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Continuous vertical aerosol profiling with a multi-wavelength Raman polarization lidar over the Pearl River Delta, China
2017, Heese, Birgit, Baars, Holger, Bohlmann, Stephanie, Althausen, Dietrich, Deng, Ruru
A dataset of particle optical properties of the highly polluted atmosphere over the Pearl River Delta (PRD), Guangzhou, China, is presented in this paper. The data were derived from the measurements of a multiwavelength Raman and depolarization lidar PollyXT and a co-located AERONET sun photometer. The measurement campaign was conducted from November 2011 to mid-June 2012. These are the first Raman lidar measurements in the PRD that lasted for several months. A mean value of aerosol optical depth (AOD) of 0.54±0.33 was observed by the sun photometer at 500 nm in the polluted atmosphere over this megacity for the whole measurement period. The lidar profiles frequently show lofted aerosol layers, which reach altitudes of up to 2 to 3 km and, especially during the spring season, up to 5 km. These layers contain between 12 and 56% of the total AOD, with the highest values in spring. The aerosol types in these lofted layers are classified by their optical properties. The observed lidar ratio values range from 30 to 80 sr with a mean value of 48.0±10.7 sr at 532 nm. The linear particle depolarization ratio at 532 nm lies mostly below 5 %, with a mean value of 3.6±3.7 %. The majority of the Ångström exponents lie between 0.5 and 1.5, indicating a mixture of fine- and coarsemode aerosols. These results reveal that mostly urban pollution particles mixed with particles produced from biomass and industrial burning are present in the atmosphere above the Pearl River Delta. Trajectory analyses show that these pollution mixtures arise mainly from local and regional sources.
Depolarization ratio profiling at several wavelengths in pure Saharan dust during SAMUM 2006
2017, Freudenthaler, Volker, Esselborn, Michael, Wiegner, Matthias, Heese, Birgit, Tesche, Matthias, Ansmann, Albert, Müller, Detlef, Althausen, Dietrich, Wirth, Martin, Fix, Andreas, Ehret, Gerhard, Knippertz, Peter, Toledano, Carlos, Gasteiger, Josef, Garhammer, Markus, Seefeldner, Meinhard
Vertical profiles of the linear particle depolarization ratio of pure dust clouds were measured during the Saharan Mineral Dust Experiment (SAMUM) at Ouarzazate, Morocco (30.9◦N, –6.9◦E), close to source regions in May–June 2006, with four lidar systems at four wavelengths (355, 532, 710 and 1064 nm). The intercomparison of the lidar systems is accompanied by a discussion of the different calibration methods, including a new, advanced method, and a detailed error analysis. Over the whole SAMUM periode pure dust layers show a mean linear particle depolarization ratio at 532 nm of 0.31, in the range between 0.27 and 0.35, with a mean Ångström exponent (AE, 440–870 nm) of 0.18 (range 0.04–0.34) and still high mean linear particle depolarization ratio between 0.21 and 0.25 during periods with aerosol optical thickness less than 0.1, with a mean AE of 0.76 (range 0.65–1.00), which represents a negative correlation of the linear particle depolarization ratio with the AE. A slight decrease of the linear particle depolarization ratio with wavelength was found between 532 and 1064 nm from 0.31 ± 0.03 to 0.27 ± 0.04.
Characterization of Saharan dust, marine aerosols and mixtures of biomass-burning aerosols and dust by means of multi-wavelength depolarization and Raman lidar measurements during SAMUM 2
2017, Groß, Silke, Tesche, Matthias, Freudenthaler, Volker, Toledano, Carlos, Wiegner, Matthias, Ansmann, Albert, Althausen, Dietrich, Seefeldner, Meinhard
The particle linear depolarization ratio δp of Saharan dust, marine aerosols and mixtures of biomass-burning aerosols from southern West Africa and Saharan dust was determined at three wavelengths with three lidar systems during the SAharan Mineral dUst experiMent 2 at the airport of Praia, Cape Verde, between 22 January and 9 February 2008. The lidar ratio Sp of these major types of tropospheric aerosols was analysed at two wavelengths. For Saharan dust, we find wavelength dependent mean particle linear depolarization ratios δp of 0.24–0.27 at 355 nm, 0.29–0.31 at 532 nm and 0.36–0.40 at 710 nm, and wavelength independent mean lidar ratios Sp of 48–70 sr. Mixtures of biomass-burning aerosols and dust show wavelength independent values of δp and Sp between 0.12–0.23 and 57–98 sr, respectively. The mean values of marine aerosols range independent of wavelength for δp from 0.01 to 0.03 and for Sp from 14 to 24 sr.
Triple-wavelength depolarization-ratio profiling of Saharan dust over Barbados during SALTRACE in 2013 and 2014
2017, Haarig, Moritz, Ansmann, Albert, Althausen, Dietrich, Klepel, André, Groß, Silke, Freudenthaler, Volker, Toledano, Carlos, Mamouri, Rodanthi-Elisavet, Farrell, David A., Prescod, Damien A., Marinou, Eleni, Burton, Sharon P., Gasteiger, Josef, Engelmann, Ronny, Baars, Holger
Triple-wavelength polarization lidar measurements in Saharan dust layers were performed at Barbados (13.1°N, 59.6°W), 5000-8000km west of the Saharan dust sources, in the framework of the Saharan Aerosol Long-range Transport and Aerosol-Cloud-Interaction Experiment (SALTRACE-1, June-July 2013, SALTRACE-3, June-July 2014). Three case studies are discussed. High quality was achieved by comparing the dust linear depolarization ratio profiles measured at 355, 532, and 1064nm with respective dual-wavelength (355, 532nm) depolarization ratio profiles measured with a reference lidar. A unique case of long-range transported dust over more than 12000km is presented. Saharan dust plumes crossing Barbados were measured with an airborne triple-wavelength polarization lidar over Missouri in the midwestern United States 7 days later. Similar dust optical properties and depolarization features were observed over both sites indicating almost unchanged dust properties within this 1 week of travel from the Caribbean to the United States. The main results of the triple-wavelength polarization lidar observations in the Caribbean in the summer seasons of 2013 and 2014 are summarized. On average, the particle linear depolarization ratios for aged Saharan dust were found to be 0.252±0.030 at 355nm, 0.280±0.020 at 532nm, and 0.225±0.022 at 1064nm after approximately 1 week of transport over the tropical Atlantic. Based on published simulation studies we present an attempt to explain the spectral features of the depolarization ratio of irregularly shaped mineral dust particles, and conclude that most of the irregularly shaped coarse-mode dust particles (particles with diameters > 1μm) have sizes around 1.5-2μm. The SALTRACE results are also set into the context of the SAMUM-1 (Morocco, 2006) and SAMUM-2 (Cabo Verde, 2008) depolarization ratio studies. Again, only minor changes in the dust depolarization characteristics were observed on the way from the Saharan dust sources towards the Caribbean.
Vertically resolved dust optical properties during SAMUM: Tinfou compared to Ouarzazate
2017, Heese, Birgit, Althausen, Dietrich, Dinter, Tilman, Esselborn, Michael, Müller, Thomas, Tesche, Matthias, Wiegner, Matthias
Vertical profiles of dust key optical properties are presented from measurements during the Saharan Mineral Dust Experiment (SAMUM) by Raman and depolarization lidar at two ground-based sites and by airborne high spectral resolution lidar. One of the sites, Tinfou, is located close to the border of the Sahara in Southern Morocco and was the main in situ site during SAMUM. The other site was Ouarzazate airport, the main lidar site. From the lidar measurements the spatial distribution of the dust between Tinfou and Ouarzazate was derived for 1 d. The retrieved profiles of backscatter and extinction coefficients and particle depolarization ratios show comparable dust optical properties, a similar vertical structure of the dust layer, and a height of about 4 km asl at both sites. The airborne cross-section of the extinction coefficient at the two sites confirms the low variability in dust properties. Although the general picture of the dust layer was similar, the lidar measurements reveal a higher dust load closer to the dust source. Nevertheless, the observed intensive optical properties were the same. These results indicate that the lidar measurements at two sites close to the dust source are both representative for the SAMUM dust conditions.
Vertical profiling of convective dust plumes in southern Morocco during SAMUM
2017, Ansmann, Albert, Tesche, Matthias, Knippertz, Peter, Bierwirth, Eike, Althausen, Dietrich, Müller, Detlef, Schulz, Oliver
Lifting of dust particles by dust devils and convective plumes may significantly contribute to the global mineral dust budget. During the Saharan Mineral Dust Experiment (SAMUM) in May–June 2006 vertical profiling of dusty plumes was performed for the first time. Polarization lidar observations taken at Ouarzazate (30.9◦N, 6.9◦W, 1133 m height above sea level) are analyzed. Two cases with typical and vigorous formation of convective plumes and statistical results of 5 d are discussed. The majority of observed convective plumes have diameters on order of 100–400 m. Most of the plumes (typically 50–95%) show top heights <1 km or 0.3DLH with the Saharan dust layer height DLH of typically 3–4 km. Height-to-diameter ratio is mostly 2–10. Maximum plume top height ranges from 1.1 to 2.9 km on the 5 d. 5–26 isolated plumes and clusters of plumes per hour were detected. A low dust optical depth (<0.3) favours plume evolution. Observed surface, 1 and 2–m air temperatures indicate that a difference of 17–20 K between surface and 2-m air temperature and of 0.9–1 K between the 1 and 2-m temperatures are required before convective plumes develop. Favourable horizontal wind speeds are 2–7 ms−1.
Doppler lidar studies of heat island effects on vertical mixing of aerosols during SAMUM-2
2017, Engelmann, Ronny, Ansmann, Albert, Horn, Stefan, Seifert, Patric, Althausen, Dietrich, Tesche, Matthias, Esselborn, Michael, Fruntke, Julia, Lieke, Kirsten, Freudenthaler, Volker, Gross, Silke
A wind Doppler lidar was deployed next to three aerosol lidars during the SAMUM–2 campaign on the main island of Cape Verde. The effects of the differential heating of the island and the surrounding ocean and the orographic impact of the capital island Santiago and the small island on its luv side, Maio, are investigated. Horizontal and vertical winds were measured in the disturbed maritime boundary layer and compared to local radiosoundings. Lidar measurements from the research aircraft Falcon and a 3-D Large Eddy Simulation (LES) model were used in addition to study the heating effects on the scale of the islands. Indications are found that these effects can widely control the downward mixing from greater heights to the surface of African aerosols, mainly Saharan dust and biomass-burning smoke, which were detected in a complex layering over the Cape Verde region.
Optical and microphysical properties of smoke over Cape Verde inferred from multiwavelength lidar measurements
2017, Tesche, Matthias, Müller, Detlef, Gross, Silke, Ansmann, Albert, Althausen, Dietrich, Freudenthaler, Volker, Weinzierl, Bernadett, Veira, Andreas, Petzold, Andreas
Lidar measurements of mixed dust/smoke plumes over the tropical Atlantic ocean were carried out during the winter campaign of SAMUM-2 at Cape Verde. Profiles of backscatter and extinction coefficients, lidar ratios, and Ångstr¨om exponents related to pure biomass-burning aerosol from southern West Africa were extracted from these observations. Furthermore, these findings were used as input for an inversion algorithm to retrieve microphysical properties of pure smoke. Seven measurement days were found suitable for the procedure of aerosol-type separation and successive inversion of optical data that describe biomass-burning smoke. We inferred high smoke lidar ratios of 87 ± 17 sr at 355 nm and 79 ± 17 sr at 532 nm. Smoke lidar ratios and Ångstr¨om exponents are higher compared to the ones for the dust/smoke mixture. These numbers indicate higher absorption and smaller sizes for pure smoke particles compared to the dust/smoke mixture. Inversion of the smoke data set results in mean effective radii of 0.22 ± 0.08 μm with individual results varying between 0.10 and 0.36 μm. The single-scattering albedo for pure biomass-burning smoke was found to vary between 0.63 and 0.89 with a very low mean value of 0.75 ± 0.07. This is in good agreement with findings of airborne in situ measurements which showed values of 0.77 ± 0.03. Effective radii from the inversion were similar to the ones found for the fine mode of the in situ size distributions.
Vertical profiling of Saharan dust with Raman lidars and airborne HSRL in southern Morocco during SAMUM
2017, Tesche, Matthias, Ansmann, Albert, MüLLER, Detlef, Althausen, Dietrich, Mattis, Ina, Heese, Birgit, Freudenthaler, Volker, Wiegner, Matthias, Esselborn, Michael, Pisani, Gianluca, Knippertz, Peter
Three ground-based Raman lidars and an airborne high-spectral-resolution lidar (HSRL) were operated duringSAMUM 2006 in southern Morocco to measure height profiles of the volume extinction coefficient, the extinction-to-backscatter ratio and the depolarization ratio of dust particles in the Saharan dust layer at several wavelengths. Aerosol Robotic Network (AERONET) Sun photometer observations and radiosoundings of meteorological parameters complemented the ground-based activities at the SAMUM station of Ouarzazate. Four case studies are presented. Two case studies deal with the comparison of observations of the three ground-based lidars during a heavy dust outbreak and of the ground-based lidars with the airborne lidar. Two further cases show profile observations during satellite overpasses on 19 May and 4 June 2006. The height resolved statistical analysis reveals that the dust layer top typically reaches 4–6 km height above sea level (a.s.l.), sometimes even 7 km a.s.l.. Usually, a vertically inhomogeneous dust plume with internal dust layers was observed in the morning before the evolution of the boundary layer started. The Saharan dust layer was well mixed in the early evening. The 500 nm dust optical depth ranged from 0.2–0.8 at the field site south of the High Atlas mountains, Ångström exponents derived from photometer and lidar data were between 0–0.4. The volume extinction coefficients (355, 532 nm) varied from 30–300Mm−1 with a mean value of 100Mm−1 in the lowest 4 km a.s.l.. On average, extinction-to-backscatter ratios of 53–55 sr (±7–13 sr) were obtained at 355, 532 and 1064 nm.