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- ItemModelling lidar-relevant optical properties of complex mineral dust aerosols(Milton Park : Taylor & Francis, 2017) Gasteiger, Josef; Wiegner, Matthias; Groß, Silke; Freudenthaler, Volker; Toledano, Carlos; Tesche, Matthias; Kandler, KonradWe model lidar-relevant optical properties of mineral dust aerosols and compare the modelling results with optical properties derived from lidar measurements during the SAMUM field campaigns. The Discrete Dipole Approximation is used for optical modelling of single particles. For modelling of ensemble properties, the desert aerosol type of the OPAC aerosol dataset is extended by mixtures of absorbing and non-absorbing irregularly shaped mineral dust particles. Absorbing and non-absorbing particles are mixed to mimic the natural mineralogical inhomogeneity of dust particles. A sensitivity study reveals that the mineralogical inhomogeneity is critical for the lidar ratio at short wavelengths; it has to be considered for agreement with the observed wavelength dependence of the lidar ratio. The amount of particles with low aspect ratios (about 1.4 and lower) affects the lidar ratio at any lidar wavelength; their amount has to be low for agreement with SAMUM observations. Irregularly shaped dust particles with typical refractive indices, in general, have higher linear depolarization ratios than corresponding spheroids, and improve the agreement with the observations.
- ItemCharacterization of the planetary boundary layer during SAMUM-2 by means of lidar measurements(Milton Park : Taylor & Francis, 2017) Groß, Silke; Gasteiger, Josef; Freudenthaler, Volker; Wiegner, Matthias; Geiß, Alexander; Schladitz, Alexander; Toledano, Carlos; Kandler, Konrad; Tesche, Matthias; Ansmann, Albert; Wiedensohler, AlfredMeasurements with two Raman-depolarization lidars of the Meteorological Institute of the Ludwig-Maximilians- Universit¨at, M¨unchen, Germany, performed during SAMUM-2, were used to characterize the planetary boundary layer (PBL) over Praia, Cape Verde. A novel approach was used to determine the volume fraction of dust υd in the PBL. This approach primarily relies on accurate measurements of the linear depolarization ratio. Comparisons with independent in situ measurements showed the reliability of this approach. Based on our retrievals, two different phases could be distinguished within the measurement period of almost one month. The first (22–31 January 2008) was characterized by high aerosol optical depth (AOD) in the PBL and large υd > 95%. During the second phase, the AOD in the PBL was considerably lower and υd less than ∼40%. These findings were in very good agreement with ground based in situ measurements, when ambient volume fractions are considered that were calculated from the actual measurements of the dry volume fraction. Only in cases when dust was not the dominating aerosol component (second phase), effects due to hygroscopic growth became important.
- ItemCharacterization of Saharan dust, marine aerosols and mixtures of biomass-burning aerosols and dust by means of multi-wavelength depolarization and Raman lidar measurements during SAMUM 2(Milton Park : Taylor & Francis, 2017) Groß, Silke; Tesche, Matthias; Freudenthaler, Volker; Toledano, Carlos; Wiegner, Matthias; Ansmann, Albert; Althausen, Dietrich; Seefeldner, MeinhardThe particle linear depolarization ratio δp of Saharan dust, marine aerosols and mixtures of biomass-burning aerosols from southern West Africa and Saharan dust was determined at three wavelengths with three lidar systems during the SAharan Mineral dUst experiMent 2 at the airport of Praia, Cape Verde, between 22 January and 9 February 2008. The lidar ratio Sp of these major types of tropospheric aerosols was analysed at two wavelengths. For Saharan dust, we find wavelength dependent mean particle linear depolarization ratios δp of 0.24–0.27 at 355 nm, 0.29–0.31 at 532 nm and 0.36–0.40 at 710 nm, and wavelength independent mean lidar ratios Sp of 48–70 sr. Mixtures of biomass-burning aerosols and dust show wavelength independent values of δp and Sp between 0.12–0.23 and 57–98 sr, respectively. The mean values of marine aerosols range independent of wavelength for δp from 0.01 to 0.03 and for Sp from 14 to 24 sr.