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- ItemImpacts of enhanced weathering on biomass production for negative emission technologies and soil hydrology(Katlenburg-Lindau [u.a.] : Copernicus, 2020) De Oliveira Garcia, Wagner; Amann, Thorben; Hartmann, Jens; Karstens, Kristine; Popp, Alexander; Boysen, Lena R.; Smith, Pete; Goll, DanielLimiting global mean temperature changes to well below 2 °C likely requires a rapid and large-scale deployment of negative emission technologies (NETs). Assessments so far have shown a high potential of biomass-based terrestrial NETs, but only a few assessments have included effects of the commonly found nutrient-deficient soils on biomass production. Here, we investigate the deployment of enhanced weathering (EW) to supply nutrients to areas of afforestation-reforestation and naturally growing forests (AR) and bioenergy grasses (BG) that are deficient in phosphorus (P), besides the impacts on soil hydrology. Using stoichiometric ratios and biomass estimates from two established vegetation models, we calculated the nutrient demand of AR and BG. Insufficient geogenic P supply limits C storage in biomass. For a mean P demand by AR and a lowgeogenic-P-supply scenario, AR would sequester 119 Gt C in biomass; for a high-geogenic-P-supply and low-AR-Pdemand scenario, 187 Gt C would be sequestered in biomass; and for a low geogenic P supply and high AR P demand, only 92 GtC would be accumulated by biomass. An average amount of ∼ 150 Gt basalt powder applied for EW would be needed to close global P gaps and completely sequester projected amounts of 190 Gt C during the years 2006-2099 for the mean AR P demand scenario (2-362 Gt basalt powder for the low-AR-P-demand and for the high-AR-P-demand scenarios would be necessary, respectively). The average potential of carbon sequestration by EW until 2099 is ∼ 12 GtC (∼ 0:2-∼ 27 Gt C) for the specified scenarios (excluding additional carbon sequestration via alkalinity production). For BG, 8 kg basaltm2 a1 might, on average, replenish the exported potassium (K) and P by harvest. Using pedotransfer functions, we show that the impacts of basalt powder application on soil hydraulic conductivity and plant-Available water, to close predicted P gaps, would depend on basalt and soil texture, but in general the impacts are marginal. We show that EW could potentially close the projected P gaps of an AR scenario and nutrients exported by BG harvest, which would decrease or replace the use of industrial fertilizers. Besides that, EW ameliorates the soil's capacity to retain nutrients and soil pH and replenish soil nutrient pools. Lastly, EW application could improve plant-Available-water capacity depending on deployed amounts of rock powder - adding a new dimension to the coupling of land-based biomass NETs with EW. © 2020 Royal Society of Chemistry. All rights reserved.
- ItemPotential and costs of carbon dioxide removal by enhanced weathering of rocks(Bristol : IOP Publishing, 2018) Strefler, Jessica; Amann, Thorben; Bauer, Nico; Kriegler, Elmar; Hartmann, JensThe chemical weathering of rocks currently absorbs about 1.1 Gt CO2 a−1 being mainly stored as bicarbonate in the ocean. An enhancement of this slow natural process could remove substantial amounts of CO2 from the atmosphere, aiming to offset some unavoidable anthropogenic emissions in order to comply with the Paris Agreement, while at the same time it may decrease ocean acidification. We provide the first comprehensive assessment of economic costs, energy requirements, technical parameterization, and global and regional carbon removal potential. The crucial parameters defining this potential are the grain size and weathering rates. The main uncertainties about the potential relate to weathering rates and rock mass that can be integrated into the soil. The discussed results do not specifically address the enhancement of weathering through microbial processes, feedback of geogenic nutrient release, and bioturbation. We do not only assess dunite rock, predominantly bearing olivine (in the form of forsterite) as the mineral that has been previously proposed to be best suited for carbon removal, but focus also on basaltic rock to minimize potential negative side effects. Our results show that enhanced weathering is an option for carbon dioxide removal that could be competitive already at 60 US $ t−1 CO2 removed for dunite, but only at 200 US $ t−1 CO2 removed for basalt. The potential carbon removal on cropland areas could be as large as 95 Gt CO2 a−1 for dunite and 4.9 Gt CO2 a−1 for basalt. The best suited locations are warm and humid areas, particularly in India, Brazil, South-East Asia and China, where almost 75% of the global potential can be realized. This work presents a techno-economic assessment framework, which also allows for the incorporation of further processes.
- ItemNegative emissions—Part 1: Research landscape and synthesis(Bristol : IOP Publ., 2018) Minx, Jan C.; Lamb, William F.; Callaghan, Max W.; Fuss, Sabine; Hilaire, Jérôme; Creutzig, Felix; Amann, Thorben; Beringer, Tim; de Oliveira Garcia, Wagner; Hartmann, Jens; Khanna, Tarun; Lenzi, Dominic; Luderer, Gunnar; Nemet, Gregory F.; Rogelj, Joeri; Smith, Pete; Vicente Vicente, José Luis; Wilcox, Jennifer; del Mar Zamora Dominguez, MariaWith the Paris Agreement's ambition of limiting climate change to well below 2 °C, negative emission technologies (NETs) have moved into the limelight of discussions in climate science and policy. Despite several assessments, the current knowledge on NETs is still diffuse and incomplete, but also growing fast. Here, we synthesize a comprehensive body of NETs literature, using scientometric tools and performing an in-depth assessment of the quantitative and qualitative evidence therein. We clarify the role of NETs in climate change mitigation scenarios, their ethical implications, as well as the challenges involved in bringing the various NETs to the market and scaling them up in time. There are six major findings arising from our assessment: first, keeping warming below 1.5 °C requires the large-scale deployment of NETs, but this dependency can still be kept to a minimum for the 2 °C warming limit. Second, accounting for economic and biophysical limits, we identify relevant potentials for all NETs except ocean fertilization. Third, any single NET is unlikely to sustainably achieve the large NETs deployment observed in many 1.5 °C and 2 °C mitigation scenarios. Yet, portfolios of multiple NETs, each deployed at modest scales, could be invaluable for reaching the climate goals. Fourth, a substantial gap exists between the upscaling and rapid diffusion of NETs implied in scenarios and progress in actual innovation and deployment. If NETs are required at the scales currently discussed, the resulting urgency of implementation is currently neither reflected in science nor policy. Fifth, NETs face severe barriers to implementation and are only weakly incentivized so far. Finally, we identify distinct ethical discourses relevant for NETs, but highlight the need to root them firmly in the available evidence in order to render such discussions relevant in practice.
- ItemNegative emissions—Part 3: Innovation and upscaling(Bristol : IOP Publ., 2018) Nemet, Gregory F.; Callaghan, Max W.; Creutzig, Felix; Fuss, Sabine; Hartmann, Jens; Hilaire, Jérôme; Lamb, William F.; Minx, Jan C.; Rogers, Sophia; Smith, PeteWe assess the literature on innovation and upscaling for negative emissions technologies (NETs) using a systematic and reproducible literature coding procedure. To structure our review, we employ the framework of sequential stages in the innovation process, with which we code each NETs article in innovation space. We find that while there is a growing body of innovation literature on NETs, 59% of the articles are focused on the earliest stages of the innovation process, 'research and development' (R&D). The subsequent stages of innovation are also represented in the literature, but at much lower levels of activity than R&D. Distinguishing between innovation stages that are related to the supply of the technology (R&D, demonstrations, scale up) and demand for the technology (demand pull, niche markets, public acceptance), we find an overwhelming emphasis (83%) on the supply side. BECCS articles have an above average share of demand-side articles while direct air carbon capture and storage has a very low share. Innovation in NETs has much to learn from successfully diffused technologies; appealing to heterogeneous users, managing policy risk, as well as understanding and addressing public concerns are all crucial yet not well represented in the extant literature. Results from integrated assessment models show that while NETs play a key role in the second half of the 21st century for 1.5 °C and 2 °C scenarios, the major period of new NETs deployment is between 2030 and 2050. Given that the broader innovation literature consistently finds long time periods involved in scaling up and deploying novel technologies, there is an urgency to developing NETs that is largely unappreciated. This challenge is exacerbated by the thousands to millions of actors that potentially need to adopt these technologies for them to achieve planetary scale. This urgency is reflected neither in the Paris Agreement nor in most of the literature we review here. If NETs are to be deployed at the levels required to meet 1.5 °C and 2 °C targets, then important post-R&D issues will need to be addressed in the literature, including incentives for early deployment, niche markets, scale-up, demand, and—particularly if deployment is to be hastened—public acceptance.
- ItemNegative emissions—Part 2: Costs, potentials and side effects(Bristol : IOP Publ., 2018) Fuss, Sabine; Lamb, William F.; Callaghan, Max W.; Hilaire, Jérôme; Creutzig, Felix; Amann, Thorben; Beringer, Tim; de Oliveira Garcia, Wagner; Hartmann, Jens; Khanna, Tarun; Luderer, Gunnar; Nemet, Gregory F.; Rogelj, Joeri; Smith, Pete; Vicente Vicente, José Luis; Wilcox, Jennifer; del Mar Zamora Dominguez, Maria; Minx, Jan C.The most recent IPCC assessment has shown an important role for negative emissions technologies (NETs) in limiting global warming to 2 °C cost-effectively. However, a bottom-up, systematic, reproducible, and transparent literature assessment of the different options to remove CO2 from the atmosphere is currently missing. In part 1 of this three-part review on NETs, we assemble a comprehensive set of the relevant literature so far published, focusing on seven technologies: bioenergy with carbon capture and storage (BECCS), afforestation and reforestation, direct air carbon capture and storage (DACCS), enhanced weathering, ocean fertilisation, biochar, and soil carbon sequestration. In this part, part 2 of the review, we present estimates of costs, potentials, and side-effects for these technologies, and qualify them with the authors' assessment. Part 3 reviews the innovation and scaling challenges that must be addressed to realise NETs deployment as a viable climate mitigation strategy. Based on a systematic review of the literature, our best estimates for sustainable global NET potentials in 2050 are 0.5–3.6 GtCO2 yr−1 for afforestation and reforestation, 0.5–5 GtCO2 yr−1 for BECCS, 0.5–2 GtCO2 yr−1 for biochar, 2–4 GtCO2 yr−1 for enhanced weathering, 0.5–5 GtCO2 yr−1 for DACCS, and up to 5 GtCO2 yr−1 for soil carbon sequestration. Costs vary widely across the technologies, as do their permanency and cumulative potentials beyond 2050. It is unlikely that a single NET will be able to sustainably meet the rates of carbon uptake described in integrated assessment pathways consistent with 1.5 °C of global warming.
- ItemThe Earth system model CLIMBER-X v1.0 - Part 2: The global carbon cycle(Katlenburg-Lindau : Copernicus, 2023) Willeit, Matteo; Ilyina, Tatiana; Liu, Bo; Heinze, Christoph; Perrette, Mahé; Heinemann, Malte; Dalmonech, Daniela; Brovkin, Victor; Munhoven, Guy; Börker, Janine; Hartmann, Jens; Romero-Mujalli, Gibran; Ganopolski, AndreyThe carbon cycle component of the newly developed Earth system model of intermediate complexity CLIMBER-X is presented. The model represents the cycling of carbon through the atmosphere, vegetation, soils, seawater and marine sediments. Exchanges of carbon with geological reservoirs occur through sediment burial, rock weathering and volcanic degassing. The state-of-the-art HAMOCC6 model is employed to simulate ocean biogeochemistry and marine sediment processes. The land model PALADYN simulates the processes related to vegetation and soil carbon dynamics, including permafrost and peatlands. The dust cycle in the model allows for an interactive determination of the input of the micro-nutrient iron into the ocean. A rock weathering scheme is implemented in the model, with the weathering rate depending on lithology, runoff and soil temperature. CLIMBER-X includes a simple representation of the methane cycle, with explicitly modelled natural emissions from land and the assumption of a constant residence time of CH4 in the atmosphere. Carbon isotopes 13C and 14C are tracked through all model compartments and provide a useful diagnostic for model-data comparison. A comprehensive evaluation of the model performance for the present day and the historical period shows that CLIMBER-X is capable of realistically reproducing the historical evolution of atmospheric CO2 and CH4 but also the spatial distribution of carbon on land and the 3D structure of biogeochemical ocean tracers. The analysis of model performance is complemented by an assessment of carbon cycle feedbacks and model sensitivities compared to state-of-the-art Coupled Model Intercomparison Project Phase 6 (CMIP6) models. Enabling an interactive carbon cycle in CLIMBER-X results in a relatively minor slow-down of model computational performance by ∼ 20 % compared to a throughput of ∼ 10 000 simulation years per day on a single node with 16 CPUs on a high-performance computer in a climate-only model set-up. CLIMBER-X is therefore well suited to investigating the feedbacks between climate and the carbon cycle on temporal scales ranging from decades to >100000 years.