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- ItemStability and excitation dynamics of an argon micro-scaled atmospheric pressure plasma jet(Bristol : IOP Publ., 2015) Dünnbier, M.; Becker, M.M.; Iseni, S.; Bansemer, R.; Loffhagen, D.; Reuter, S.; Weltmann, K.-D.A megahertz-driven plasma jet at atmospheric pressure—the so-called micro-scaled atmospheric pressure plasma jet (μAPPJ)—operating in pure argon has been investigated experimentally and by numerical modelling. To ignite the discharge in argon within the jet geometry, a self-made plasma tuning unit was designed, which additionally enables measurements of the dissipated power in the plasma itself. Discharges in the α-mode up to their transition to the γ-mode were studied experimentally for varying frequencies. It was found that the voltage at the α–γ transition behaves inversely proportional to the applied frequency f and that the corresponding power scales with an f 3/2law. Both these findings agree well with the results of time-dependent, spatially one-dimensional fluid modelling of the discharge behaviour, where the f 3/2 scaling of the α–γ transition power is additionally verified by the established concept of a critical plasma density for sheath breakdown. Furthermore, phase resolved spectroscopy of the optical emission at 750.39 nm as well as at 810.37 nm and 811.53 nm was applied to analyse the excitation dynamics of the discharge at 27 MHz for different applied powers. The increase of the power leads to an additional maximum in the excitation structure of the 750.39 nm line emission at the α–γ transition point, whereas the emission structure around 811 nm does not change qualitatively. According to the fluid modelling results, this differing behaviour originates from the different population mechanisms of the corresponding energy levels of argon.
- ItemAdvanced fluid modeling and PIC/MCC simulations of low-pressure ccrf discharges(Bristol : IOP Publ., 2017-3-2) Becker, M.M.; Kählert, H.; Sun, A.; Bonitz, M.; Loffhagen, D.Comparative studies of capacitively coupled radio-frequency discharges in helium and argon at pressures between 10 and 80 Pa are presented applying two different fluid modeling approaches as well as two independently developed particle-in-cell/Monte Carlo collision (PIC/MCC) codes. The focus is on the analysis of the range of applicability of a recently proposed fluid model including an improved drift-diffusion approximation for the electron component as well as its comparison with fluid modeling results using the classical drift-diffusion approximation and benchmark results obtained by PIC/MCC simulations. Main features of this time- and space-dependent fluid model are given. It is found that the novel approach shows generally quite good agreement with the macroscopic properties derived by the kinetic simulations and is largely able to characterize qualitatively and quantitatively the discharge behavior even at conditions when the classical fluid modeling approach fails. Furthermore, the excellent agreement between the two PIC/MCC simulation codes using the velocity Verlet method for the integration of the equations of motion verifies their accuracy and applicability.
- ItemExtended reaction kinetics model for non-thermal argon plasmas and its test against experimental data(Bristol : IOP Publ., 2022) Stankov, M.; Becker, M.M.; Hoder, T.; Loffhagen, D.An extended reaction kinetics model (RKM) suitable for the analysis of weakly ionised, non-thermal argon plasmas with gas temperatures around 300 K at sub-atmospheric and atmospheric pressures is presented. It considers 23 different species including electrons as well as the ground state atom, an atomic and molecular ion, four excited molecular states, and 15 excited atomic states of argon, where all individual 1s and 2p states (in Paschen notation) are included as a separate species. This 23-species RKM involves 409 collision processes and radiative transitions and recent electron collision cross section data. It is evaluated by means of results of time- and space-dependent fluid modelling of argon discharges and their comparison with measured data for two different dielectric barrier discharge configurations as well as a micro-scaled atmospheric-pressure plasma jet setup. The results are also compared with those obtained by use of a previously established 15-species RKM involving only the two lumped 2p states 2p10…5 and 2´p4 … 1. It is found that the 23-species RKM shows generally better agreement with experimental data and provides more options for direct comparison with measurements than the frequently used 15-species RKM.
- ItemInfluence of surface parameters on dielectric-barrier discharges in argon at subatmospheric pressure(Bristol : IOP Publ., 2020) Stankov, M.; Becker, M.M.; Bansemer, R.; Weltmann, K.-D.; Loffhagen, D.The influence of the secondary electron emission coefficient, γ, and the relative permittivity, ɛr, of the dielectric layers on the characteristics of dielectric-barrier discharges (DBDs) is studied by means of numerical modelling and calculated results are compared with experimental data. The analysis has been performed for a geometrically symmetric, plane-parallel DBD in argon with copper electrodes covered by quartz dielectrics. A time-dependent, spatially one-dimensional fluid model involving the drift-diffusion approximation is applied for the numerical analysis of the DBD operating sinusoidally at a frequency of 24 kHz with applied voltages between 1.8 and 3.4 kV and pressures from 100 to 650 mbar. Main features of the model as well as the experimental setup and procedures are given. The modelling studies show especially the sensitivity of the results on the specific choice of γ and ɛr regarding the occurrence and intensity of discharge peaks, the appearance of one or more smaller peaks after the main peak, as well the establishment of a single periodic, multiperiodic or even chaotic temporal evolution of the DBD. In particular, generally good agreement between measured and calculated discharge current signals and the power dissipated in the discharge is found for γ = 0.02 and ɛr = 4.2.