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Structural properties of Co2TiSi films on GaAs(001)

2016, Jenichen, B., Herfort, J., Hanke, M., Jahn, U., Kong, X., Dau, M.T., Trampert, A., Kirmse, H., Erwin, S.C.

Co2TiSi films were grown by molecular beam epitaxy on GaAs(001) and analyzed using reflection high-energy electron diffraction, and electron microscopy. In addition, X-ray diffraction was combined with lattice parameter calculations by density functional theory comparing the L21 and B2 structures and considering the influence of non-stoichiometry. Columnar growth is found and attributed to inhomogeneous epitaxial strain from non-random alloying. In films with thicknesses up to 13 nm, these columns may be the origin of perpendicular magnetization with the easy axis perpendicular to the sample surface. We found L21 and B2 ordered regions, however the [Co]/[Ti]-ratio is changing in dependence of the position in the film. The resulting columnar structure is leading to anisotropic B2-ordering with the best order parallel to the axes of the columns.

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BMBF-Förderschwerpunkt: Quantenstruktursysteme auf der Basis von III-V-Halbleitern, Teilvorhaben: Quantendrähte und Quantenpunkte durch Überwachsen von lateral strukturierten nicht-[100]-orientierten Substraten und Schichtsystemen ; Schlußbericht

2000, Nötzel, R., Fricke, J., Jahn, U., Niu, Z.C., Ramsteiner, M., Schönherr, H.P., Trampert, A.

[no abstract available]

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Growth of Fe3Si/Ge/Fe3Si trilayers on GaAs(001) using solid-phase epitaxy

2017, Gaucher, S., Jenichen, B., Kalt, J., Jahn, U., Trampert, A., Herfort, J.

Ferromagnetic Heusler alloys can be used in combination with semiconductors to create spintronic devices. The materials have cubic crystal structures, making it possible to grow lattice-matched heterojunctions by molecular beam epitaxy. However, the development of devices is limited by the difficulty of growing epitaxial semiconductors over metallic surfaces while preventing chemical reactions, a requirement to obtain abrupt interfaces and achieve efficient spin-injection by tunneling. We used a solid-phase epitaxy approach to grow crystalline thin film stacks on GaAs(001) substrates, while preventing interfacial reactions. The crystallized Ge layer forms superlattice regions, which are caused by the migration of Fe and Si atoms into the film. X-ray diffraction and transmission electron microscopy indicate that the trilayers are fully crystalline, lattice-matched, and have ideal interface quality over extended areas.

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Molecular beam epitaxy of graphene on ultra-smooth nickel: growth mode and substrate interactions

2014, Wofford, J.M., Oliveira Jr, M.H., Schumann, T., Jenichen, B., Ramsteiner, M., Jahn, U., Fölsch, S., Lopes, J.M.J., Riechert, H.

Graphene is grown by molecular beam epitaxy using epitaxial Ni films on MgO(111) as substrates. Raman spectroscopy and scanning tunneling microscopy reveal the graphene films to have few crystalline defects. While the layers are ultra-smooth over large areas, we find that Ni surface features lead to local non-uniformly thick graphene inclusions. The influence of the Ni surface structure on the position and morphology of these inclusions strongly suggests that multilayer graphene on Ni forms at the interface of the first complete layer and metal substrate in a growth-from-below mechanism. The interplay between Ni surface features and graphene growth behavior may facilitate the production of films with spatially resolved multilayer inclusions through engineered substrate surface morphology.