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- ItemSurface matters: Limitations of CALIPSO V3 aerosol typing in coastal regions(München : European Geopyhsical Union, 2014) Kanitz, T.; Ansmann, A.; Foth, A.; Seifert, P.; Wandinger, U.; Engelmann, R.; Baars, H.; Althausen, D.; Casiccia, C.; Zamorano, F.In the CALIPSO data analysis, surface type (land/ocean) is used to augment the aerosol characterization. However, this surface-dependent aerosol typing prohibits a correct classification of marine aerosol over land that is advected from ocean to land. This might result in a systematic overestimation of the particle extinction coefficient and of the aerosol optical thickness (AOT) of up to a factor of 3.5 over land in coastal areas. We present a long-term comparison of CALIPSO and ground-based lidar observations of the aerosol conditions in the coastal environment of southern South America (Punta Arenas, Chile, 53° S), performed in December 2009–April 2010. Punta Arenas is almost entirely influenced by marine particles throughout the year, indicated by a rather low AOT of 0.02–0.04. However, we found an unexpectedly high fraction of continental aerosol in the aerosol types inferred by means of CALIOP observations and, correspondingly, too high values of particle extinction. Similar features of the CALIOP data analysis are presented for four other coastal areas around the world. Since CALIOP data serve as important input for global climate models, the influence of this systematic error was estimated by means of simplified radiative-transfer calculations.
- ItemRadiative effect of aerosols above the northern and southern Atlantic Ocean as determined from shipborne lidar observations(Hoboken, NJ : Wiley, 2013) Kanitz, T.; Ansmann, Albert; Seifert, P.; Engelmann, R.; Althausen, D.The direct solar radiative effect of aerosols over the Atlantic Ocean was investigated on the basis of aerosol Raman/polarization lidar observations aboard the research vessel Polarsternbetween Germany (50°N) and either South America (50°S) or South Africa (40°S) in 2009 and 2010. First, a case study of complex aerosol conditions with marine aerosol, dust, and smoke particles in the boundary layer and free troposphere is presented to demonstrate that detailed knowledge of aerosol layering (boundary layer, free troposphere) and aerosol mixing state is required for an accurate determination of the resulting radiative effects. A statistical analysis based on all lidar observations revealed the highest daily mean radiative effect (−43±59 W m−2at the surface, −14±18 W m−2at top of atmosphere) in the latitudinal belt from 0°N–15°N in the Saharan dust outflow region. Mean aerosol radiative effects of the polluted northern and clean southern midlatitudes were contrasted. In the northern midlatitudes, the averaged aerosol radiative effect of all simulations was −24±33 W m−2at the surface which is a factor of 1.6 higher than at similar southern hemispheric latitudes. The simulations based on the lidar observations are in good agreement with colocated pyranometer measurements.
- ItemTracking the Saharan Air Layer with shipborne lidar across the tropical Atlantic(Hoboken, NJ : Wiley, 2014) Kanitz, T.; Engelmann, R.; Heinold, B.; Baars, H.; Skupin, A.; Ansmann, A.Saharan dust was observed with shipborne lidar from 60° to 20°W along 14.5°N during a 1-month transatlantic cruise of the research vessel Meteor. About 4500 km off the coast of Africa, mean extinction and backscatter-related Ångström exponent of 0.1, wavelength-independent extinction-to-backscatter ratios (lidar ratios) of around 45 sr, and particle linear depolarization ratio of 20% were found for aged dust (transport time >10 days). In contrast, dust with a shorter atmospheric residence time of 2–3 days showed Ångström exponents of −0.5 (backscatter coefficient) and 0.1 (extinction coefficient), mean lidar ratios of 64 and 50 sr, and particle linear depolarization ratios of 22 and 26% at 355 and 532 nm wavelength, respectively. Traces of fire smoke were also detected in the observed dust layers. The lidar observations were complemented by Aerosol Robotic Network handheld Sun photometer measurements, which revealed a mean total atmospheric column aerosol optical thickness of 0.05 for pure marine conditions (in the absence of lofted aerosol layers) and roughly 0.9 during a strong Saharan dust outbreak. The achieved data set was compared with first Consortium for Small Scale Modeling-Multi-Scale Chemistry Aerosol Transport simulations. The simulated vertical aerosol distribution showed good agreement with the lidar observations.