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- ItemElectron–phonon coupling in 122 Fe pnictides analyzed by femtosecond time-resolved photoemission(Milton Park : Taylor & Francis, 2013) Rettig, L.; Cortés, R.; Jeevan, H.S.; Gegenwart, P.; Wolf, T.; Fink, J.; Bovensiepen, U.Based on the results from femtosecond time-resolved photoemission, we compare three different methods for the determination of the electron–phonon coupling constant λ in Eu- and Ba-based 122 FeAs compounds. We find good agreement between all three methods, which reveal a small λ < 0.2. This makes simple electron–phonon-mediated superconductivity unlikely in these compounds.
- ItemDoping dependence and electron–boson coupling in the ultrafast relaxation of hot electron populations in Ba(Fe1–x Co x )2As2(Milton Park : Taylor & Francis, 2016) Avigo, I.; Thirupathaiah, S.; Ligges, M.; Wolf, T.; Fink, J.; Bovensiepen, U.Using femtosecond time- and angle-resolved photoemission spectroscopy we investigate the effect of electron doping on the electron dynamics in $\mathrm{Ba}{({\mathrm{Fe}}_{1-x}{\mathrm{Co}}_{x})}_{2}{\mathrm{As}}_{2}$ in a range of $0\leqslant x\lt 0.15$ at temperatures slightly above the Néel temperature. By analyzing the time-dependent photoemission intensity of the pump laser excited population as a function of energy, we found that the relaxation times at $0\lt E-{E}_{{\rm{F}}}\lt 0.2\,\mathrm{eV}$ are doping dependent and about 100 fs shorter at optimal doping than for overdoped and parent compounds. Analysis of the relaxation rates also reveals the presence of a pump fluence dependent step in the relaxation time at $E-{E}_{{\rm{F}}}=200\,\mathrm{meV}$ which we explain by coupling of the excited electronic system to a boson of this energy. We compare our results with static ARPES and transport measurements and find disagreement and agreement concerning the doping-dependence, respectively. We discuss the effect of the electron–boson coupling on the energy-dependent relaxation and assign the origin of the boson to a magnetic excitation.