsuzsanna; Schnürer, Matthias
    Laser induced periodic surface structures (LIPSS) are generated on titanium and silicon nitride surfaces by multiple femtosecond laser pulses. An optical imaging system is used to observe the backscattered light during the patterning process. A characteristic fringe pattern in the backscattered light is observed and evidences the surface modification. Experiments are complemented by finite difference time domain numerical simulations which clearly show that the periodic surface modulation leads to characteristic modulations in the coherently scattered light field. It is proposed that these characteristic fringe pattern can be used as a very fast and low-cost monitor of LIPSS formation formation during the manufacturing process. © 2019 by the authors.
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    Micro Fresnel mirror array with individual mirror control
    (Bristol : IOP Publ., 2020) Poyyathuruthy Bruno, Binal; Schütze, Robert; Grunwald, Ruediger; Wallrabe, Ulrike
    We present the design and fabrication of a miniaturized array of piezoelectrically actuated high speed Fresnel mirrors with individual mirror control. These Fresnel mirrors can be used to generate propagation invariant and self-healing interference patterns. The mirrors are actuated using piezobimorph actuators, and the consequent change of the tilting angle of the mirrors changes the fringe spacing of the interference pattern generated. The array consists of four Fresnel mirrors each having an area of 2 × 2 mm2 arranged in a 2x2 configuration. The device, optimized using FEM simulations, is able to achieve maximum mirror deflections of 15 mrad, and has a resonance frequency of 28 kHz.
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    Correlated electronic decay in expanding clusters triggered by intense XUV pulses from a Free-Electron-Laser
    (London : Nature Publishing Group, 2017) Oelze, Tim; Schütte, Bernd; Müller, Maria; Müller, Jan P.; Wieland, Marek; Frühling, Ulrike; Drescher, Markus; Al-Shemmary, Alaa; Golz, Torsten; Stojanovic, Nikola; Krikunova, Maria
    Irradiation of nanoscale clusters and large molecules with intense laser pulses transforms them into highly-excited non- equilibrium states. The dynamics of intense laser-cluster interaction is encoded in electron kinetic energy spectra, which contain signatures of direct photoelectron emission as well as emission of thermalized nanoplasma electrons. In this work we report on a so far not observed spectrally narrow bound state signature in the electron kinetic energy spectra from mixed Xe core - Ar shell clusters ionized by intense extreme-ultraviolet (XUV) pulses from a free-electron-laser. This signature is attributed to the correlated electronic decay (CED) process, in which an excited atom relaxes and the excess energy is used to ionize the same or another excited atom or a nanoplasma electron. By applying the terahertz field streaking principle we demonstrate that CED-electrons are emitted at least a few picoseconds after the ionizing XUV pulse has ended. Following the recent finding of CED in clusters ionized by intense near-infrared laser pulses, our observation of CED in the XUV range suggests that this process is of general relevance for the relaxation dynamics in laser produced nanoplasmas.
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    Switchable plasmonic routers controlled by external magnetic fields by using magneto-plasmonic waveguides
    (London : Nature Publishing Group, 2018) Ho, Kum-Song; Im, Song-Jin; Pae, Ji-Song; Ri, Chol-Song; Han, Yong-Ha; Herrmann, Joachim
    We analytically and numerically investigate magneto-plasmons in metal films surrounded by a ferromagnetic dielectric. In such waveguide using a metal film with a thickness exceeding the Skin depth, an external magnetic field in the transverse direction can induce a significant spatial asymmetry of mode distribution. Superposition of the odd and the even asymmetric modes over a distance leads to a concentration of the energy on one interface which is switched to the other interface by the magnetic field reversal. The requested magnitude of magnetization is exponentially reduced with the increase of the metal film thickness. Based on this phenomenon, we propose a waveguide-integrated magnetically controlled switchable plasmonic routers with 99-%-high contrast within the optical bandwidth of tens of THz. This configuration can also operate as a magneto-plasmonic modulator.
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    Cationic double K-hole pre-edge states of CS2 and SF6
    (London : Nature Publishing Group, 2017) Feifel, R.; Eland, J.H.D.; Carniato, S.; Selles, P.; Püttner, R.; Koulentianos, D.; Marchenko, T.; Journel, L.; Guillemin, R.; Goldsztejn, G.; Travnikova, O.; Ismail, I.; Miranda, B. Cunha de; Lago, A.F.; Céolin, D.; Lablanquie, P.; Penent, F.; Piancastelli, M.N.; Simon, M.
    Recent advances in X-ray instrumentation have made it possible to measure the spectra of an essentially unexplored class of electronic states associated with double inner-shell vacancies. Using the technique of single electron spectroscopy, spectra of states in CS2 and SF6 with a double hole in the K-shell and one electron exited to a normally unoccupied orbital have been obtained. The spectra are interpreted with the aid of a high-level theoretical model giving excellent agreement with the experiment. The results shed new light on the important distinction between direct and conjugate shake-up in a molecular context. In particular, systematic similarities and differences between pre-edge states near single core holes investigated in X-ray absorption spectra and the corresponding states near double core holes studied here are brought out.