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- ItemRadiative budget and cloud radiative effect over the Atlantic from ship-based observations(München : European Geopyhsical Union, 2012) Kalisch, J.; Macke, A.The aim of this study is to determine cloud-type resolved cloud radiative budgets and cloud radiative effects from surface measurements of broadband radiative fluxes over the Atlantic Ocean. Furthermore, based on simultaneous observations of the state of the cloudy atmosphere, a radiative closure study has been performed by means of the ECHAM5 single column model in order to identify the model's ability to realistically reproduce the effects of clouds on the climate system. An extensive database of radiative and atmospheric measurements has been established along five meridional cruises of the German research icebreaker Polarstern. Besides pyranometer and pyrgeometer for downward broadband solar and thermal radiative fluxes, a sky imager and a microwave radiometer have been utilized to determine cloud fraction and cloud type on the one hand and temperature and humidity profiles as well as liquid water path for warm non-precipitating clouds on the other hand. Averaged over all cruise tracks, we obtain a total net (solar + thermal) radiative flux of 144 W m−2 that is dominated by the solar component. In general, the solar contribution is large for cirrus clouds and small for stratus clouds. No significant meridional dependencies were found for the surface radiation budgets and cloud effects. The strongest surface longwave cloud effects were shown in the presence of low level clouds. Clouds with a high optical density induce strong negative solar radiative effects under high solar altitudes. The mean surface net cloud radiative effect is −33 W m−2. For the purpose of quickly estimating the mean surface longwave, shortwave and net cloud effects in moderate, subtropical and tropical climate regimes, a new parameterisation was created, considering the total cloud amount and the solar zenith angle. The ECHAM5 single column model provides a surface net cloud effect that is more cooling by 17 W m−2 compared to the radiation observations. This overestimation in solar cooling is mostly caused by the shortwave impact of convective clouds. The latter show a large overestimation in solar cooling of up to 114 W m−2. Mean cloud radiative effects of cirrus and stratus clouds were simulated close to the observations.
- ItemIn-cloud sulfate addition to single particles resolved with sulfur isotope analysis during HCCT-2010(München : European Geopyhsical Union, 2014) Harris, E.; Sinha, B.; van Pinxteren, D.; Schneider, J.; Poulain, L.; Collett, J.; D'Anna, B.; Fahlbusch, B.; Foley, S.; Fomba, K.W.; George, C.; Gnauk, T.; Henning, S.; Lee, T.; Mertes, S.; Roth, A.; Stratmann, F.; Borrmann, S.; Hoppe, P.; Herrmann, H.In-cloud production of sulfate modifies aerosol size distribution, with important implications for the magnitude of indirect and direct aerosol cooling and the impact of SO2 emissions on the environment. We investigate which sulfate sources dominate the in-cloud addition of sulfate to different particle classes as an air parcel passes through an orographic cloud. Sulfate aerosol, SO2 and H2SO4 were collected upwind, in-cloud and downwind of an orographic cloud for three cloud measurement events during the Hill Cap Cloud Thuringia campaign in autumn 2010 (HCCT-2010). Combined SEM and NanoSIMS analysis of single particles allowed the δ34S of particulate sulfate to be resolved for particle size and type. The most important in-cloud SO2 oxidation pathway at HCCT-2010 was aqueous oxidation catalysed by transition metal ions (TMI catalysis), which was shown with single particle isotope analyses to occur primarily in cloud droplets nucleated on coarse mineral dust. In contrast, direct uptake of H2SO4 (g) and ultrafine particulate were the most important sources modifying fine mineral dust, increasing its hygroscopicity and facilitating activation. Sulfate addition to "mixed" particles (secondary organic and inorganic aerosol) and coated soot was dominated by in-cloud aqueous SO2 oxidation by H2O2 and direct uptake of H2SO4 (g) and ultrafine particle sulfate, depending on particle size mode and time of day. These results provide new insight into in-cloud sulfate production mechanisms, and show the importance of single particle measurements and models to accurately assess the environmental effects of cloud processing.
- ItemImmersion freezing of birch pollen washing water(München : European Geopyhsical Union, 2013) Augustin, S.; Wex, H.; Niedermeier, D.; Pummer, B.; Grothe, H.; Hartmann, S.; Tomsche, L.; Clauss, T.; Voigtländer, J.; Ignatius, K.; Stratmann, F.Birch pollen grains are known to be ice nucleating active biological particles. The ice nucleating activity has previously been tracked down to biological macromolecules that can be easily extracted from the pollen grains in water. In the present study, we investigated the immersion freezing behavior of these ice nucleating active (INA) macromolecules. Therefore we measured the frozen fractions of particles generated from birch pollen washing water as a function of temperature at the Leipzig Aerosol Cloud Interaction Simulator (LACIS). Two different birch pollen samples were considered, with one originating from Sweden and one from the Czech Republic. For the Czech and Swedish birch pollen samples, freezing was observed to start at −19 and −17 °C, respectively. The fraction of frozen droplets increased for both samples down to −24 °C. Further cooling did not increase the frozen fractions any more. Instead, a plateau formed at frozen fractions below 1. This fact could be used to determine the amount of INA macromolecules in the droplets examined here, which in turn allowed for the determination of nucleation rates for single INA macromolecules. The main differences between the Swedish birch pollen and the Czech birch pollen were obvious in the temperature range between −17 and −24 °C. In this range, a second plateau region could be seen for Swedish birch pollen. As we assume INA macromolecules to be the reason for the ice nucleation, we concluded that birch pollen is able to produce at least two different types of INA macromolecules. We were able to derive parameterizations for the heterogeneous nucleation rates for both INA macromolecule types, using two different methods: a simple exponential fit and the Soccer ball model. With these parameterization methods we were able to describe the ice nucleation behavior of single INA macromolecules from both the Czech and the Swedish birch pollen.
- ItemAsymmetry and uncertainties in biogeophysical climate-vegetation feedback over a range of CO2 forcings(München : European Geopyhsical Union, 2014) Willeit, M.; Ganopolski, A.; Feulner, G.Climate–vegetation feedback has the potential to significantly contribute to climate change, but little is known about its range of uncertainties. Here, using an Earth system model of intermediate complexity we address possible uncertainties in the strength of the biogeophysical climate–vegetation feedback using a single-model multi-physics ensemble. Equilibrium experiments with halving (140 ppm) and doubling (560 ppm) of CO2 give a contribution of the vegetation–climate feedback to global temperature change in the range −0.3 to −0.1 °C and −0.1 to 0.2 °C, respectively. There is an asymmetry between warming and cooling, with a larger, positive vegetation–climate feedback in the lower CO2 climate. Hotspots of climate–vegetation feedback are the boreal zone, the Amazon rainforest and the Sahara. Albedo parameterization is the dominant source of uncertainty in the subtropics and at high northern latitudes, while uncertainties in evapotranspiration are more relevant in the tropics. We analyse the separate impact of changes in stomatal conductance, leaf area index and vegetation dynamics on climate and we find that different processes are dominant in lower and higher CO2 worlds. The reduction in stomatal conductance gives the main contribution to temperature increase for a doubling of CO2, while dynamic vegetation is the dominant process in the CO2 halving experiments. Globally the climate–vegetation feedback is rather small compared to the sum of the fast climate feedbacks. However, it is comparable to the amplitude of the fast feedbacks at high northern latitudes where it can contribute considerably to polar amplification. The uncertainties in the climate–vegetation feedback are comparable to the multi-model spread of the fast climate feedbacks.
- ItemPolar middle atmosphere temperature climatology from Rayleigh lidar measurements at ALOMAR (69° N)(München : European Geopyhsical Union, 2008) Schöch, A.; Baumgarten, G.; Fiedler, J.Rayleigh lidar temperature profiles have been derived in the polar middle atmosphere from 834 measurements with the ALOMAR Rayleigh/Mie/Raman lidar (69.3° N, 16.0° E) in the years 1997–2005. Since our instrument is able to operate under full daylight conditions, the unique data set presented here extends over the entire year and covers the altitude region 30 km–85 km in winter and 30 km–65 km in summer. Comparisons of our lidar data set to reference atmospheres and ECMWF analyses show agreement within a few Kelvin in summer but in winter higher temperatures below 55 km and lower temperatures above by as much as 25 K, due likely to superior resolution of stratospheric warming and associated mesospheric cooling events. We also present a temperature climatology for the entire lower and middle atmosphere at 69° N obtained from a combination of lidar measurements, falling sphere measurements and ECMWF analyses. Day to day temperature variability in the lidar data is found to be largest in winter and smallest in summer.