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- ItemAll-optical supercontinuum switching(London : Springer Nature, 2020) Melchert, Oliver; Brée, Carsten; Tajalli, Ayhan; Pape, Alexander; Arkhipov, Rostislav; Willms, Stephanie; Babushkin, Ihar; Skryabin, Dmitry; Steinmeyer, Günter; Morgner, Uwe; Demircan, AyhanEfficient all-optical switching is a challenging task as photons are bosons and cannot immediately interact with each other. Consequently, one has to resort to nonlinear optical interactions, with the Kerr gate being the classical example. However, the latter requires strong pulses to switch weaker ones. Numerous approaches have been investigated to overcome the resulting lack of fan-out capability of all-optical switches, most of which relied on types of resonant enhancement of light-matter interaction. Here we experimentally demonstrate a novel approach that utilizes switching between different portions of soliton fission induced supercontinua, exploiting an optical event horizon. This concept enables a high switching efficiency and contrast in a dissipation free setting. Our approach enables fan-out, does not require critical biasing, and is at least partially cascadable. Controlling complex soliton dynamics paves the way towards building all-optical logic gates with advanced functionalities. © 2020, The Author(s).
- ItemSymmetry breaking and strong persistent plasma currents via resonant destabilization of atoms(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2017) Brée, Carsten; Hofmann, Michael; Babushkin, Ihar; Demircan, Ayhan; Morgner, Uwe; Kosareva, Olga G.; Savelev, Andrei B.; Husakou, Anton; Ivanov, MishaThe ionization rate of an atom in a strong optical field can be resonantly enhanced by the presence of long-living atomic levels (so called Freeman resonances). This process is most prominent in the multiphoton ionization regime meaning that ionization event takes many optical cycles. Nevertheless, here we show that these resonances can lead to fast subcycle-scale plasma buildup at the resonant values of the intensity in the pump pulse. The fast buildup can break the cycletocycle symmetry of the ionization process, resulting in generation of persistent macroscopic plasma currents which remain after the end of the pulse. This, in turn, gives rise to a broadband radiation of unusual spectral structure forming a comb from terahertz (THz) to visible. This radiation contains fingerprints of the attosecond electronic dynamics in Rydberg states during ionization.
- ItemAdjustable pulse compression scheme for generation of few-cycle pulses in the mid-infrared(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2014) Demircan, Ayhan; Amiranashvili, Shalva; Brée, Carsten; Morgner, Uwe; Steinmeyer, GünterAn novel adjustable adiabatic soliton compression scheme is presented, enabling a coherent pulse source with pedestal-free few-cycle pulses in the infrared or mid-infrared regime. This scheme relies on interaction of a dispersive wave and a soliton copropagating at nearly identical group velocities in a fiber with enhanced infrared transmission. The compression is achieved directly in one stage, without necessity of an external compensation scheme. Numerical simulations are employed to demonstrate this scheme for silica and fluoride fibers, indicating ultimate limitations as well as the possibility of compression down to the single-cycle regime. Such output pulses appear ideally suited as seed sources for parametric amplification schemes in the mid-infrared.
- ItemSelf-compression of 120 fs pulses in a white-light filament(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2010) Bethge, Jens; Steinmeyer, Günter; Stibenz, Gero; Staudt, Peter; Brée, Carsten; Demircan, Ayhan; Redlin, Harald; Düsterer, StefanSelf-compression of pulses with >100 fs input pulse duration from a 10 Hz laser system is experimentally demonstrated, with a compression factor of 3.3 resulting in output pulse durations of 35 fs. This measurement substantially widens the range of applicability of this compression method, enabling self-compression of pulsed laser sources that neither exhibit extremely low pulse-to-pulse energy fluctuations nor a particularly clean beam profile. The experimental demonstration is numerically modeled, revealing the exact same mechanisms at work as at shorter input pulse duration. Additionally, the role of controlled beam clipping with an adjustable aperture is numerically substantiated
- ItemSaturation of the all-optical Kerr effect(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2010) Brée, Carsten; Demircan, Ayhan; Steinmeyer, GünterSaturation of the intensity dependence of the refractive index is directly computed from ionization rates via a Kramers-Kronig transform. The linear intensity dependence and its dispersion are found in excellent agreement with complete quantum mechanical orbital computations. Higher-order terms concur with solutions of the time-dependent Schrödinger equation. Expanding the formalism to all orders up to the ionization potential of the atom, we derive a model for saturation of the Kerr effect. This model widely confirms recently published and controversially discussed experimental data and corroborates the importance of higher-order Kerr terms for filamentation.
- ItemPlasma induced pulse breaking in filamentary self-compression(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2009) Brée, Carsten; Demircan, Ayhan; Skupin, Stefan; Berg´e, Luc; Steinmeyer, GünterA plasma induced temporal break-up in filamentary propagation has recently been identified as one of the key events in the temporal self-compression of femtosecond laser pulses. An analysis of the Nonlinear Schrödinger Equation coupled to a noninstantaneous plasma response yields a set of stationary states. This analysis clearly indicates that the emergence of double-hump, characteristically asymmetric temporal on-axis intensity profiles in regimes where plasma defocusing saturates the optical collapse caused by Kerr self-focusing is an inherent property of the underlying dynamical model.
- ItemRogue wave formation by accelerated solitons at an optical event horizon(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2013) Demircan, Ayhan; Amiranashvili, Shalva; Brée, Carsten; Mahnke, Christoph; Mitschke, Fedor; Steinmeyer, GünterRogue waves, by definition, are rare events of extreme amplitude, but at the same time they are frequent in the sense that they can exist in a wide range of physical contexts. While many mechanisms have been demonstrated to explain the appearance of rogue waves in various specific systems, there is no known generic mechanism or general set of criteria shown to rule their appearance. Presupposing only the existence of a nonlinear Schrödinger-type equation together with a concave dispersion profile around a zero dispersion wavelength we demonstrate that solitons may experience acceleration and strong reshaping due to the interaction with continuum radiation, giving rise to extreme-value phenomena. The mechanism is independent of the optical Raman effect. A strong increase of the peak power is accompanied by a mild increase of the pulse energy and carrier frequency, whereas the photon number of the soliton remains practically constant. This reshaping mechanism is particularly robust and is naturally given in optics in the supercontinuum generation process.
- ItemKramers-Kronig relations and high order nonlinear susceptibilities(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2011) Brée, Carsten; Demircan, Ayhan; Steinmeyer, GünterAs previous theoretical results recently revealed, a Kramers-Kronig transform of multiphoton absorption rates allows for a precise prediction on the dispersion of the nonlinear refractive index $n_2$ in the near IR. It was shown that this method allows to reproduce recent experimental results on the importance of the higher-order Kerr effect. Extending these results, the current manuscript provides the dispersion of $n_2$ for all noble gases in excellent agreement with reference data. It is furthermore established that the saturation and inversion of the nonlinear refractive index is highly dispersive with wavelength, which indicates the existence of different filamentation regimes. While shorter laser wavelengths favor the well-established plasma clamping regime, the influence of the higher-order Kerr effect dominates in the long wavelength regime.
- ItemCascaded self-compression of femtosecond pulses in filaments(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2010) Brée, Carsten; Bethge, Jens; Skupin, Stefan; Demircan, Ayhan; Steinmeyer, GünterHighly nonlinear wave propagation scenarios hold the potential to serve for energy concentration or pulse duration reduction of the input wave form, provided that a small range of input parameters be maintained. In particular when phenomena like rogue-wave formation or few-cycle optical pulses generation come into play, it becomes increasingly difficult to maintain control of the waveforms. Here we suggest an alternative approach towards the control of waveforms in a highly nonlinear system. Cascading pulse self-compression cycles at reduced nonlinearity limits the increase of input parameter sensitivity while still enabling an enhanced compression effect. This cascaded method is illustrated by experiments and in numerical simulations of the Nonlinear Schrödinger Equation, simulating the propagation of short optical pulses in a self-generated plasma.
- ItemMethod for computing the nonlinear refractive index via Keldysh theory(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2008) Brée, Carsten; Demircan, Ayhan; Steinmeyer, GünterBy making use of the multiphoton limit of Keldysh theory, we show that for the case of two-photon absorption a Kramers-Kronig expansion can be used to calculate the nonlinear refractive index for different wavelenghts. We apply this method to various inert gases and compare the obtained numerical values to different experimental and theoretical results for the dispersion of the Kerr nonlinearity.