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    Ship-borne aerosol profiling with lidar over the Atlantic Ocean: From pure marine conditions to complex dust-smoke mixtures
    (Göttingen : Copernicus GmbH, 2018) Bohlmann, S.; Baars, H.; Radenz, M.; Engelmann, R.; Macke, A.
    The multi-wavelength Raman lidar PollyXT has been regularly operated aboard the research vessel Polarstern on expeditions across the Atlantic Ocean from north to south and vice versa. The lidar measurements of the RV Polarstern cruises PS95 from Bremerhaven, Germany, to Cape Town, Republic of South Africa (November 2015), and PS98 from Punta Arenas, Chile, to Bremerhaven, Germany (April/May 2016), are presented and analysed in detail. The latest set-up of PollyXT allows improved coverage of the marine boundary layer (MBL) due to an additional near-range receiver. Three case studies provide an overview of the aerosol detected over the Atlantic Ocean. In the first case, marine conditions were observed near South Africa on the autumn cruise PS95. Values of optical properties (depolarisation ratios close to zero, lidar ratios of 23 sr at 355 and 532 nm) within the MBL indicate pure marine aerosol. A layer of dried marine aerosol, indicated by an increase of the particle depolarisation ratio to about 10% at 355 nm (9% at 532 nm) and thus confirming the non-sphericity of these particles, could be detected on top of the MBL. On the same cruise, an almost pure Saharan dust plume was observed near the Canary Islands, presented in the second case. The third case deals with several layers of Saharan dust partly mixed with biomass-burning smoke measured on PS98 near the Cabo Verde islands. While the MBL was partly mixed with dust in the pure Saharan dust case, an almost marine MBL was observed in the third case. A statistical analysis showed latitudinal differences in the optical properties within the MBL, caused by the downmixing of dust in the tropics and anthropogenic influences in the northern latitudes, whereas the optical properties of the MBL in the Southern Hemisphere correlate with typical marine values. The particle depolarisation ratio of dried marine layers ranged between 4 and 9% at 532 nm. Night measurements from PS95 and PS98 were used to illustrate the potential of aerosol classification using lidar ratio, particle depolarisation ratio at 355 and 532 nm, and Angström exponent. Lidar ratio and particle depolarisation ratio have been found to be the main indicator for particle type, whereas the Ångström exponent is rather variable.
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    Local and Remote Controls on Arctic Mixed-Layer Evolution
    (Malden MA: Wiley-Blackwell, 2020) Neggers, R.A.J.; Chylik, J.; Egerer, U.; Griesche, H.; Schemann, V.; Seifert, P.; Siebert, H.; Macke, A.
    In this study Lagrangian large-eddy simulation of cloudy mixed layers in evolving warm air masses in the Arctic is constrained by in situ observations from the recent PASCAL field campaign. A key novelty is that time dependence is maintained in the large-scale forcings. An iterative procedure featuring large-eddy simulation on microgrids is explored to calibrate the case setup, inspired by and making use of the typically long memory of Arctic air masses for upstream conditions. The simulated mixed-phase clouds are part of a turbulent mixed layer that is weakly coupled to the surface and is occasionally capped by a shallow humidity layer. All eight simulated mixed layers exhibit a strong time evolution across a range of time scales, including diurnal but also synoptic fingerprints. A few cases experience rapid cloud collapse, coinciding with a rapid decrease in mixed-layer depth. To gain insight, composite budget analyses are performed. In the mixed-layer interior the heat and moisture budgets are dominated by turbulent transport, radiative cooling, and precipitation. However, near the thermal inversion the large-scale vertical advection also contributes significantly, showing a distinct difference between subsidence and upsidence conditions. A bulk mass budget analysis reveals that entrainment deepening behaves almost time-constantly, as long as clouds are present. In contrast, large-scale subsidence fluctuates much more strongly and can both counteract and boost boundary-layer deepening resulting from entrainment. Strong and sudden subsidence events following prolonged deepening periods are found to cause the cloud collapses, associated with a substantial reduction in the surface downward longwave radiative flux. ©2019. The Authors.
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    Radiative effects of the cloudy atmosphere from ground and satellite based observations
    (Les Ulis : EDP Sciences, 2010) Macke, A.; Kalisch, J.; Zoll, Y.; Bumke, K.
    The radiation budget from surface observations and parameterizations is combined with that from satellite observations along the cruise tracks of the German icebreaker POLARSTERN in the North and South Atlantic under tropical, subtropical and mid-latitude conditions. Between 2008 and 2010 The German Leibniz-network OCEANET participated in six transfers from or to Bremerhaven, Germany to or from Punta Arenas, Southern Chile or Cape Town, South Africa. The present chapter introduces exemplarily the atmospheric measurements and resulting radiation products. The following properties are derived: Standard meteorological data, broadband downward solar and thermal irradiances, underwater profiles of spectral irradiance, latent and sensible heat fluxes, humidity and temperature profiles, water vapour and liquid water path, aerosol optical thickness and vertical profiles of aerosol optical thickness, cloud cover and cloud type. Cloud radiative effects at the surface have been determined for different marine cloud types. Together with top-of-atmosphere radiation fluxes from the SEVIRI radiometer onboard METEOSAT, the effect of clouds on atmospheric heating or cooling have been determined. The resulting cloud/radiation correlations will help to quantify the effects of clouds on the surface, ToA- and atmospheric radiation budget and to evaluate the ability of climate models to simulate these effects. © Owned by the authors, published by EDP Sciences, 2010.