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- ItemDepolarization ratio profiling at several wavelengths in pure Saharan dust during SAMUM 2006(Milton Park : Taylor & Francis, 2017) Freudenthaler, Volker; Esselborn, Michael; Wiegner, Matthias; Heese, Birgit; Tesche, Matthias; Ansmann, Albert; Müller, Detlef; Althausen, Dietrich; Wirth, Martin; Fix, Andreas; Ehret, Gerhard; Knippertz, Peter; Toledano, Carlos; Gasteiger, Josef; Garhammer, Markus; Seefeldner, MeinhardVertical profiles of the linear particle depolarization ratio of pure dust clouds were measured during the Saharan Mineral Dust Experiment (SAMUM) at Ouarzazate, Morocco (30.9◦N, –6.9◦E), close to source regions in May–June 2006, with four lidar systems at four wavelengths (355, 532, 710 and 1064 nm). The intercomparison of the lidar systems is accompanied by a discussion of the different calibration methods, including a new, advanced method, and a detailed error analysis. Over the whole SAMUM periode pure dust layers show a mean linear particle depolarization ratio at 532 nm of 0.31, in the range between 0.27 and 0.35, with a mean Ångström exponent (AE, 440–870 nm) of 0.18 (range 0.04–0.34) and still high mean linear particle depolarization ratio between 0.21 and 0.25 during periods with aerosol optical thickness less than 0.1, with a mean AE of 0.76 (range 0.65–1.00), which represents a negative correlation of the linear particle depolarization ratio with the AE. A slight decrease of the linear particle depolarization ratio with wavelength was found between 532 and 1064 nm from 0.31 ± 0.03 to 0.27 ± 0.04.
- ItemPotential of polarization lidar to provide profiles of CCN-and INP-relevant aerosol parameters(München : European Geopyhsical Union, 2016) Mamouri, Rodanthi-Elisavet; Ansmann, AlbertWe investigate the potential of polarization lidar to provide vertical profiles of aerosol parameters from which cloud condensation nucleus (CCN) and ice nucleating particle (INP) number concentrations can be estimated. We show that height profiles of particle number concentrations n50, dry considering dry aerosol particles with radius > 50 nm (reservoir of CCN in the case of marine and continental non-desert aerosols), n100, dry (particles with dry radius > 100 nm, reservoir of desert dust CCN), and of n250, dry (particles with dry radius > 250 nm, reservoir of favorable INP), as well as profiles of the particle surface area concentration sdry (used in INP parameterizations) can be retrieved from lidar-derived aerosol extinction coefficients σ with relative uncertainties of a factor of 1.5–2 in the case of n50, dry and n100, dry and of about 25–50 % in the case of n250, dry and sdry. Of key importance is the potential of polarization lidar to distinguish and separate the optical properties of desert aerosols from non-desert aerosol such as continental and marine particles. We investigate the relationship between σ, measured at ambient atmospheric conditions, and n50, dry for marine and continental aerosols, n100, dry for desert dust particles, and n250, dry and sdry for three aerosol types (desert, non-desert continental, marine) and for the main lidar wavelengths of 355, 532, and 1064 nm. Our study is based on multiyear Aerosol Robotic Network (AERONET) photometer observations of aerosol optical thickness and column-integrated particle size distribution at Leipzig, Germany, and Limassol, Cyprus, which cover all realistic aerosol mixtures. We further include AERONET data from field campaigns in Morocco, Cabo Verde, and Barbados, which provide pure dust and pure marine aerosol scenarios. By means of a simple CCN parameterization (with n50, dry or n100, dry as input) and available INP parameterization schemes (with n250, dry and sdry as input) we finally compute profiles of the CCN-relevant particle number concentration nCCN and the INP number concentration nINP. We apply the method to a lidar observation of a heavy dust outbreak crossing Cyprus and a case dominated by continental aerosol pollution.
- ItemVertical profiles of aerosol mass concentration derived by unmanned airborne in situ and remote sensing instruments during dust events(Katlenburg-Lindau : Copernicus, 2018) Mamali, Dimitra; Marinou, Eleni; Sciare, Jean; Pikridas, Michael; Kokkalis, Panagiotis; Kottas, Michael; Binietoglou, Ioannis; Tsekeri, Alexandra; Keleshis, Christos; Engelmann, Ronny; Baars, Holger; Ansmann, Albert; Amiridis, Vassilis; Russchenberg, Herman; Biskos, GeorgeIn situ measurements using unmanned aerial vehicles (UAVs) and remote sensing observations can independently provide dense vertically resolved measurements of atmospheric aerosols, information which is strongly required in climate models. In both cases, inverting the recorded signals to useful information requires assumptions and constraints, and this can make the comparison of the results difficult. Here we compare, for the first time, vertical profiles of the aerosol mass concentration derived from light detection and ranging (lidar) observations and in situ measurements using an optical particle counter on board a UAV during moderate and weak Saharan dust episodes. Agreement between the two measurement methods was within experimental uncertainty for the coarse mode (i.e. particles having radii > 0.5 μm), where the properties of dust particles can be assumed with good accuracy. This result proves that the two techniques can be used interchangeably for determining the vertical profiles of aerosol concentrations, bringing them a step closer towards their systematic exploitation in climate models.
- ItemSaharan Mineral Dust Experiments SAMUM-1 and SAMUM-2: What have we learned?(Milton Park : Taylor & Francis, 2011) Ansmann, Albert; Petzold, Andreas; Kandler, Konrad; Tegen, Ina; Wendisch, Manfred; Müller, Detlef; Weinzierl, Bernadett; Müller, Thomas; Heintzenberg, JostTwo comprehensive field campaigns were conducted in 2006 and 2008 in the framework of the Saharan Mineral Dust Experiment (SAMUM) project. The relationship between chemical composition, shape morphology, size distribution and optical effects of the dust particles was investigated. The impact of Saharan dust on radiative transfer and the feedback of radiative effects upon dust emission and aerosol transport were studied. Field observations (ground-based, airborne and remote sensing) and modelling results were compared within a variety of dust closure experiments with a strong focus on vertical profiling. For the first time, multiwavelength Raman/polarization lidars and an airborne high spectral resolution lidar were involved in major dust field campaigns and provided profiles of the volume extinction coefficient of the particles at ambient conditions (for the full dust size distribution), of particle-shape-sensitive optical properties at several wavelengths, and a clear separation of dust and smoke profiles allowing for an estimation of the single-scattering albedo of the biomass-burning aerosol. SAMUM–1 took place in southern Morocco close to the Saharan desert in the summer of 2006, whereas SAMUM–2 was conducted in Cape Verde in the outflow region of desert dust and biomass-burning smoke from western Africa in the winter of 2008. This paper gives an overview of the SAMUM concept, strategy and goals, provides snapshots (highlights) of SAMUM–2 observations and modelling efforts, summarizes main findings of SAMUM–1 and SAMUM–2 and finally presents a list of remaining problems and unsolved questions.
- ItemVertical profiling of Saharan dust with Raman lidars and airborne HSRL in southern Morocco during SAMUM(Milton Park : Taylor & Francis, 2017) Tesche, Matthias; Ansmann, Albert; MüLLER, Detlef; Althausen, Dietrich; Mattis, Ina; Heese, Birgit; Freudenthaler, Volker; Wiegner, Matthias; Esselborn, Michael; Pisani, Gianluca; Knippertz, PeterThree ground-based Raman lidars and an airborne high-spectral-resolution lidar (HSRL) were operated duringSAMUM 2006 in southern Morocco to measure height profiles of the volume extinction coefficient, the extinction-to-backscatter ratio and the depolarization ratio of dust particles in the Saharan dust layer at several wavelengths. Aerosol Robotic Network (AERONET) Sun photometer observations and radiosoundings of meteorological parameters complemented the ground-based activities at the SAMUM station of Ouarzazate. Four case studies are presented. Two case studies deal with the comparison of observations of the three ground-based lidars during a heavy dust outbreak and of the ground-based lidars with the airborne lidar. Two further cases show profile observations during satellite overpasses on 19 May and 4 June 2006. The height resolved statistical analysis reveals that the dust layer top typically reaches 4–6 km height above sea level (a.s.l.), sometimes even 7 km a.s.l.. Usually, a vertically inhomogeneous dust plume with internal dust layers was observed in the morning before the evolution of the boundary layer started. The Saharan dust layer was well mixed in the early evening. The 500 nm dust optical depth ranged from 0.2–0.8 at the field site south of the High Atlas mountains, Ångström exponents derived from photometer and lidar data were between 0–0.4. The volume extinction coefficients (355, 532 nm) varied from 30–300Mm−1 with a mean value of 100Mm−1 in the lowest 4 km a.s.l.. On average, extinction-to-backscatter ratios of 53–55 sr (±7–13 sr) were obtained at 355, 532 and 1064 nm.
- Item1064nm rotational Raman lidar for particle extinction and lidar-ratio profiling: Cirrus case study(München : European Geopyhsical Union, 2016) Haarig, Moritz; Engelmann, Ronny; Ansmann, Albert; Veselovskii, Igor; Whiteman, David N.; Althausen, DietrichFor the first time, vertical profiles of the 1064 nm particle extinction coefficient obtained from Raman lidar observations at 1058 nm (nitrogen and oxygen rotational Raman backscatter) are presented. We applied the new technique in the framework of test measurements and performed several cirrus observations of particle backscatter and extinction coefficients, and corresponding extinction-to-backscatter ratios at the wavelengths of 355, 532, and 1064 nm. The cirrus backscatter coefficients were found to be equal for all three wavelengths keeping the retrieval uncertainties in mind. The multiple-scattering-corrected cirrus extinction coefficients at 355 nm were on average about 20–30 % lower than the ones for 532 and 1064 nm. The cirrus-mean extinction-to-backscatter ratio (lidar ratio) was 31 ± 5 sr (355 nm), 36 ± 5 sr (532 nm), and 38 ± 5 sr (1064 nm) in this single study. We further discussed the requirements needed to obtain aerosol extinction profiles in the lower troposphere at 1064 nm with good accuracy (20 % relative uncertainty) and appropriate temporal and vertical resolution.
- ItemRegional Saharan dust modelling during the SAMUM 2006 campaign(Milton Park : Taylor & Francis, 2017) Heinold, Bernd; Tegen, Ina; Esselborn, Michael; Kandler, Konrad; Knippertz, Peter; Müller, Detlef; Schladitz, Alexander; Tesche, Matthias; Weinzierl, Bernadett; Ansmann, Albert; Althausen, Dietrich; Laurent, Benoit; Massling, Andreas; Müller, Thomas; Petzold, Andreas; Schepanski, Kerstin; Wiedensohler, AlfredThe regional dust model system LM-MUSCAT-DES was developed in the framework of the SAMUM project. Using the unique comprehensive data set of near-source dust properties during the 2006SAMUMfield campaign, the performance of the model system is evaluated for two time periods in May and June 2006. Dust optical thicknesses, number size distributions and the position of the maximum dust extinction in the vertical profiles agree well with the observations. However, the spatio-temporal evolution of the dust plumes is not always reproduced due to inaccuracies in the dust source placement by the model. While simulated winds and dust distributions are well matched for dust events caused by dry synoptic-scale dynamics, they are often misrepresented when dust emissions are caused by moist convection or influenced by small-scale topography that is not resolved by the model. In contrast to long-range dust transport, in the vicinity of source regions the model performance strongly depends on the correct prediction of the exact location of sources. Insufficiently resolved vertical grid spacing causes the absence of inversions in the model vertical profiles and likely explains the absence of the observed sharply defined dust layers.
- ItemVertical profiling of convective dust plumes in southern Morocco during SAMUM(Milton Park : Taylor & Francis, 2017) Ansmann, Albert; Tesche, Matthias; Knippertz, Peter; Bierwirth, Eike; Althausen, Dietrich; Müller, Detlef; Schulz, OliverLifting of dust particles by dust devils and convective plumes may significantly contribute to the global mineral dust budget. During the Saharan Mineral Dust Experiment (SAMUM) in May–June 2006 vertical profiling of dusty plumes was performed for the first time. Polarization lidar observations taken at Ouarzazate (30.9◦N, 6.9◦W, 1133 m height above sea level) are analyzed. Two cases with typical and vigorous formation of convective plumes and statistical results of 5 d are discussed. The majority of observed convective plumes have diameters on order of 100–400 m. Most of the plumes (typically 50–95%) show top heights <1 km or 0.3DLH with the Saharan dust layer height DLH of typically 3–4 km. Height-to-diameter ratio is mostly 2–10. Maximum plume top height ranges from 1.1 to 2.9 km on the 5 d. 5–26 isolated plumes and clusters of plumes per hour were detected. A low dust optical depth (<0.3) favours plume evolution. Observed surface, 1 and 2–m air temperatures indicate that a difference of 17–20 K between surface and 2-m air temperature and of 0.9–1 K between the 1 and 2-m temperatures are required before convective plumes develop. Favourable horizontal wind speeds are 2–7 ms−1.
- ItemDust mobilization and transport in the northern Sahara during SAMUM 2006 - A meteorological overview(Milton Park : Taylor & Francis, 2017) Knippertz, Peter; Ansmann, Albert; Althausen, Dietrich; Müller, Detlef; Tesche, Matthias; Bierwirth, Eike; Dinter, Tilman; Müller, Thomas; Von Hoyningen-Huene, Wolfgang; Schepanski, Kerstin; Wendisch, Manfred; Heinold, Bernd; Kandler, Konrad; Petzold, Andreas; Tegen, InaThe SAMUM field campaign in southern Morocco in May/June 2006 provides valuable data to study the emission, and the horizontal and vertical transports of mineral dust in the Northern Sahara. Radiosonde and lidar observations show differential advection of air masses with different characteristics during stable nighttime conditions and up to 5-km deep vertical mixing in the strongly convective boundary layer during the day. Lagrangian and synoptic analyses of selected dust periods point to a topographic channel from western Tunisia to central Algeria as a dust source region. Significant emission events are related to cold surges from the Mediterranean in association with eastward passing upper-level waves and lee cyclogeneses south of the Atlas Mountains. Other relevant events are local emissions under a distinct cut-off low over northwestern Africa and gust fronts associated with dry thunderstorms over the Malian and Algerian Sahara. The latter are badly represented in analyses from the European Centre for Medium–Range Weather Forecasts and in a regional dust model, most likely due to problems with moist convective dynamics and a lack of observations in this region. This aspect needs further study. The meteorological source identification is consistent with estimates of optical and mineralogical properties of dust samples.