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- ItemEnhancing the spatiotemporal features of polar mesosphere summer echoes using coherent MIMO and radar imaging at MAARSY(Göttingen : Copernicus GmbH, 2019) Urco, J.M.; Chau, J.L.; Weber, T.; Latteck, R.Polar mesospheric summer echoes (PMSEs) are very strong radar echoes caused by the presence of ice particles, turbulence, and free electrons in the mesosphere over polar regions. For more than three decades, PMSEs have been used as natural tracers of the complicated atmospheric dynamics of this region. Neutral winds and turbulence parameters have been obtained assuming PMSE horizontal homogeneity on scales of tens of kilometers. Recent radar imaging studies have shown that PMSEs are not homogeneous on these scales and instead they are composed of kilometer-scale structures. In this paper, we present a technique that allows PMSE observations with unprecedented angular resolution (∼0.6). The technique combines the concept of coherent MIMO (Multiple Input Multiple Output) and two high-resolution imaging techniques, i.e., Capon and maximum entropy (MaxEnt). The resulting resolution is evaluated by imaging specular meteor echoes. The gain in angular resolution compared to previous approaches using SIMO (Single Input Multiple Output) and Capon is at least a factor of 2; i.e., at 85 km, we obtain a horizontal resolution of ∼900 m. The advantage of the new technique is evaluated with two events of 3-D PMSE structures showing: (1) horizontal wavelengths of 8-10 km and periods of 4-7 min, drifting with the background wind, and (2) horizontal wavelengths of 12-16 km and periods of 15-20 min, not drifting with the background wind. Besides the advantages of the implemented technique, we discuss its current challenges, like the use of reduced power aperture and processing time, as well as the future opportunities for improving the understanding of the complex small-scale atmospheric dynamics behind PMSEs. © 2019 Author(s).
- ItemMulti-static spatial and angular studies of polar mesospheric summer echoes combining MAARSY and KAIRA(Göttingen : Copernicus GmbH, 2018) Chau, J.L.; McKay, D.; Vierinen, J.P.; La Hoz, C.; Ulich, T.; Lehtinen, M.; Latteck, R.Polar mesospheric summer echoes (PMSEs) have been long associated with noctilucent clouds (NLCs). For large ice particles sizes and relatively high ice densities, PMSEs at 3m Bragg wavelengths are known to be good tracers of the atmospheric wind dynamics and to be highly correlated with NLC occurrence. Combining the Middle Atmosphere ALOMAR Radar System (MAARSY) and the Kilpisjärvi Atmospheric Imaging Receiver Array (KAIRA), i.e., monostatic and bistatic observations, we show for the first time direct evidence of limited-volume PMSE structures drifting more than 90 km almost unchanged. These structures are shown to have horizontal widths of 5-15 km and are separated by 20-60 km, consistent with structures due to atmospheric waves previously observed in NLCs from the ground and from space. Given the lower sensitivity of KAIRA, the observed features are attributed to echoes from regions with high Schmidt numbers that provide a large radar cross section. The bistatic geometry allows us to determine an upper value for the angular sensitivity of PMSEs at meter scales. We find no evidence for strong aspect sensitivity for PMSEs, which is consistent with recent observations using radar imaging approaches. Our results indicate that multi-static allsky interferometric radar observations of PMSEs could be a powerful tool for studying mesospheric wind fields within large geographic areas. © Author(s) 2018.
- ItemEnantio-sensitive unidirectional light bending([London] : Nature Publishing Group UK, 2021) Ayuso, David; Ordonez, Andres F.; Decleva, Piero; Ivanov, Misha; Smirnova, OlgaStructured light, which exhibits nontrivial intensity, phase, and polarization patterns in space, has key applications ranging from imaging and 3D micromanipulation to classical and quantum communication. However, to date, its application to molecular chirality has been limited by the weakness of magnetic interactions. Here we structure light’s local handedness in space to introduce and realize an enantio-sensitive interferometer for efficient chiral recognition without magnetic interactions, which can be seen as an enantio-sensitive version of Young’s double slit experiment. Upon interaction with isotropic chiral media, such chirality-structured light effectively creates chiral emitters of opposite handedness, located at different positions in space. We show that if the distribution of light’s handedness breaks left-right symmetry, the interference of these chiral emitters leads to unidirectional bending of the emitted light, in opposite directions in media of opposite handedness, even if the number of the left-handed and right-handed emitters excited in the medium is exactly the same. Our work introduces the concepts of polarization of chirality and chirality-polarized light, exposes the immense potential of sculpting light’s local chirality, and offers novel opportunities for efficient chiral discrimination, enantio-sensitive optical molecular fingerprinting and imaging on ultrafast time scales.
- ItemX-ray imaging of chemically active valence electrons during a pericyclic reaction(London : Nature Publishing Group, 2014) Bredtmann, T.; Ivanov, M.; Dixit, G.Time-resolved imaging of chemically active valence electron densities is a long-sought goal, as these electrons dictate the course of chemical reactions. However, X-ray scattering is always dominated by the core and inert valence electrons, making time-resolved X-ray imaging of chemically active valence electron densities extremely challenging. Here we demonstrate an effective and robust method, which emphasizes the information encoded in weakly scattered photons, to image chemically active valence electron densities. The degenerate Cope rearrangement of semibullvalene, a pericyclic reaction, is used as an example to visually illustrate our approach. Our work also provides experimental access to the long-standing problem of synchronous versus asynchronous bond formation and breaking during pericyclic reactions.
- ItemMemory effect assisted imaging through multimode optical fibres([London] : Nature Publishing Group UK, 2021) Li, Shuhui; Horsley, Simon A.R.; Tyc, Tomáš; Čižmár, Tomáš; Phillips, David B.When light propagates through opaque material, the spatial information it holds becomes scrambled, but not necessarily lost. Two classes of techniques have emerged to recover this information: methods relying on optical memory effects, and transmission matrix (TM) approaches. Here we develop a general framework describing the nature of memory effects in structures of arbitrary geometry. We show how this framework, when combined with wavefront shaping driven by feedback from a guide-star, enables estimation of the TM of any such system. This highlights that guide-star assisted imaging is possible regardless of the type of memory effect a scatterer exhibits. We apply this concept to multimode fibres (MMFs) and identify a ‘quasi-radial’ memory effect. This allows the TM of an MMF to be approximated from only one end - an important step for micro-endoscopy. Our work broadens the applications of memory effects to a range of novel imaging and optical communication scenarios.
- ItemCoherent diffractive imaging of single helium nanodroplets with a high harmonic generation source([London] : Nature Publishing Group UK, 2017) Rupp, Daniela; Monserud, Nils; Langbehn, Bruno; Sauppe, Mario; Zimmermann, Julian; Ovcharenko, Yevheniy; Möller, Thomas; Frassetto, Fabio; Poletto, Luca; Trabattoni, Andrea; Calegari, Francesca; Nisoli, Mauro; Sander, Katharina; Peltz, Christian; J. Vrakking, Marc; Fennel, Thomas; Rouzée, ArnaudCoherent diffractive imaging of individual free nanoparticles has opened routes for the in situ analysis of their transient structural, optical, and electronic properties. So far, single-shot single-particle diffraction was assumed to be feasible only at extreme ultraviolet and X-ray free-electron lasers, restricting this research field to large-scale facilities. Here we demonstrate single-shot imaging of isolated helium nanodroplets using extreme ultraviolet pulses from a femtosecond-laser-driven high harmonic source. We obtain bright wide-Angle scattering patterns, that allow us to uniquely identify hitherto unresolved prolate shapes of superfluid helium droplets. Our results mark the advent of single-shot gas-phase nanoscopy with lab-based short-wavelength pulses and pave the way to ultrafast coherent diffractive imaging with phase-controlled multicolor fields and attosecond pulses.
- ItemPore-scale tomography and imaging: applications, techniques and recommended practice(Göttingen : Copernicus Publ., 2016) Halisch, Matthias; Steeb, Holger; Henkel, Steven; Krawczyk, Charlotte M.[No abstract available]
- ItemSeismic imaging of sandbox experiments – laboratory hardware setup and first reflection seismic sections(Göttingen : Copernicus Publ., 2013) Krawczyk, C.M.; Buddensiek, M.-L.; Oncken, O.; Kukowski, N.With the study and technical development introduced here, we combine analogue sandbox simulation techniques with seismic physical modelling of sandbox models. For that purpose, we designed and developed a new mini-seismic facility for laboratory use, comprising a seismic tank, a PC-driven control unit, a positioning system, and piezoelectric transducers used here for the first time in an array mode. To assess the possibilities and limits of seismic imaging of small-scale structures in sandbox models, different geometry setups were tested in the first 2-D experiments that also tested the proper functioning of the device and studied the seismo-elastic properties of the granular media used. Simple two-layer models of different materials and layer thicknesses as well as a more complex model comprising channels and shear zones were tested using different acquisition geometries and signal properties. We suggest using well sorted and well rounded grains with little surface roughness (glass beads). Source receiver-offsets less than 14 cm for imaging structures as small as 2.0–1.5 mm size have proven feasible. This is the best compromise between wide beam and high energy output, and is applicable with a consistent waveform. Resolution of the interfaces of layers of granular materials depends on the interface preparation rather than on the material itself. Flat grading of interfaces and powder coverage yields the clearest interface reflections. Finally, sandbox seismic sections provide images of high quality showing constant thickness layers as well as predefined channel structures and indications of the fault traces from shear zones. Since these were artificially introduced in our test models, they can be regarded as zones of disturbance rather than tectonic shear zones characterized by decompaction. The multiple-offset surveying introduced here, improves the quality with respect to S / N ratio and source signature even more; the maximum depth penetration in glass-bead layers thereby amounts to 5 cm. Thus, the presented mini-seismic device is already able to resolve structures within simple models of saturated porous media, so that multiple-offset seismic imaging of shallow sandbox models, that are structurally evolving, is generally feasible.