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- ItemAnalyzing the causes and spatial pattern of the European 2003 carbon flux anomaly using seven models(München : European Geopyhsical Union, 2008) Vetter, M.; Churkina, G.; Jung, M.; Reichstein, M.; Zaehle, S.; Bondeau, A.; Chen, Y.; Ciais, P.; Feser, F.; Freibauer, A.; Geyer, R.; Jones, C.; Papale, D.; Tenhunen, J.; Tomelleri, E.; Trusilova, K.; Viovy, N.; Heimann, M.Globally, the year 2003 is associated with one of the largest atmospheric CO2 rises on record. In the same year, Europe experienced an anomalously strong flux of CO2 from the land to the atmosphere associated with an exceptionally dry and hot summer in Western and Central Europe. In this study we analyze the magnitude of this carbon flux anomaly and key driving ecosystem processes using simulations of seven terrestrial ecosystem models of different complexity and types (process-oriented and diagnostic). We address the following questions: (1) how large were deviations in the net European carbon flux in 2003 relative to a short-term baseline (1998–2002) and to longer-term variations in annual fluxes (1980 to 2005), (2) which European regions exhibited the largest changes in carbon fluxes during the growing season 2003, and (3) which ecosystem processes controlled the carbon balance anomaly . In most models the prominence of 2003 anomaly in carbon fluxes declined with lengthening of the reference period from one year to 16 years. The 2003 anomaly for annual net carbon fluxes ranged between 0.35 and –0.63 Pg C for a reference period of one year and between 0.17 and –0.37 Pg C for a reference period of 16 years for the whole Europe. In Western and Central Europe, the anomaly in simulated net ecosystem productivity (NEP) over the growing season in 2003 was outside the 1σ variance bound of the carbon flux anomalies for 1980–2005 in all models. The estimated anomaly in net carbon flux ranged between –42 and –158 Tg C for Western Europe and between 24 and –129 Tg C for Central Europe depending on the model used. All models responded to a dipole pattern of the climate anomaly in 2003. In Western and Central Europe NEP was reduced due to heat and drought. In contrast, lower than normal temperatures and higher air humidity decreased NEP over Northeastern Europe. While models agree on the sign of changes in simulated NEP and gross primary productivity in 2003 over Western and Central Europe, models diverge in the estimates of anomalies in ecosystem respiration. Except for two process models which simulate respiration increase, most models simulated a decrease in ecosystem respiration in 2003. The diagnostic models showed a weaker decrease in ecosystem respiration than the process-oriented models. Based on the multi-model simulations we estimated the total carbon flux anomaly over the 2003 growing season in Europe to range between –0.02 and –0.27 Pg C relative to the net carbon flux in 1998–2002.
- ItemAirborne observations of newly formed boundary layer aerosol particles under cloudy conditions(Katlenburg-Lindau : EGU, 2018) Altstädter, Barbara; Platis, Andreas; Jähn, Michael; Baars, Holger; Lückerath, Janine; Held, Andreas; Lampert, Astrid; Bange, Jens; Hermann, Markus; Wehner, BirgitThis study describes the appearance of ultrafine boundary layer aerosol particles under classical “non-favourable” conditions at the research site of TROPOS (Leibniz Institute for Tropospheric Research). Airborne measurements of meteorological and aerosol properties of the atmospheric boundary layer (ABL) were repeatedly performed with the unmanned aerial system ALADINA (Application of Light-weight Aircraft for Detecting IN-situ Aerosol) during three seasons between October 2013 and July 2015. More than 100 measurement flights were conducted on 23 different days with a total flight duration of 53 h. In 26 % of the cases, maxima of ultrafine particles were observed close to the inversion layer at altitudes between 400 and 600 m and the particles were rapidly mixed vertically and mainly transported downwards during short time intervals of cloud gaps. This study focuses on two measurement days affected by low-level stratocumulus clouds, but different wind directions (NE, SW) and minimal concentrations (< 4.6 µg m−3) of SO2, as a common indicator for precursor gases at ground. Taken from vertical profiles, the onset of clouds led to a non-linearity of humidity that resulted in an increased turbulence at the local-scale and caused fast nucleation (e.g. Bigg, 1997; Wehner et al., 2010), but in relation to rapid dilution of surrounding air, seen in sporadic clusters of ground data, so that ultrafine particles disappeared in the verticality. The typical “banana shape” (Heintzenberg et al., 2007) of new particle formation (NPF) and growth was not seen at ground and thus these days might not have been classified as NPF event days by pure surface studies.
- ItemCoupled and decoupled stratocumulus-topped boundary layers: turbulence properties(Katlenburg-Lindau : European Geosciences Union, 2021) Nowak, Jakub L.; Siebert, Holger; Szodry, Kai-Erik; Malinowski, Szymon P.We compare turbulence properties in coupled and decoupled marine stratocumulus-topped boundary layers (STBLs) using high-resolution in situ measurements performed by the helicopter-borne Airborne Cloud Turbulence Observation System (ACTOS) platform in the region of the eastern North Atlantic. The thermodynamically well-mixed coupled STBL was characterized by a comparable latent heat flux at the surface and in the cloud-top region, and substantially smaller sensible heat flux in the entire depth. Turbulence kinetic energy (TKE) was efficiently generated by buoyancy in the cloud and at the surface, and dissipated with comparable rate across the entire depth. Structure functions and power spectra of velocity fluctuations in the inertial range were reasonably consistent with the predictions of Kolmogorov theory. The turbulence was close to isotropic. In the decoupled STBL, decoupling was most obvious in humidity profiles. Heat fluxes and buoyant TKE production at the surface were similar to the coupled case. Around the transition level, latent heat flux decreased to zero and TKE was consumed by weak stability. In the cloud-top region, heat fluxes almost vanished and buoyancy production was significantly smaller than for the coupled case. The TKE dissipation rate inside the decoupled STBL varied between its sublayers. Structure functions and power spectra in the inertial range deviated from Kolmogorov scaling. This was more pronounced in the cloud and subcloud layer in comparison to the surface mixed layer. The turbulence was more anisotropic than in the coupled STBL, with horizontal fluctuations dominating. The degree of anisotropy was largest in the cloud and subcloud layer of the decoupled STBL. Integral length scales, of the order of 100gm in both cases, indicate turbulent eddies smaller than the depth of the coupled STBL or of the sublayers of the decoupled STBL. We hypothesize that turbulence produced in the cloud or close to the surface is redistributed across the entire coupled STBL but rather only inside the sublayers where it was generated in the case of the decoupled STBL. Scattered cumulus convection, developed below the stratocumulus base, may play a role in transport between those sublayers. © 2021 Jakub L. Nowak et al.
- ItemThe second ACTRIS inter-comparison (2016) for Aerosol Chemical Speciation Monitors (ACSM): Calibration protocols and instrument performance evaluations(Philadelphia, Pa.: Taylor & Francis, 2019) Freney, Evelyn; Zhang, Yunjiang; Croteau, Philip; Amodeo, Tanguy; Williams, Leah; Truong, François; Petit, Jean-Eudes; Sciare, Jean; Sarda-Esteve, Roland; Bonnaire, Nicolas; Arumae, Tarvo; Aurela, Minna; Bougiatioti, Aikaterini; Mihalopoulos, Nikolaos; Coz, Esther; Artinano, Begoña; Crenn, Vincent; Elste, Thomas; Heikkinen, Liine; Poulain, Laurent; Wiedensohler, Alfred; Herrmann, Hartmut; Priestman, Max; Alastuey, Andres; Stavroulas, Iasonas; Tobler, Anna; Vasilescu, Jeni; Zanca, Nicola; Canagaratna, Manjula; Carbone, Claudio; Flentje, Harald; Green, David; Maasikmets, Marek; Marmureanu, Luminita; Cruz Minguillon, Maria; Prevot, Andre S.H.; Gros, Valerie; Jayne, John; Favez, OlivierThis work describes results obtained from the 2016 Aerosol Chemical Speciation Monitor (ACSM) intercomparison exercise performed at the Aerosol Chemical Monitor Calibration Center (ACMCC, France). Fifteen quadrupole ACSMs (Q_ACSM) from the European Research Infrastructure for the observation of Aerosols, Clouds and Trace gases (ACTRIS) network were calibrated using a new procedure that acquires calibration data under the same operating conditions as those used during sampling and hence gets information representative of instrument performance. The new calibration procedure notably resulted in a decrease in the spread of the measured sulfate mass concentrations, improving the reproducibility of inorganic species measurements between ACSMs as well as the consistency with co-located independent instruments. Tested calibration procedures also allowed for the investigation of artifacts in individual instruments, such as the overestimation of m/z 44 from organic aerosol. This effect was quantified by the m/z (mass-to-charge) 44 to nitrate ratio measured during ammonium nitrate calibrations, with values ranging from 0.03 to 0.26, showing that it can be significant for some instruments. The fragmentation table correction previously proposed to account for this artifact was applied to the measurements acquired during this study. For some instruments (those with high artifacts), this fragmentation table adjustment led to an “overcorrection” of the f44 (m/z 44/Org) signal. This correction based on measurements made with pure NH4NO3, assumes that the magnitude of the artifact is independent of chemical composition. Using data acquired at different NH4NO3 mixing ratios (from solutions of NH4NO3 and (NH4)2SO4) we observe that the magnitude of the artifact varies as a function of composition. Here we applied an updated correction, dependent on the ambient NO3 mass fraction, which resulted in an improved agreement in organic signal among instruments. This work illustrates the benefits of integrating new calibration procedures and artifact corrections, but also highlights the benefits of these intercomparison exercises to continue to improve our knowledge of how these instruments operate, and assist us in interpreting atmospheric chemistry. © 2019, © 2019 Author(s). Published with license by Taylor & Francis Group, LLC.
- ItemEffects of climate model radiation, humidity and wind estimates on hydrological simulations(Chichester : John Wiley and Sons Ltd, 2012) Haddeland, I.; Heinke, J.; Voß, F.; Eisner, S.; Chen, C.; Hagemann, S.; Ludwig, F.Due to biases in the output of climate models, a bias correction is often needed to make the output suitable for use in hydrological simulations. In most cases only the temperature and precipitation values are bias corrected. However, often there are also biases in other variables such as radiation, humidity and wind speed. In this study we tested to what extent it is also needed to bias correct these variables. Responses to radiation, humidity and wind estimates from two climate models for four large-scale hydrological models are analysed. For the period 1971-2000 these hydrological simulations are compared to simulations using meteorological data based on observations and reanalysis; i.e. the baseline simulation. In both forcing datasets originating from climate models precipitation and temperature are bias corrected to the baseline forcing dataset. Hence, it is only effects of radiation, humidity and wind estimates that are tested here. The direct use of climate model outputs result in substantial different evapotranspiration and runoff estimates, when compared to the baseline simulations. A simple bias correction method is implemented and tested by rerunning the hydrological models using bias corrected radiation, humidity and wind values. The results indicate that bias correction can successfully be used to match the baseline simulations. Finally, historical (1971-2000) and future (2071-2100) model simulations resulting from using bias corrected forcings are compared to the results using non-bias corrected forcings. The relative changes in simulated evapotranspiration and runoff are relatively similar for the bias corrected and non bias corrected hydrological projections, although the absolute evapotranspiration and runoff numbers are often very different. The simulated relative and absolute differences when using bias corrected and non bias corrected climate model radiation, humidity and wind values are, however, smaller than literature reported differences resulting from using bias corrected and non bias corrected climate model precipitation and temperature values.
- ItemA critical humidity threshold for monsoon transitions(München : European Geopyhsical Union, 2012) Schewe, J.; Levermann, A.; Cheng, H.Monsoon systems around the world are governed by the so-called moisture-advection feedback. Here we show that, in a minimal conceptual model, this feedback implies a critical threshold with respect to the atmospheric specific humidity qo over the ocean adjacent to the monsoon region. If qo falls short of this critical value qoc, monsoon rainfall over land cannot be sustained. Such a case could occur if evaporation from the ocean was reduced, e.g. due to low sea surface temperatures. Within the restrictions of the conceptual model, we estimate qoc from present-day reanalysis data for four major monsoon systems, and demonstrate how this concept can help understand abrupt variations in monsoon strength on orbital timescales as found in proxy records.
- ItemEffects of the Lake Sobradinho Reservoir (Northeastern Brazil) on the Regional Climate(Basel : MDPI, 2017) Ekhtiari, Nikoo; Grossman-Clarke, Susanne; Koch, Hagen; de Souza, Werônica Meira; Donner, Reik V.; Volkholz, JanThis study investigates the effects of Lake Sobradinho, a large reservoir in Northeastern Brazil, on the local near-surface atmospheric and boundary layer conditions. For this purpose, simulations with the regional climate model COSMO-CLM are compared for two different scenarios: (1) with the lake being replaced by the average normal native vegetation cover and (2) with the lake as it exists today, for two different two-month periods reflecting average and very dry conditions, respectively. The performance of the simulation is evaluated against data from surface meteorological stations as well as satellite data in order to ensure the model’s ability to capture atmospheric conditions in the vicinity of Lake Sobradinho. The obtained results demonstrate that the lake affects the near-surface air temperature of the surrounding area as well as its humidity and wind patterns. Specifically, Lake Sobradinho cools down the air during the day and warms it up during the night by up to several ∘ C depending on the large-scale meteorological conditions. Moreover, the humidity is significantly increased as a result of the lake’s presence and causes a lake breeze. The observed effects on humidity and air temperature also extend over areas relatively far away from the lake.
- ItemOn statistics of the free-troposphere synoptic component: An evaluation of skewnesses and mixed third-order moments contribution to the synoptic-scale dynamics and fluxes of heat and humidity(Abingdon : Taylor and Francis Ltd., 2008) Petoukhov, V.; Eliseev, A.V.; Klein, R.; Oesterle, H.Based on the ERA40 data for 1976-2002 we calculated skewnesses and mixed third-order statistical moments (TOMs) for the synoptic variations [with (2.5-6) d timescales]of horizontal winds, temperature, vertical velocity and the specific humidity in Eulerian coordinates. All these variables show skewnesses which markedly deviate from zero, basically at the entries and the outlets of the mid-latitude storm tracks. In these regions, high values of skewness for vertical velocity, temperature and the specific humidity are revealed throughout the entire free troposphere, while the marked skewnesses for horizontal winds are traced in the lower free troposphere. We found a notable deviation of the synoptic-component statistics from the Gaussian statistics. We also made an estimate of the contribution from TOMs to the prognostic equations for the synoptic-scale kinetic energy and the meridional fluxes of sensible and latent heat, which appeared to be non-negligible, mainly in the storm tracks in winter. Our analysis attests that the most pronounced contribution of TOMs to the aforementioned equations comes from the self-advection by the horizontal synoptic-scale motions, while the TOMs induced by the metric terms in the original equations, and specifically the TOMs associated with the vertical self-advection by the synoptic-scale motions, are much less important.