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- ItemA new model of meteoric calcium in the mesosphere and lower thermosphere(Katlenburg-Lindau : EGU, 2018-10-16) Plane, John M. C.; Feng, Wuhu; Gómez Martín, Juan Carlos; Gerding, Michael; Raizada, ShikhaMeteoric ablation produces layers of metal atoms in the mesosphere and lower thermosphere (MLT). It has been known for more than 30 years that the Ca atom layer is depleted by over 2 orders of magnitude compared with Na, despite these elements having nearly the same elemental abundance in chondritic meteorites. In contrast, the Ca+ ion abundance is depleted by less than a factor of 10. To explain these observations, a large database of neutral and ion–molecule reaction kinetics of Ca species, measured over the past decade, was incorporated into the Whole Atmosphere Community Climate Model (WACCM). A new meteoric input function for Ca and Na, derived using a chemical ablation model that has been tested experimentally with a Meteoric Ablation Simulator, shows that Ca ablates almost 1 order of magnitude less efficiently than Na. WACCM-Ca simulates the seasonal Ca layer satisfactorily when compared with lidar observations, but tends to overestimate Ca+ measurements made by rocket mass spectrometry and lidar. A key finding is that CaOH and CaCO3 are very stable reservoir species because they are involved in essentially closed reaction cycles with O2 and O. This has been demonstrated experimentally for CaOH, and in this study for CaCO3 using electronic structure and statistical rate theory. Most of the neutral Ca is therefore locked in these reservoirs, enabling rapid loss through polymerization into meteoric smoke particles, and this explains the extreme depletion of Ca.
- ItemSolar 27-day signatures in standard phase height measurements above central Europe(Katlenburg-Lindau : EGU, 2019) von Savigny, Christian; Peters, Dieter H.W.; Entzian, GünterWe report on the effect of solar variability at the 27-day and the 11-year timescales on standard phase heightmeasurements in the ionospheric D region carried out in cen-tral Europe. Standard phase height corresponds to the re-flection height of radio waves (for constant solar zenith dis-tance) in the ionosphere near 80 km altitude, where NO isionized by solar Lyman-αradiation. Using the superposedepoch analysis (SEA) method, we extract statistically highlysignificant solar 27-day signatures in standard phase heights.The 27-day signatures are roughly inversely correlated to so-lar proxies, such as the F10.7 cm radio flux or the Lyman-αflux. The sensitivity of standard phase height change to so-lar forcing at the 27-day timescale is found to be in goodagreement with the sensitivity for the 11-year solar cycle,suggesting similar underlying mechanisms. The amplitude ofthe 27-day signature in standard phase height is larger duringsolar minimum than during solar maximum, indicating thatthe signature is not only driven by photoionization of NO. Weidentified statistical evidence for an influence of ultra-longplanetary waves on the quasi 27-day signature of standardphase height in winters of solar minimum periods.
- ItemRetrieval of ice-nucleating particle concentrations from lidar observations and comparison with UAV in situ measurements(Katlenburg-Lindau : EGU, 2019) Marinou, Eleni; Tesche, Matthias; Nenes, Athanasios; Ansmann, Albert; Schrod, Jann; Mamali, Dimitra; Tsekeri, Alexandra; Pikridas, Michael; Baars, Holger; Engelmann, Ronny; Voudouri, Kalliopi-Artemis; Solomos, Stavros; Sciare, Jean; Groß, Silke; Ewald, Florian; Amiridis, VassilisAerosols that are efficient ice-nucleating particles (INPs) are crucial for the formation of cloud ice via heterogeneous nucleation in the atmosphere. The distribution of INPs on a large spatial scale and as a function of height determines their impact on clouds and climate. However, in situ measurements of INPs provide sparse coverage over space and time. A promising approach to address this gap is to retrieve INP concentration profiles by combining particle concentration profiles derived by lidar measurements with INP efficiency parameterizations for different freezing mechanisms (immersion freezing, deposition nucleation). Here, we assess the feasibility of this new method for both ground-based and spaceborne lidar measurements, using in situ observations collected with unmanned aerial vehicles (UAVs) and subsequently analyzed with the FRIDGE (FRankfurt Ice nucleation Deposition freezinG Experiment) INP counter from an experimental campaign at Cyprus in April 2016. Analyzing five case studies we calculated the cloud-relevant particle number concentrations using lidar measurements (n250,dry with an uncertainty of 20 % to 40 % and Sdry with an uncertainty of 30 % to 50 %), and we assessed the suitability of the different INP parameterizations with respect to the temperature range and the type of particles considered. Specifically, our analysis suggests that our calculations using the parameterization of Ullrich et al. (2017) (applicable for the temperature range −50 to −33 ∘C) agree within 1 order of magnitude with the in situ observations of nINP; thus, the parameterization of Ullrich et al. (2017) can efficiently address the deposition nucleation pathway in dust-dominated environments. Additionally, our calculations using the combination of the parameterizations of DeMott et al. (2015, 2010) (applicable for the temperature range −35 to −9 ∘C) agree within 2 orders of magnitude with the in situ observations of INP concentrations (nINP) and can thus efficiently address the immersion/condensation pathway of dust and nondust particles. The same conclusion is derived from the compilation of the parameterizations of DeMott et al. (2015) for dust and Ullrich et al. (2017) for soot.
- ItemResults from the validation campaign of the ozone radiometer GROMOS-C at the NDACC station of Réunion island(Katlenburg-Lindau : EGU, 2016) Fernandez, Susana; Rüfenacht, Rolf; Kämpfer, Niklaus; Portafaix, Thierry; Posny, Françoise; Payen, GuillaumeOzone performs a key role in the middle atmosphere and its monitoring is thus necessary. At the Institute of Applied Physics of the University of Bern, Switzerland, we built a new ground-based microwave radiometer, GROMOS-C (GRound based Ozone MOnitoring System for Campaigns). It has a compact design and can be operated remotely with very little maintenance requirements, being therefore suitable for remote deployments. It has been conceived to measure the vertical distribution of ozone in the middle atmosphere, by observing pressure-broadened emission spectra at a frequency of 110.836 GHz. In addition, meridional and zonal wind profiles can be retrieved, based on the Doppler shift of the ozone line measured in the four directions of observation (north, east, south and west). In June 2014 the radiometer was installed at the Maïdo observatory, on Réunion island (21.2° S, 55.5° E). High-resolution ozone spectra were recorded continuously over 7 months. Vertical profiles of ozone have been retrieved through an optimal estimation inversion process, using the Atmospheric Radiative Transfer Simulator ARTS2 as the forward model. The validation is performed against ozone profiles from the Microwave Limb Sounder (MLS) on the Aura satellite, the ozone lidar located at the observatory and with ozone profiles from weekly radiosondes. Zonal and meridional winds retrieved from GROMOS-C data are validated against another wind radiometer located in situ, WIRA. In addition, we compare both ozone and winds with ECMWF (European Centre for Medium-Range Weather Forecasts) model data. Results show that GROMOS-C provides reliable ozone profiles between 30 and 0.02 hPa. The comparison with lidar profiles shows a very good agreement at all levels. The accordance with the MLS data set is within 5 % for pressure levels between 25 and 0.2 hPa. GROMOS-C's wind profiles are in good agreement with the observations by WIRA and with the model data, differences are below 5 m s−1 for both.
- ItemNOy production, ozone loss and changes in net radiative heating due to energetic particle precipitation in 2002–2010(Katlenburg-Lindau : EGU, 2018-1-29) Sinnhuber, Miriam; Berger, Uwe; Funke, Bernd; Nieder, Holger; Reddmann, Thomas; Stiller, Gabriele; Versick, Stefan; von Clarmann, Thomas; Wissing, Jan MaikWe analyze the impact of energetic particle precipitation on the stratospheric nitrogen budget, ozone abundances and net radiative heating using results from three global chemistry-climate models considering solar protons and geomagnetic forcing due to auroral or radiation belt electrons. Two of the models cover the atmosphere up to the lower thermosphere, the source region of auroral NO production. Geomagnetic forcing in these models is included by prescribed ionization rates. One model reaches up to about 80 km, and geomagnetic forcing is included by applying an upper boundary condition of auroral NO mixing ratios parameterized as a function of geomagnetic activity. Despite the differences in the implementation of the particle effect, the resulting modeled NOy in the upper mesosphere agrees well between all three models, demonstrating that geomagnetic forcing is represented in a consistent way either by prescribing ionization rates or by prescribing NOy at the model top. Compared with observations of stratospheric and mesospheric NOy from the Michelson Interferometer for Passive Atmospheric Sounding (MIPAS) instrument for the years 2002–2010, the model simulations reproduce the spatial pattern and temporal evolution well. However, after strong sudden stratospheric warmings, particle-induced NOy is underestimated by both high-top models, and after the solar proton event in October 2003, NOy is overestimated by all three models. Model results indicate that the large solar proton event in October 2003 contributed about 1–2 Gmol (109 mol) NOy per hemisphere to the stratospheric NOy budget, while downwelling of auroral NOx from the upper mesosphere and lower thermosphere contributes up to 4 Gmol NOy. Accumulation over time leads to a constant particle-induced background of about 0.5–1 Gmol per hemisphere during solar minimum, and up to 2 Gmol per hemisphere during solar maximum. Related negative anomalies of ozone are predicted by the models in nearly every polar winter, ranging from 10–50 % during solar maximum to 2–10 % during solar minimum. Ozone loss continues throughout polar summer after strong solar proton events in the Southern Hemisphere and after large sudden stratospheric warmings in the Northern Hemisphere. During mid-winter, the ozone loss causes a reduction of the infrared radiative cooling, i.e., a positive change of the net radiative heating (effective warming), in agreement with analyses of geomagnetic forcing in stratospheric temperatures which show a warming in the late winter upper stratosphere. In late winter and spring, the sign of the net radiative heating change turns to negative (effective cooling). This spring-time cooling lasts well into summer and continues until the following autumn after large solar proton events in the Southern Hemisphere, and after sudden stratospheric warmings in the Northern Hemisphere.
- ItemGravity waves excited during a minor sudden stratospheric warming(Katlenburg-Lindau : EGU, 2018-9-7) Dörnbrack, Andreas; Gisinger, Sonja; Kaifler, Natalie; Portele, Tanja Christina; Bramberger, Martina; Rapp, Markus; Gerding, Michael; Söder, Jens; Žagar, Nedjeljka; Jelić, DamjanAn exceptionally deep upper-air sounding launched from Kiruna airport (67.82∘ N, 20.33∘ E) on 30 January 2016 stimulated the current investigation of internal gravity waves excited during a minor sudden stratospheric warming (SSW) in the Arctic winter 2015/16. The analysis of the radiosonde profile revealed large kinetic and potential energies in the upper stratosphere without any simultaneous enhancement of upper tropospheric and lower stratospheric values. Upward-propagating inertia-gravity waves in the upper stratosphere and downward-propagating modes in the lower stratosphere indicated a region of gravity wave generation in the stratosphere. Two-dimensional wavelet analysis was applied to vertical time series of temperature fluctuations in order to determine the vertical propagation direction of the stratospheric gravity waves in 1-hourly high-resolution meteorological analyses and short-term forecasts. The separation of upward- and downward-propagating waves provided further evidence for a stratospheric source of gravity waves. The scale-dependent decomposition of the flow into a balanced component and inertia-gravity waves showed that coherent wave packets preferentially occurred at the inner edge of the Arctic polar vortex where a sub-vortex formed during the minor SSW.
- ItemQuasi 18 h wave activity in ground-based observed mesospheric H2O over Bern, Switzerland(Katlenburg-Lindau : EGU, 2017-12-18) Lainer, Martin; Hocke, Klemens; Rüfenacht, Rolf; Kämpfer, NiklausObservations of oscillations in the abundance of middle-atmospheric trace gases can provide insight into the dynamics of the middle atmosphere. Long-term, high-temporal-resolution and continuous measurements of dynamical tracers within the strato- and mesosphere are rare but would facilitate better understanding of the impact of atmospheric waves on the middle atmosphere. Here we report on water vapor measurements from the ground-based microwave radiometer MIAWARA (MIddle Atmospheric WAter vapor RAdiometer) located close to Bern during two winter periods of 6 months from October to March. Oscillations with periods between 6 and 30 h are analyzed in the pressure range 0.02–2 hPa. Seven out of 12 months have the highest wave amplitudes between 15 and 21 h periods in the mesosphere above 0.1 hPa. The quasi 18 h wave signature in the water vapor tracer is studied in more detail by analyzing its temporal evolution in the mesosphere up to an altitude of 75 km. Eighteen-hour oscillations in midlatitude zonal wind observations from the microwave Doppler wind radiometer WIRA (WInd RAdiometer) could be identified within the pressure range 0.1–1 hPa during an ARISE (Atmospheric dynamics Research InfraStructure in Europe)-affiliated measurement campaign at the Observatoire de Haute-Provence (355 km from Bern) in France in 2013. The origin of the observed upper-mesospheric quasi 18 h oscillations is uncertain and could not be determined with our available data sets. Possible drivers could be low-frequency inertia-gravity waves or a nonlinear wave–wave interaction between the quasi 2-day wave and the diurnal tide.
- ItemImpact of particle shape on the morphology of noctilucent clouds(Katlenburg-Lindau : EGU, 2015) Kiliani, J.; Baumgarten, G.; Lübken, F.-J.; Berger, U.Noctilucent clouds (NLCs) occur during summer in the polar region at altitudes around 83 km. They consist of ice particles with a typical size around 50 nm. The shape of NLC particles is less well known but is important both for interpreting optical measurements and modeling ice cloud characteristics. In this paper, NLC modeling of microphysics and optics is adapted to use cylindrical instead of spherical particle shape. The optical properties of the resulting ice clouds are compared directly to NLC three-color measurements by the Arctic Lidar Observatory for Middle Atmosphere Research (ALOMAR) Rayleigh/Mie/Raman (RMR) lidar between 1998 and 2014. Shape distributions including both needle- and disc-shaped particles are consistent with lidar measurements. The best agreement occurs if disc shapes are 60 % more common than needles, with a mean axis ratio of 2.8. Cylindrical particles cause stronger ice clouds on average than spherical shapes with an increase of backscatter at 532 nm by ≈ 30 % and about 20 % in ice mass density. This difference is less pronounced for bright than for weak ice clouds. Cylindrical shapes also cause NLCs to have larger but a smaller number of ice particles than for spherical shapes.
- ItemOzone–gravity wave interaction in the upper stratosphere/lower mesosphere(Katlenburg-Lindau : EGU, 2022) Gabriel, AxelThe increase in amplitudes of upward propagating gravity waves (GWs) with height due to decreasing density is usually described by exponential growth. Recent measurements show some evidence that the upper stratospheric/lower mesospheric gravity wave potential energy density (GWPED) increases more strongly during the daytime than during the nighttime. This paper suggests that ozone-gravity wave interaction can principally produce such a phenomenon. The coupling between ozone-photochemistry and temperature is particularly strong in the upper stratosphere where the time-mean ozone mixing ratio decreases with height. Therefore, an initial ascent (or descent) of an air parcel must lead to an increase (or decrease) in ozone and in the heating rate compared to the environment, and, hence, to an amplification of the initial wave perturbation. Standard solutions of upward propagating GWs with linear ozone-temperature coupling are formulated, suggesting amplitude amplifications at a specific level during daytime of 5ĝ€¯% to 15ĝ€¯% for low-frequency GWs (periods ≥4ĝ€¯h), as a function of the intrinsic frequency which decreases if ozone-temperature coupling is included. Subsequently, the cumulative amplification during the upward level-by-level propagation leads to much stronger GW amplitudes at upper mesospheric altitudes, i.e., for single low-frequency GWs, up to a factor of 1.5 to 3 in the temperature perturbations and 3 to 9 in the GWPED increasing from summer low to polar latitudes. Consequently, the mean GWPED of a representative range of mesoscale GWs (horizontal wavelengths between 200 and 1100ĝ€¯km, vertical wavelengths between 3 and 9ĝ€¯km) is stronger by a factor of 1.7 to 3.4 (2 to 50ĝ€¯Jĝ€¯kg-1, or 2ĝ€¯% to 50ĝ€¯% in relation to the observed order of 100ĝ€¯Jĝ€¯kg-1, assuming initial GW perturbations of 1 to 2ĝ€¯K in the middle stratosphere). Conclusively, the identified process might be an important component in the middle atmospheric circulation, which has not been considered up to now.
- ItemGround-based noontime D-region electron density climatology over northern Norway(Katlenburg-Lindau : EGU, 2023) Renkwitz, Toralf; Sivakandan, Mani; Jaen, Juliana; Singer, WernerThe bottom part of the Earth's ionosphere is the so-called D region, which is typically less dense than the upper regions. Despite the comparably lower electron density, the ionization state of the D region has a significant influence on signal absorption for propagating lower to medium radio frequencies. We present local noon climatologies of electron densities in the upper middle atmosphere (50-90km) at high latitudes as observed by an active radar experiment. The radar measurements cover 9 years (2014-2022) from the solar maximum of cycle 24 to the beginning of cycle 25. Reliable electron densities are derived by employing signal processing, applying interferometry methods, and applying the Faraday-International Reference Ionosphere (FIRI) model. For all years a consistent spring-fall asymmetry of the electron density pattern with a gradual increase during summer as well as a sharp decrease at the beginning of October was found. These findings are consistent with very low frequency (VLF) studies showing equivalent signatures for nearby propagation paths. It is suggested that the meridional circulation associated with downwelling in winter could cause enhanced electron densities through NO transport. However, this mechanism can not explain the reduction in electron density in early October.