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    Comparing two years of Saharan dust source activation obtained by regional modelling and satellite observations
    (München : European Geopyhsical Union, 2013) Tegen, I.; Schepanski, K.; Heinold, B.
    A regional-scale dust model is used to simulate Saharan dust emissions and atmospheric distributions in the years 2007 and 2008. The model results are compared to dust source activation events compiled from infrared dust index imagery from the geostationary Meteosat Second Generation (MSG) satellite. The observed morning maximum in dust source activation frequencies indicates that the breakdown of nocturnal low level jets is an important mechanism for dust source activation in the Sahara. The comparison shows that the time of the day of the onset of dust emission is delayed in the model compared to the observations. Also, the simulated number of dust emission events associated with nocturnal low level jets in mountainous regions is underestimated in the model. The MSG dust index observations indicate a strong increase in dust source activation frequencies in the year 2008 compared to 2007. The difference between the two years is less pronounced in the model. Observations of dust optical thickness, e.g. at stations of the sunphotometer network AERONET, do not show such increase, in agreement with the model results. This indicates that the number of observed dust activation events is only of limited use for estimating actual dust emission fluxes in the Sahara. The ability to reproduce interannual variability of Saharan dust with models remains an important challenge for understanding the controls of the atmospheric dust load.
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    Mass deposition fluxes of Saharan mineral dust to the tropical northeast Atlantic Ocean: An intercomparison of methods
    (München : European Geopyhsical Union, 2014) Niedermeier, N.; Held, A.; Müller, T.; Heinold, B.; Schepanski, K.; Tegen, I.; Kandler, K.; Ebert, M.; Weinbruch, S.; Read, K.; Lee, J.; Fomba, K.W.; Müller, K.; Herrmann, H.; Wiedensohler, A.
    Mass deposition fluxes of mineral dust to the tropical northeast Atlantic Ocean were determined within this study. In the framework of SOPRAN (Surface Ocean Processes in the Anthropocene), the interaction between the atmosphere and the ocean in terms of material exchange were investigated at the Cape Verde atmospheric observatory (CVAO) on the island Sao Vicente for January 2009. Five different methods were applied to estimate the deposition flux, using different meteorological and physical measurements, remote sensing, and regional dust transport simulations. The set of observations comprises micrometeorological measurements with an ultra-sonic anemometer and profile measurements using 2-D anemometers at two different heights, and microphysical measurements of the size-resolved mass concentrations of mineral dust. In addition, the total mass concentration of mineral dust was derived from absorption photometer observations and passive sampling. The regional dust model COSMO-MUSCAT was used for simulations of dust emission and transport, including dry and wet deposition processes. This model was used as it describes the AOD's and mass concentrations realistic compared to the measurements and because it was run for the time period of the measurements. The four observation-based methods yield a monthly average deposition flux of mineral dust of 12–29 ng m−2 s−1. The simulation results come close to the upper range of the measurements with an average value of 47 ng m−2 s−1. It is shown that the mass deposition flux of mineral dust obtained by the combination of micrometeorological (ultra-sonic anemometer) and microphysical measurements (particle mass size distribution of mineral dust) is difficult to compare to modeled mass deposition fluxes when the mineral dust is inhomogeneously distributed over the investigated area.
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    How important are atmospheric depressions and mobile cyclones for emitting mineral dust aerosol in North Africa?
    (München : European Geopyhsical Union, 2014) Fiedler, S.; Schepanski, K.; Knippertz, P.; Heinold, B.; Tegen, I.
    This study presents the first quantitative estimate of the mineral dust emission associated with atmospheric depressions and mobile cyclones in North Africa. Atmospheric depressions are automatically tracked at 925 hPa based on ERA-Interim data from the European Centre for Medium-Range Weather Forecasts for 1989–2008. A set of filter criteria is applied to identify mobile cyclones, i.e. migrating and long-lived cyclones. The shorter term cyclone is used as a synonym for mobile cyclones. Dust emission is calculated with a dust emission model driven by 10 m winds and soil moisture from ERA-Interim. Emission peaks during winter and spring with spatial averages of 250–380 g m−2 per month. Comparison of the dust source activation frequency from the model against SEVIRI satellite observation shows a good agreement in the Bodélé Depression but differences in the north and west of North Africa. Depressions are abundant, particularly in summer when the Saharan heat low is situated over West Africa and during spring in the lee of the Atlas Mountains. Up to 90% (55% annually and spatially averaged) of dust emission occurs within 10 degrees of these depressions, with embedded mechanisms such as nocturnal low-level jets playing a role. Cyclones are rarer and occur primarily north of 20° N in spring in agreement with previous studies and over summertime West Africa consistent with near-surface signatures of African Easterly Waves. Dust emission within 10 degrees of cyclones peaks over Libya with up to 25% in spring. Despite the overall small contribution of 4% annually and spatially averaged, cyclones coincide with particularly intense dust emission events exceeding the climatological mean by a factor of four to eight. Soil moisture weakens dust emission during cyclone passage by about 10%.
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    Large-scale modeling of absorbing aerosols and their semi-direct effects
    (Basel : MDPI AG, 2018) Tegen, I.; Heinold, B.
    Radiative effects of absorbing black carbon and mineral dust aerosols are estimated from global aerosol climate model simulations with fixed sea surface temperatures as a boundary condition. Semi-direct effects are approximated as the residual between the total direct radiative effect and the instantaneous direct radiative effect of the simulated absorbing aerosol species. No distinction is made for aerosols from natural and anthropogenic sources. Results for global average are highly uncertain due to high model variability, but consistent with previous estimates. The global average results for black carbon aerosol semi-direct effects are small due to cancellation of regionally positive or negative effects, and may be positive or negative overall, depending on the model setup. The presence of mineral dust aerosol above dark surfaces and below a layer containing black carbon aerosol may enhance the reflectivity and act to enhance the positive radiative effect of black carbon aerosol. When mineral dust is absent the semi-direct effect at the top-of-atmosphere of black carbon aerosol from both anthropogenic and natural sources is -0.03 Wm-2, while averaging to +0.09 Wm-2 if dust is included.
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    The sensitivity of the colour of dust in MSG-SEVIRI Desert Dust infrared composite imagery to surface and atmospheric conditions
    (Göttingen : Copernicus GmbH, 2019) Banks, J.R.; Hünerbein, A.; Heinold, B.; Brindley, H.E.; Deneke, H.; Schepanski, K.
    Infrared "Desert Dust" composite imagery taken by the Spinning Enhanced Visible and InfraRed Imager (SEVIRI), onboard the Meteosat Second Generation (MSG) series of satellites above the equatorial East Atlantic, has been widely used for more than a decade to identify and track the presence of dust storms from and over the Sahara Desert, the Middle East, and southern Africa. Dust is characterised by distinctive pink colours in the Desert Dust false-colour imagery; however, the precise colour is influenced by numerous environmental properties, such as the surface thermal emissivity and skin temperature, the atmospheric water vapour content, the quantity and height of dust in the atmosphere, and the infrared optical properties of the dust itself. For this paper, simulations of SEVIRI infrared measurements and imagery have been performed using a modelling system, which combines dust concentrations simulated by the aerosol transport model COSMO-MUSCAT (COSMO: COnsortium for Small-scale MOdelling; MUSCAT: MUltiScale Chemistry Aerosol Transport Model) with radiative transfer simulations from the RTTOV (Radiative Transfer for TOVS) model. Investigating the sensitivity of the synthetic infrared imagery to the environmental properties over a 6-month summertime period from 2011 to 2013, it is confirmed that water vapour is a major control on the apparent colour of dust, obscuring its presence when the moisture content is high. Of the three SEVIRI channels used in the imagery (8.7, 10.8, and 12.0 μm), the channel at 10.8 μm has the highest atmospheric transmittance and is therefore the most sensitive to the surface skin temperature. A direct consequence of this sensitivity is that the background desert surface exhibits a strong diurnal cycle in colour, with light blue colours possible during the day and purple hues prevalent at night. In dusty scenes, the clearest pink colours arise from high-altitude dust in dry atmospheres. Elevated dust influences the dust colour primarily by reducing the contrast in atmospheric transmittance above the dust layer between the SEVIRI channels at 10.8 and 12.0 μm, thereby boosting red and pink colours in the imagery. Hence, the higher the dust altitude, the higher the threshold column moisture needed for dust to be obscured in the imagery: for a sample of dust simulated to have an aerosol optical depth (AOD) at 550 nm of 2-3 at an altitude of 3-4 km, the characteristic colour of the dust may only be impaired when the total column water vapour is particularly moist ('39 mm). Meanwhile, dust close to the surface (altitude < 1 km) is only likely to be apparent when the atmosphere is particularly dry and when the surface is particularly hot, requiring column moisture/13 mm and skin temperatures '314 K, and is highly unlikely to be apparent when the skin temperature is/300 K. Such low-altitude dust will regularly be almost invisible within the imagery, since it will usually be beneath much of the atmospheric water vapour column. It is clear that the interpretation of satellite-derived dust imagery is greatly aided by knowledge of the background environment.
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    The global aerosol-climate model echam6.3-ham2.3 -Part 1: Aerosol evaluation
    (Göttingen : Copernicus GmbH, 2019) Tegen, I.; Neubauer, D.; Ferrachat, S.; Drian, C.S.-L.; Bey, I.; Schutgens, N.; Stier, P.; Watson-Parris, D.; Stanelle, T.; Schmidt, H.; Rast, S.; Kokkola, H.; Schultz, M.; Schroeder, S.; Daskalakis, N.; Barthel, S.; Heinold, B.; Lohmann, U.
    We introduce and evaluate aerosol simulations with the global aerosol-climate model ECHAM6.3-HAM2.3, which is the aerosol component of the fully coupled aerosol-chemistry-climate model ECHAM-HAMMOZ. Both the host atmospheric climate model ECHAM6.3 and the aerosol model HAM2.3 were updated from previous versions. The updated version of the HAM aerosol model contains improved parameterizations of aerosol processes such as cloud activation, as well as updated emission fields for anthropogenic aerosol species and modifications in the online computation of sea salt and mineral dust aerosol emissions. Aerosol results from nudged and free-running simulations for the 10-year period 2003 to 2012 are compared to various measurements of aerosol properties. While there are regional deviations between the model and observations, the model performs well overall in terms of aerosol optical thickness, but may underestimate coarse-mode aerosol concentrations to some extent so that the modeled particles are smaller than indicated by the observations. Sulfate aerosol measurements in the US and Europe are reproduced well by the model, while carbonaceous aerosol species are biased low. Both mineral dust and sea salt aerosol concentrations are improved compared to previous versions of ECHAM-HAM. The evaluation of the simulated aerosol distributions serves as a basis for the suitability of the model for simulating aerosol-climate interactions in a changing climate.
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    Modelling soil dust aerosol in the Bodélé depression during the BoDEx campaign
    (München : European Geopyhsical Union, 2006) Tegen, I.; Heinold, B.; Todd, M.; Helmert, J.; Washington, R.; Dubovik, O.
    We present regional model simulations of the dust emission events during the Bodélé Dust Experiment (BoDEx) that was carried out in February and March 2005 in Chad. A box model version of the dust emission model is used to test different input parameters for the emission model, and to compare the dust emissions computed with observed wind speeds to those calculated with wind speeds from the regional model simulation. While field observations indicate that dust production occurs via self-abrasion of saltating diatomite flakes in the Bodélé, the emission model based on the assumption of dust production by saltation and using observed surface wind speeds as input parameters reproduces observed dust optical thicknesses well. Although the peak wind speeds in the regional model underestimate the highest wind speeds occurring on 10–12 March 2005, the spatio-temporal evolution of the dust cloud can be reasonably well reproduced by this model. Dust aerosol interacts with solar and thermal radiation in the regional model; it is responsible for a decrease in maximum daytime temperatures by about 5 K at the beginning the dust storm on 10 March 2005. This direct radiative effect of dust aerosol accounts for about half of the measured temperature decrease compared to conditions on 8 March. Results from a global dust model suggest that the dust from the Bodélé is an important contributor to dust crossing the African Savannah region towards the Gulf of Guinea and the equatorial Atlantic, where it can contribute up to 40% to the dust optical thickness.
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    The impact of mineral dust on cloud formation during the Saharan dust event in April 2014 over Europe
    (Göttingen : Copernicus GmbH, 2018) Weger, M.; Heinold, B.; Engler, C.; Schumann, U.; Seifert, A.; Fößig, R.; Voigt, C.; Baars, H.; Blahak, U.; Borrmann, S.; Hoose, C.; Kaufmann, S.; Krämer, M.; Seifert, P.; Senf, F.; Schneider, J.; Tegen, I.
    A regional modeling study on the impact of desert dust on cloud formation is presented for a major Saharan dust outbreak over Europe from 2 to 5 April 2014. The dust event coincided with an extensive and dense cirrus cloud layer, suggesting an influence of dust on atmospheric ice nucleation. Using interactive simulation with the regional dust model COSMO-MUSCAT, we investigate cloud and precipitation representation in the model and test the sensitivity of cloud parameters to dust-cloud and dust-radiation interactions of the simulated dust plume. We evaluate model results with ground-based and spaceborne remote sensing measurements of aerosol and cloud properties, as well as the in situ measurements obtained during the ML-CIRRUS aircraft campaign. A run of the model with single-moment bulk microphysics without online dust feedback considerably underestimated cirrus cloud cover over Germany in the comparison with infrared satellite imagery. This was also reflected in simulated upper-Tropospheric ice water content (IWC), which accounted for only 20 % of the observed values. The interactive dust simulation with COSMO-MUSCAT, including a two-moment bulk microphysics scheme and dust-cloud as well as dust-radiation feedback, in contrast, led to significant improvements. The modeled cirrus cloud cover and IWC were by at least a factor of 2 higher in the relevant altitudes compared to the noninteractive model run. We attributed these improvements mainly to enhanced deposition freezing in response to the high mineral dust concentrations. This was corroborated further in a significant decrease in ice particle radii towards more realistic values, compared to in situ measurements from the ML-CIRRUS aircraft campaign. By testing different empirical ice nucleation parameterizations, we further demonstrate that remaining uncertainties in the ice-nucleating properties of mineral dust affect the model performance at least as significantly as including the online representation of the mineral dust distribution. Dust-radiation interactions played a secondary role for cirrus cloud formation, but contributed to a more realistic representation of precipitation by suppressing moist convection in southern Germany. In addition, a too-low specific humidity in the 7 to 10 km altitude range in the boundary conditions was identified as one of the main reasons for misrepresentation of cirrus clouds in this model study.
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    Tracking the Saharan Air Layer with shipborne lidar across the tropical Atlantic
    (Hoboken, NJ : Wiley, 2014) Kanitz, T.; Engelmann, R.; Heinold, B.; Baars, H.; Skupin, A.; Ansmann, A.
    Saharan dust was observed with shipborne lidar from 60° to 20°W along 14.5°N during a 1-month transatlantic cruise of the research vessel Meteor. About 4500 km off the coast of Africa, mean extinction and backscatter-related Ångström exponent of 0.1, wavelength-independent extinction-to-backscatter ratios (lidar ratios) of around 45 sr, and particle linear depolarization ratio of 20% were found for aged dust (transport time >10 days). In contrast, dust with a shorter atmospheric residence time of 2–3 days showed Ångström exponents of −0.5 (backscatter coefficient) and 0.1 (extinction coefficient), mean lidar ratios of 64 and 50 sr, and particle linear depolarization ratios of 22 and 26% at 355 and 532 nm wavelength, respectively. Traces of fire smoke were also detected in the observed dust layers. The lidar observations were complemented by Aerosol Robotic Network handheld Sun photometer measurements, which revealed a mean total atmospheric column aerosol optical thickness of 0.05 for pure marine conditions (in the absence of lofted aerosol layers) and roughly 0.9 during a strong Saharan dust outbreak. The achieved data set was compared with first Consortium for Small Scale Modeling-Multi-Scale Chemistry Aerosol Transport simulations. The simulated vertical aerosol distribution showed good agreement with the lidar observations.
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    EARLINET observations of the 14-22-May long-range dust transport event during SAMUM 2006: Validation of results from dust transport modelling
    (Milton Park : Taylor & Francis, 2017) Müller, D.; Heinold, B.; Tesche, M.; Tegen, I.; Althausen, D.; Alados Arboledas, L.; Amiridis, V.; Amodeo, A.; Ansmann, A.; Balis, D.; Comeron, A.; D’mico, G.; Gerasopoulos, E.; Guerrero-Rascado, J.L.; Freudenthaler, V.; Giannakaki, E.; Heese, B.; Iarlori, M.; Knippertz, P.; Mamouri, R.E.; Mona, L.; Papayannis, A.; Pappalardo, G.; Perrone, R-M.; Pisani, G.; Rizi, V.; Sicard, M.; Spinelli, N.; Tafuro, A.; Wiegner, M.
    We observed a long-range transport event of mineral dust from North Africa to South Europe during the Saharan Mineral Dust Experiment (SAMUM) 2006. Geometrical and optical properties of that dust plume were determined with Sun photometer of the Aerosol Robotic Network (AERONET) and Raman lidar near the North African source region, and with Sun photometers of AERONET and lidars of the European Aerosol Research Lidar Network (EARLINET) in the far field in Europe. Extinction-to-backscatter ratios of the dust plume over Morocco and Southern Europe do not differ. Ångstr¨om exponents increase with distance from Morocco. We simulated the transport, and geometrical and optical properties of the dust plume with a dust transport model. The model results and the experimental data show similar times regarding the appearance of the dust plume over each EARLINET site. Dust optical depth from the model agrees in most cases to particle optical depth measured with the Sun photometers. The vertical distribution of the mineral dust could be satisfactorily reproduced, if we use as benchmark the extinction profiles measured with lidar. In some cases we find differences. We assume that insufficient vertical resolution of the dust plume in the model calculations is one reason for these deviations.