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- ItemMineral dust in Central Asia: Combining lidar and other measurements during the Central Asian dust experiment (CADEX)(Les Ulis : EDP Sciences, 2018) Althausen, Dietrich; Hofer, Julian; Abdullaev, Sabur; Makhmudov, Abduvosit; Baars, Holger; Engelmann, Ronny; Wadinga Fomba, Khanneh; Müller, Konrad; Schettler, Georg; Klüser, Lars; Kandler, Konrad; Nicolae, D.; Makoto, A.; Vassilis, A.; Balis, D.; Behrendt, A.; Comeron, A.; Gibert, F.; Landulfo, E.; McCormick, M.P.; Senff, C.; Veselovskii, I.; Wandinger, U.Mineral dust needs to be characterized comprehensively since it contributes to the climate change in Tajikistan / Central Asia. Lidar results from the measurements of mineral dust during CADEX are compared with results of sun photometer measurements, satellite-based measurements, and chemical analysis of ground samples. Although the dust is often advected from far-range sources, it impacts on the local conditions considerably.
- ItemCalibration of Raman lidar water vapor profiles by means of AERONET photometer observations and GDAS meteorological data(München : European Geopyhsical Union, 2018) Dai, Guangyao; Althausen, Dietrich; Hofer, Julian; Engelmann, Ronny; Seifert, Patric; Bühl, Johannes; Mamouri, Rodanthi-Elisavet; Wu, Songhua; Ansmann, AlbertWe present a practical method to continuously calibrate Raman lidar observations of water vapor mixing ratio profiles. The water vapor profile measured with the multiwavelength polarization Raman lidar PollyXT is calibrated by means of co-located AErosol RObotic NETwork (AERONET) sun photometer observations and Global Data Assimilation System (GDAS) temperature and pressure profiles. This method is applied to lidar observations conducted during the Cyprus Cloud Aerosol and Rain Experiment (CyCARE) in Limassol, Cyprus. We use the GDAS temperature and pressure profiles to retrieve the water vapor density. In the next step, the precipitable water vapor from the lidar observations is used for the calibration of the lidar measurements with the sun photometer measurements. The retrieved calibrated water vapor mixing ratio from the lidar measurements has a relative uncertainty of 11 % in which the error is mainly caused by the error of the sun photometer measurements. During CyCARE, nine measurement cases with cloud-free and stable meteorological conditions are selected to calculate the precipitable water vapor from the lidar and the sun photometer observations. The ratio of these two precipitable water vapor values yields the water vapor calibration constant. The calibration constant for the PollyXT Raman lidar is 6.56 g kg−1 ± 0.72 g kg−1 (with a statistical uncertainty of 0.08 g kg−1 and an instrumental uncertainty of 0.72 g kg−1). To check the quality of the water vapor calibration, the water vapor mixing ratio profiles from the simultaneous nighttime observations with Raman lidar and Vaisala radiosonde sounding are compared. The correlation of the water vapor mixing ratios from these two instruments is determined by using all of the 19 simultaneous nighttime measurements during CyCARE. Excellent agreement with the slope of 1.01 and the R2 of 0.99 is found. One example is presented to demonstrate the full potential of a well-calibrated Raman lidar. The relative humidity profiles from lidar, GDAS (simulation) and radiosonde are compared, too. It is found that the combination of water vapor mixing ratio and GDAS temperature profiles allow us to derive relative humidity profiles with the relative uncertainty of 10–20 %.
- ItemEARLINET evaluation of the CATS Level 2 aerosol backscatter coefficient product(Katlenburg-Lindau : EGU, 2019) Proestakis, Emmanouil; Amiridis, Vassilis; Marinou, Eleni; Binietoglou, Ioannis; Ansmann, Albert; Wandinger, Ulla; Hofer, Julian; Yorks, John; Nowottnick, Edward; Makhmudov, Abduvosit; Papayannis, Alexandros; Pietruczuk, Aleksander; Gialitaki, Anna; Apituley, Arnoud; Szkop, Artur; Muñoz Porcar, Constantino; Bortoli, Daniele; Dionisi, Davide; Althausen, Dietrich; Mamali, Dimitra; Balis, Dimitris; Nicolae, Doina; Tetoni, Eleni; Liberti, Gian Luigi; Baars, Holger; Mattis, Ina; Stachlewska, Iwona Sylwia; Voudouri, Kalliopi Artemis; Mona, Lucia; Mylonaki, Maria; Perrone, Maria Rita; Costa, Maria João; Sicard, Michael; Papagiannopoulos, Nikolaos; Siomos, Nikolaos; Burlizzi, Pasquale; Pauly, Rebecca; Engelmann, Ronny; Abdullaev, Sabur; Pappalardo, GelsominaWe present the evaluation activity of the European Aerosol Research Lidar Network (EARLINET) for the quantitative assessment of the Level 2 aerosol backscatter coefficient product derived by the Cloud-Aerosol Transport System (CATS) aboard the International Space Station (ISS; Rodier et al., 2015). The study employs correlative CATS and EARLINET backscatter measurements within a 50km distance between the ground station and the ISS overpass and as close in time as possible, typically with the starting time or stopping time of the EARLINET performed measurement time window within 90min of the ISS overpass, for the period from February 2015 to September 2016. The results demonstrate the good agreement of the CATS Level 2 backscatter coefficient and EARLINET. Three ISS overpasses close to the EARLINET stations of Leipzig, Germany; Évora, Portugal; and Dushanbe, Tajikistan, are analyzed here to demonstrate the performance of the CATS lidar system under different conditions. The results show that under cloud-free, relative homogeneous aerosol conditions, CATS is in good agreement with EARLINET, independent of daytime and nighttime conditions. CATS low negative biases are observed, partially attributed to the deficiency of lidar systems to detect tenuous aerosol layers of backscatter signal below the minimum detection thresholds; these are biases which may lead to systematic deviations and slight underestimations of the total aerosol optical depth (AOD) in climate studies. In addition, CATS misclassification of aerosol layers as clouds, and vice versa, in cases of coexistent and/or adjacent aerosol and cloud features, occasionally leads to non-representative, unrealistic, and cloud-contaminated aerosol profiles. Regarding solar illumination conditions, low negative biases in CATS backscatter coefficient profiles, of the order of 6.1%, indicate the good nighttime performance of CATS. During daytime, a reduced signal-to-noise ratio by solar background illumination prevents retrievals of weakly scattering atmospheric layers that would otherwise be detectable during nighttime, leading to higher negative biases, of the order of 22.3%. © Author(s) 2019.
- ItemIce-nucleating particle versus ice crystal number concentrationin altocumulus and cirrus layers embedded in Saharan dust: a closure study(Katlenburg-Lindau : EGU, 2019) Ansmann, Albert; Mamouri, Rodanthi-Elisavet; Bühl, Johannes; Seifert, Patric; Engelmann, Ronny; Hofer, Julian; Nisantzi, Argyro; Atkinson, James D.; Kanji, Zamin A.; Sierau, Berko; Vrekoussis, Mihalis; Sciare, JeanFor the first time, a closure study of the relationship between the ice-nucleating particle concentration (INP; INPC) and ice crystal number concentration (ICNC) in altocumulus and cirrus layers, solely based on groundbased active remote sensing, is presented. Such aerosol- cloud closure experiments are required (a) to better understand aerosol-cloud interaction in the case of mixed-phase clouds, (b) to explore to what extent heterogeneous ice nucleation can contribute to cirrus formation, which is usually controlled by homogeneous freezing, and (c) to check the usefulness of available INPC parameterization schemes, applied to lidar profiles of aerosol optical and microphysical properties up to the tropopause level. The INPC-ICNC closure studies were conducted in Cyprus (Limassol and Nicosia) during a 6-week field campaign in March-April 2015 and during the 17-month CyCARE (Cyprus Clouds Aerosol and Rain Experiment) campaign. The focus was on altocumulus and cirrus layers which developed in pronounced Saharan dust layers at heights from 5 to 11 km. As a highlight, a long-lasting cirrus event was studied which was linked to the development of a very strong dust-infused baroclinic storm (DIBS) over Algeria. The DIBS was associated with strong convective cloud development and lifted large amounts of Saharan dust into the upper troposphere, where the dust influenced the evolution of an unusually large anvil cirrus shield and the subsequent transformation into an cirrus uncinus cloud system extending from the eastern Mediterranean to central Asia, and thus over more than 3500 km. Cloud top temperatures of the three discussed closure study cases ranged from - 20 to -57 °C. The INPC was estimated from polarization/Raman lidar observations in combination with published INPC parameterization schemes, whereas the ICNC was retrieved from combined Doppler lidar, aerosol lidar, and cloud radar observations of the terminal velocity of falling ice crystals, radar reflectivity, and lidar backscatter in combination with the modeling of backscattering at the 532 and 8.5 mm wavelengths. A good-to-acceptable agreement between INPC (observed before and after the occurrence of the cloud layer under investigation) and ICNC values was found in the discussed three proof-of-concept closure experiments. In these case studies, INPC and ICNC values matched within an order of magnitude (i.e., within the uncertainty ranges of the INPC and ICNC estimates), and they ranged from 0.1 to 10 L-1 in the altocumulus layers and 1 to 50 L-1 in the cirrus layers observed between 8 and 11 km height. The successful closure experiments corroborate the important role of heterogeneous ice nucleation in atmospheric ice formation processes when mineral dust is present. The observed longlasting cirrus event could be fully explained by the presence of dust, i.e., without the need for homogeneous ice nucleation processes. © 2019 Author(s).
- ItemMineral dust in central Asia: 18-month lidar measurements in Tajikistan during the central Asian dust experiment (CADEX)(Les Ulis : EDP Sciences, 2018) Hofer, Julian; Althausen, Dietrich; Abdullaev, Sabur F.; Makhmudov, Abduvosit; Nazarov, Bakhron I.; Schettler, Georg; Fomba, K.Wadinga; Müller, Konrad; Heinold, Bernd; Baars, Holger; Engelmann, Ronny; Ansmann, Albert; Nicolae, D.; Makoto, A.; Vassilis, A.; Balis, D.; Behrendt, A.; Comeron, A.; Gibert, F.; Landulfo, E.; McCormick, M.P.; Senff, C.; Veselovskii, I.; Wandinger, U.Tajikistan is often affected by atmospheric mineral dust. The direct and indirect radiative effects of dust play a sensitive role in the climate system in Central Asia. The Central Asian Dust Experiment (CADEX) provides first lidar measurements in Tajikistan. The autonomous multiwavelength polarization Raman lidar PollyXT was operated for 1.5 years (2015/16) in Dushanbe. In spring, lofted layers of long-range transported dust and in summer/ autumn, lower laying dust from local or regional sources with large optical thicknesses occurred.
- ItemCADEX and beyond: Installation of a new PollyXT site in Dushanbe(Les Ulis : EDP Sciences, 2019) Engelmann, Ronny; Hofer, Julian; Makhmudov, Abduvosit N.; Baars, Holger; Hanbuch, Karsten; Ansmann, Albert; Abdullaev, Sabur F.; Macke, Andreas; Althausen, DietrichDuring the 18-month Central Asian Dust Experiment we conducted continuous lidar measurements at the Physical Technical Institute of the Academy of Sciences of Tajikistan in Dushanbe between 2015 and 2016. Mineral dust plumes from various source regions have been observed and characterized in terms of their occurrence, and their optical and microphysical properties with the Raman lidar PollyXT. Currently a new container-based lidar system is constructed which will be installed for continuous long-term measurements in Dushanbe. © 2019 The Authors, published by EDP Sciences.
- ItemLidar/radar approach to quantify the dust impact on ice nucleation in mid and high level clouds(Les Ulis : EDP Sciences, 2019) Ansmann, Albert; Mamouri, Rodanthi-Elisavet; Bühl, Johannes; Seifert, Patric; Engelmann, Ronny; Nisantzi, Agyro; Hofer, Julian; Baars, HolgerWe present the first attempt of a closure experiment regarding the relationship between ice nucleating particle concentration (INPC) and ice crystal number concentration (ICNC), solely based on active remote sensing. The approach combines aerosol and cloud observations with polarization lidar, Doppler lidar, and cloud radar. Several field campaigns were conducted on the island of Cyprus in the Eastern Mediterranean from 2015-2018 to study heterogeneous ice formation in altocumulus and cirrus layers embedded in Saharan dust. A case study observed on 10 April 2017 is discussed in this contribution. © 2019 The Authors, published by EDP Sciences.
- ItemVariations of the aerosol chemical composition during Asian dust storm at Dushanbe, Tajikistan(Les Ulis : EDP Sciences, 2019) Fomba, Khanneh Wadinga; Müller, Konrad; Hofer, Julian; Makhmudov, Abduvosit N.; Althausen, Dietrich; Nazarov, Bahron I.; Abdullaev, Sabur F.; Herrmann, HartmutAerosol chemical composition was characterized during the Central Asian Dust Experiment (CADEX) at Dushanbe (Tajikistan). Aerosol samples were collected during a period of 2 months from March to May 2015 using a high volume DIGITEL DHA-80 sampler on quartz fiber filters. The filters were analyzed for their ionic, trace metals as well as organic and elemental carbon (OC/EC) content. The aerosol mass showed strong variation with mass concentration ranging from 18 μg/m3 to 110 μg/m3. The mineral dust concentrations varied between 0.9 μg/m3 and 88 μg/m3. Days of high aerosol mass loadings were dominated by mineral dust, which made up to about 80% of the aerosol mass while organic matter and inorganic ions made up about 70% of the aerosol mass during days of low aerosol mass loadings. The mineral dust composition showed different trace metal signatures in comparison to Saharan dust with higher Ca content and Ca/Fe ratios twice as high as that observed in Saharan dust. Strong influence of anthropogenic activities was observed in the trace metal concentrations with Zn and Pb concentrations ranging from 7 to 197 ng/m3 and 2 to 20 ng/m3, respectively. Mineral dust and anthropogenic activities relating to traffic, combustion as well as metallurgical industrial emissions are identified as the sources of the aerosol during this period. © 2019 The Authors, published by EDP Sciences.
- ItemAerosol layer heights above Tajikistan during the CADEX campaign(Les Ulis : EDP Sciences, 2019) Hofer, Julian; Althausen, Dietrich; Abdullaev, Sabur F.; Nazarov, Bakhron I.; Makhmudov, Abduvosit N.; Baars, Holger; Engelmann, Ronny; Ansmann, AlbertMineral dust influences climate and weather by direct and indirect effects. Surrounded by dust sources, Central Asian countries are affected by atmospheric mineral dust on a regular basis. Climate change effects like glacier retreat and desertification are prevalent in Central Asia as well. Therefore, the role of dust in the climate system in Central Asia needs to be clarified and quantified. During the Central Asian Dust EXperiment (CADEX) first lidar observations in Tajikistan were conducted. Long-term vertically resolved aerosol measurements were performed with the multiwavelength polarization Raman lidar PollyXT from March 2015 to August 2016 in Dushanbe, Tajikistan. In this contribution, a climatology of the aerosol layer heights is presented, which was retrieved from the 18-month lidar measurements. Automatic detection based on backscatter coefficient thresholds were used to retrieve the aerosol layer heights and yield similar layer heights as manual layer height determination. The significant aerosol layer height has a maximum in summer and a minimum in winter. The highest layers occurred in spring, but in summer uppermost layer heights above 6 km AGL are frequent, too. © 2019 The Authors, published by EDP Sciences.
- ItemVertical profiles of dust and other aerosol types above a coastal site(Les Ulis : EDP Sciences, 2019) Althausen, Dietrich; Mewes, Silke; Heese, Birgit; Hofer, Julian; Schechner, Yoav; Aides, Amit; Holodovsky, VadimMonthly mean vertical profiles of aerosol type occurrences are determined from multiwavelength Raman and polarization lidar measurements above Haifa, Israel, in 2017. This contribution presents the applied methods and threshold values. The results are discussed for one example, May 2017. This month shows more often large, non-spherical particles in lofted layers than within the planetary boundary layer. Small particles are observed at higher altitudes only when they are observed in lower altitudes, too. © 2019 The Authors, published by EDP Sciences.