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High-spectral-resolution terahertz imaging with a quantum-cascade laser

2016, Hagelschuer, Till, Rothbart, Nick, Richter, Heiko, Wienold, Martin, Schrottke, Lutz, Grahn, Holger T., Hübers, Heinz-Wilhelm

We report on a high-spectral-resolution terahertz imaging system operating with a multi-mode quantum-cascade laser (QCL), a fast scanning mirror, and a sensitive Ge:Ga detector. By tuning the frequency of the QCL, several spectra can be recorded in 1.5 s during the scan through a gas cell filled with methanol (CH3OH). These experiments yield information about the local absorption and the linewidth. Measurements with a faster frame rate of up to 3 Hz allow for the dynamic observation of CH3OH gas leaking from a terahertz-transparent tube into the evacuated cell. In addition to the relative absorption, the local pressure is mapped by exploiting the effect of pressure broadening.

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Real-time gas sensing based on optical feedback in a terahertz quantum-cascade laser

2017, Hagelschuer, Till, Wienold, Martin, Richter, Heiko, Schrottke, Lutz, Grahn, Holger T., Hübers, Heinz-Wilhelm

We report on real-time gas sensing with a terahertz quantum-cascade laser (QCL). The method is solely based on the modulation of the external cavity length, exploiting the intermediate optical feedback regime. While the QCL is operated in continuous-wave mode, optical feedback results in a change of the QCL frequency as well as its terminal voltage. The first effect is exploited to tune the lasing frequency across a molecular absorption line. The second effect is used for the detection of the self-mixing signal. This allows for fast measurement times on the order of 10 ms per spectrum and for real-time measurements of gas concentrations with a rate of 100 Hz. This technique is demonstrated with a mixture of D2O and CH3OD in an absorption cell.