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Sporadic Ca and Ca+ layers at mid-latitudes: Simultaneous observations and implications for their formation

2001, Gerding, M., Alpers, M., Höffner, J., von Zahn, U.

We report on the observations of 188 sporadic layers of either Ca atoms and/or Ca ions that we have observed during 112 nights of lidar soundings of Ca, and 58 nights of Ca+ soundings, at Kühlungsborn, Germany (54° N, 12° E). The Ca+ soundings have been performed simultaneously and in a common volume with the Ca soundings by two separate lidars. Correlations between sporadic neutral and ionized metal layers are demonstrated through four case studies. A systematic study of the variations of occurrence of sporadic Ca and Ca+ layers reveals that neutral and ionized Ca layers are not as closely correlated as expected earlier: (a) The altitude distribution shows the simultaneous occurrence of both sporadic Ca and Ca+ layers to be most likely only in the narrow altitude range between 90 and 95 km. Above that region, in the lower thermosphere, the sporadic ion layers are much more frequent than atom layers. Below 90 km only very few sporadic layers have been observed; (b) The seasonal variation of sporadic Ca layers exhibits a minimum of occurrence in summer, while sporadic Ca+ layers do not show a significant seasonal variation (only the dense Ca+ layers appear to have a maximum in summer). At mid-latitudes sporadic Ca layers are more frequent than sporadic layers of other atmospheric metals like Na or K. For the explanation of our observations new formation mechanisms are discussed.

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The noctilucent cloud (NLC) display during the ECOMA/MASS sounding rocket flights on 3 August 2007: Morphology on global to local scales

2009, Baumgarten, G., Fiedler, J., Fricke, K.H., Gerding, M., Hervig, M., Hoffmann, P., Müller, N., Pautet, P.-D., Rapp, M., Robert, C., Rusch, D., von Savigny, C., Singer, W.

During the ECOMA/MASS rocket campaign large scale NLC/PMC was observed by satellite, lidar and camera from polar to mid latitudes. We examine the observations from different instruments to investigate the morphology of the cloud. Satellite observations show a planetary wave 2 structure. Lidar observations from Kühlungsborn (54° N), Esrange (68° N) and ALOMAR (69° N) show a highly dynamic NLC layer. Under favorable solar illumination the cloud is also observable by ground-based cameras. The cloud was detected by cameras from Trondheim (63° N), Juliusruh (55° N) and Kühlungsborn. We investigate planetary scale morphology and local scale gravity wave structures, important for the interpretation of the small scale rocket soundings. We compare in detail the lidar observations with the NLC structure observed by the camera in Trondheim. The ALOMAR RMR-lidar observed only a faint NLC during the ECOMA launch window, while the camera in Trondheim showed a strong NLC display in the direction of ALOMAR. Using the high resolution camera observations (t~30 s, Δx<5 km) and the wind information from the meteor radar at ALOMAR we investigate the formation and destruction of NLC structures. We observe that the NLC brightness is reduced by a factor of 20–40 within 100 s which can be caused by a temperature about 15 K above the frostpoint temperature. A horizontal temperature gradient of more than 3 K/km is estimated.

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Vortex-averaged Arctic ozone depletion in the winter 2002/2003

2005, Christensen, T., Knudsen, B.M., Streibel, M., Andersen, S.B., Benesova, A., Braathen, G., Claude, H., Davies, J., De Backer, H., Dier, H., Dorokhov, V., Gerding, M., Gil, M., Henchoz, B., Kelder, H., Kivi, R., Kyrö, E., Litynska, Z., Moore, D., Peters, G., Skrivankova, P., Stübi, R., Turunen, T., Vaughan, G., Viatte, P., Vik, A.F., von der Gathen, P.

A total ozone depletion of 68±7 Dobson units between 380 and 525K from 10 December 2002 to 10 March 2003 is derived from ozone sonde data by the vortex-average method, taking into account both diabatic descent of the air masses and transport of air into the vortex. When the vortex is divided into three equal-area regions, the results are 85±9DU for the collar region (closest to the edge), 52±5DU for the vortex centre and 68±7DU for the middle region in between centre and collar. Our results compare well with other studies: We find good agreement with ozone loss deduced from SAOZ data, with results inferred from POAM III observations and with results from tracer-tracer correlations using HF as the long-lived tracer. We find a higher ozone loss than that deduced by tracer-tracer correlations using CH4. We have made a careful comparison with Match results: The results were recalculated using a common time period, vortex edge definition and height interval. The two methods generally compare very well, except at the 475K level which exhibits an unexplained discrepancy.

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Observation of an unusual mid-stratospheric aerosol layer in the Arctic: Possible sources and implications for polar vortex dynamics

2003, Gerding, M., Baumgarten, G., Blum, U., Thayer, J.P., Fricke, K.-H., Neuber, R., Fiedler, J.

By the beginning of winter 2000/2001, a mysterious stratospheric aerosol layer had been detected by four different Arctic lidar stations. The aerosol layer was observed first on 16 November 2000, at an altitude of about 38 km near Søndre Strømfjord, Greenland (67° N, 51° W) and on 19 November 2000, near Andenes, Norway (69° N, 16° E). Subsequently, in early December 2000, the aerosol layer was observed near Kiruna, Sweden (68° N, 21° E) and Ny-Ålesund, Spitsbergen (79° N, 12° E). No mid-latitude lidar station observed the presence of aerosols in this altitude region. The layer persisted throughout the winter 2000/2001, at least up to 12 February 2001. In November 2000, the backscatter ratio at a wavelength of 532 nm was up to 1.1, with a FWHM of about 2.5 km. By early February 2001, the layer had sedimented from an altitude of 38 km to about 26 km. Measurements at several wavelengths by the ALOMAR and Koldewey lidars indicate the particle size was between 30 and 50 nm. Depolarisation measurements reveal that the particles in the layer are aspherical, hence solid. In the mid-stratosphere, the ambient atmospheric temperature was too high to support in situ formation or existence of cloud particles consisting of ice or an acid-water solution. Furthermore, in the year 2000 there was no volcanic eruption, which could have injected aerosols into the upper stratosphere. Therefore, other origins of the aerosol, such as meteoroid debris, condensed rocket fuel, or aerosols produced under the influence of charged solar particles, will be discussed in the paper. Trajectory calculations illustrate the path of the aerosol cloud within the polar vortex and are used to link the observations at the different lidar sites. From the descent rate of the layer and particle sedimentation rates, the mean down-ward motion of air within the polar vortex was estimated to be about 124 m/d between 35 and 30 km, with higher values at the edge of the vortex.

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Validation of the Atmospheric Chemistry Experiment (ACE) version 2.2 temperature using ground-based and space-borne measurements

2008, Sica, R.J., Izawa, M.R.M., Walker, K.A., Boone, C., Petelina, S.V., Argall, P.S., Bernath, P., Burns, G.B., Catoire, V., Collins, R.L., Daffer, W.H., De Clercq, C., Fan, Z.Y., Firanski, B.J., French, W.J.R., Gerard, P., Gerding, M., Granville, J., Innis, J.L., Keckhut, P., Kerzenmacher, T., Klekociuk, A.R., Kyrö, E., Lambert, J.C., Llewellyn, E.J., Manney, G.L., McDermid, I.S., Mizutani, K., Murayama, Y., Piccolo, C., Raspollini, P., Ridolfi, M., Robert, C., Steinbrecht, W., Strawbridge, K.B., Strong, K., Stübi, R., Thurairajah, B.

An ensemble of space-borne and ground-based instruments has been used to evaluate the quality of the version 2.2 temperature retrievals from the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS). The agreement of ACE-FTS temperatures with other sensors is typically better than 2 K in the stratosphere and upper troposphere and 5 K in the lower mesosphere. There is evidence of a systematic high bias (roughly 3–6 K) in the ACE-FTS temperatures in the mesosphere, and a possible systematic low bias (roughly 2 K) in ACE-FTS temperatures near 23 km. Some ACE-FTS temperature profiles exhibit unphysical oscillations, a problem fixed in preliminary comparisons with temperatures derived using the next version of the ACE-FTS retrieval software. Though these relatively large oscillations in temperature can be on the order of 10 K in the mesosphere, retrieved volume mixing ratio profiles typically vary by less than a percent or so. Statistical comparisons suggest these oscillations occur in about 10% of the retrieved profiles. Analysis from a set of coincident lidar measurements suggests that the random error in ACE-FTS version 2.2 temperatures has a lower limit of about ±2 K.

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Non-coincident inter-instrument comparisons of ozone measurements using quasi-conservative coordinates

2004, Lait, L.R., Newman, P.A., Schoeberl, M.R., McGee, T., Twigg, L., Browell, E.V., Fenn, M.A., Grant, W.B., Butler, C.F., Bevilacqua, R., Davies, J., DeBacker, H., Andersen, S.B., Kyrö, E., Kivi, E., von der Gathen, P., Claude, H., Benesova, A., Skrivankova, P., Dorokhov, V., Zaitcev, I., Braathen, G., Gil, M., Litynska, Z., Moore, D., Gerding, M.

Ozone measurements from ozonesondes, AROTAL, DIAL, and POAM III instruments during the SOLVE-2/VINTERSOL period are composited in a time-varying, flow-following quasi-conservative (PV-θ) coordinate space; the resulting composites from each instrument are mapped onto the other instruments' locations and times. The mapped data are then used to intercompare data from the different instruments. Overall, the four ozone data sets are found to be in good agreement. AROTAL shows somewhat lower values below 16 km, and DIAL has a positive bias at the upper limits of its altitude range. These intercomparisons are consistent with those obtained from more conventional near-coincident profiles, where available. Although the PV-θ mapping technique entails larger uncertainties of individual profile differences compared to direct near-coincident comparisons, the ability to include much larger numbers of comparisons can make this technique advantageous.

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Seasonal variation of nocturnal temperatures between 1 and 105 km altitude at 54° N observed by lidar

2008, Gerding, M., Höffner, J., Lautenbach, J., Rauthe, M., Lübken, F.-J.

Temperature soundings are performed by lidar at the mid-latitude station of Kühlungsborn (Germany, 54° N, 12° E). The profiles cover the complete range from the lower troposphere (~1 km) to the lower thermosphere (~105 km) by simultaneous and co-located operation of a Rayleigh-Mie-Raman lidar and a potassium resonance lidar. Observations have been done during 266 nights between June 2002 and July 2007, each of 3–15 h length. This large and unique data set provides comprehensive information on the altitudinal and seasonal variation of temperatures from the troposphere to the lower thermosphere. The remaining day-to-day-variability is strongly reduced by harmonic fits at constant altitude levels and a representative data set is achieved. This data set reveals a two-level mesopause structure with an altitude of about 86–87 km (~144 K) in summer and ~102 km (~170 K) during the rest of the year. The average stratopause altitude is ~48 km throughout the whole year, with temperatures varying between 258 and 276 K. From the fit parameters amplitudes and phases of annual, semi-annual, and quarter-annual variations are derived. The amplitude of the annual component is largest with amplitudes of up to 30 K in 85 km, while the quarter-annual variation is smallest and less than 3 K at all altitudes. The lidar data set is compared with ECMWF temperatures below about 70 km altitude and reference data from the NRLMSISE-00 model above. Apart from the temperature soundings the aerosol backscatter ratio is measured between 20 and 35 km. The seasonal variation of these values is presented here for the first time.

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Temperature lidar measurements from 1 to 105 km altitude using resonance, Rayleigh, and Rotational Raman scattering

2004, Alpers, M., Eixmann, R., Fricke-Begemann, C., Gerding, M., Höffner, J.

For the first time, three different temperature lidar methods are combined to obtain time-resolved complete temperature profiles with high altitude resolution over an altitude range from the planetary boundary layer up to the lower thermosphere (about 1–105 km). The Leibniz-Institute of Atmospheric Physics (IAP) at Kühlungsborn, Germany (54° N, 12° E) operates two lidar instruments, using three different temperature measurement methods, optimized for three altitude ranges: (1) Probing the spectral Doppler broadening of the potassium D1 resonance lines with a tunable narrow-band laser allows atmospheric temperature profiles to be determined at metal layer altitudes (80–105 km). (2) Between about 20 and 90 km, temperatures were calculated from Rayleigh backscattering by air molecules, where the upper start values for the calculation algorithm were taken from the potassium lidar results. Correction methods have been applied to account for, e.g. Rayleigh extinction or Mie scattering of aerosols below about 32 km. (3) At altitudes below about 25 km, backscattering in the Rotational Raman lines is strong enough to obtain temperatures by measuring the temperature dependent spectral shape of the Rotational Raman spectrum. This method works well down to about 1 km. The instrumental configurations of the IAP lidars were optimized for a 3–6 km overlap of the temperature profiles at the method transition altitudes. We present two night-long measurements with clear wave structures propagating from the lower stratosphere up to the lower thermosphere.