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- ItemFemtosecond Field‐Driven On‐Chip Unidirectional Electronic Currents in Nonadiabatic Tunneling Regime(Weinheim : Wiley VCH, 2021) Shi, Liping; Babushkin, Ihar; Husakou, Anton; Melchert, Oliver; Frank, Bettina; Yi, Juemin; Wetzel, Gustav; Demircan, Ayhan; Lienau, Christoph; Giessen, Harald; Ivanov, Misha; Morgner, Uwe; Kovacev, MilutinRecently, asymmetric plasmonic nanojunctions have shown promise as on-chip electronic devices to convert femtosecond optical pulses to current bursts, with a bandwidth of multi-terahertz scale, although yet at low temperatures and pressures. Such nanoscale devices are of great interest for novel ultrafast electronics and opto-electronic applications. Here, the device is operated in air and at room temperature, revealing the mechanisms of photoemission from plasmonic nanojunctions, and the fundamental limitations on the speed of optical-to-electronic conversion. Inter-cycle interference of coherent electronic wavepackets results in a complex energy electron distribution and birth of multiphoton effects. This energy structure, as well as reshaping of the wavepackets during their propagation from one tip to the other, determine the ultrafast dynamics of the current. It is shown that, up to some level of approximation, the electron flight time is well-determined by the mean ponderomotive velocity in the driving field.
- ItemInfluence of tunnel ionization to third-harmonic generation of infrared femtosecond laser pulses in air([London] : Macmillan Publishers Limited, part of Springer Nature, 2020) Tamulienė, Viktorija; Juškevičiūtė, Greta; Buožius, Danas; Vaičaitis, Virgilijus; Babushkin, Ihar; Morgner, UweHere we present an experimental as well as theoretical study of third-harmonic generation in tightly focused femtosecond filaments in air at the wavelength of 1.5μm. At low intensities, longitudinal phase matching is dominating in the formation of 3rd harmonics, whereas at higher intensities locked X-waves are formed. We provide the arguments that the X-wave formation is governed mainly by the tunnel-like ionization dynamics rather than by the multiphoton one. Despite of this fact, the impact of the ionization-induced nonlinearity is lower than the one from bound–bound transitions at all intensities. © 2020, The Author(s).