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- ItemSelf-cleaning stainless steel surfaces induced by laser processing and chemical engineering(Amsterdam [u.a.] : Elsevier, 2022) Lorenz, Pierre; Zajadacz, Joachim; Marquardt, Franka; Ehrhardt, Martin; Hommes, Gregor; Peter, Sebastian; Zimmer, KlausNanostructured surfaces show a variety of beneficial macroscopic effects. The combination of hierarchic nanostructures with a suitable chemical surface composition allows for the fabrication of surfaces with interesting fluidic properties beyond such effects. This approach enables the specification of nano/microstructure and chemical composition independent of each other. Various hierarchical micro- and nanostructures can be realized by laser texturing of stainless steel surfaces with infrared picosecond laser. Simultaneously, the surface is activated for chemical processing. The surface can now be tuned by bonding of a self-assembled monolayer on the laser-treated surface by chemical treatment. This two-step functionalization process allows the for separated adjusting of the surface topography and chemical composition and thus for the well-defined setting of the surface properties. The fabrication of superhydrophobic surfaces with self-cleaning properties are performed that can be functionalized further by subsequent laser-irradiation. Furthermore, the long-time stability of the surface functionalization in relation to the impact chemicals or radiation was investigated.
- ItemFrom statistic to deterministic nanostructures in fused silica induced by nanosecond laser radiation(Amsterdam [u.a.] : Elsevier, 2018) Lorenz, Pierre; Klöppel, Michael; Zagoranskiy, Igor; Zimmer, KlausThe production of structures by laser machining below the diffraction limit is still a challenge. However, self-organization processes can be useful. The laser-induced self-organized modification of the shape of photolithographic produced chromium structures on fused silica as well as the structuring of the fused silica surface by nanosecond UV laser radiation was studied, respectively. Low fluence single pulse laser irradiation (□ > 300 mJ/cm2) cause the formation from chromium squares to droplets due to the mass transport in the molten chromium film. This process is governed by the instability of the molten metal due to the surface tension driven liquid phase mass transport. For a chromium pattern size similar to the instability length two specific droplet distributions were found which are single droplets with a determined position near the centre of the original pattern or random distributed smaller droplets arranged circularly. Each of the metal patterns can be transferred into the fused silica by a multi-pulse irradiation. The experimental results can be simulated well for low fluences by sequential solving the heat and Navier-Stokes equation.
- ItemSecondary electron yield engineering of copper surfaces by 532 nm ultrashort laser pulses(Amsterdam [u.a.] : Elsevier, 2022) Lorenz, Pierre; Bez, Elena; Himmerlich, Marcel; Ehrhardt, Martin; Taborelli, Mauro; Zimmer, KlausNanostructured surfaces exhibit outstanding properties and enable manifold industrial applications. In this study the laser surface processing of polycrystalline, flat copper surfaces by 532 nm picosecond laser irradiation for secondary electron yield (SEY) reduction is reported. The laser beam was scanned in parallel lines across the sample surface in order to modify large surface areas. Morphology and SEY are characterized in dependence of the process parameters to derive correlations and mechanisms of the laser-based SEY engineering process. The nano- and microstructure morphology of the laser-modified surface was characterized by scanning electron microscopy and the secondary electron yield was measured. In general, an SEY reduction with increasing accumulated laser fluence was found. In particular, at low scanning speed (1 mm/s - 10 mm/s) and “high” laser power (~ 1 W) compact nanostructures with a very low SEY maximum of 0.7 are formed.