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- ItemImpact of spatial inhomogeneities on on-axis pulse reconstruction in femtosecond filaments(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2014) Brée, Carsten; Kretschmar, Martin; Nagy, Tamas; Kurz, Heiko G.; Morgner, Uwe; Kovačev, MilutinWe demonstrate a strong influence of the spatial beam profile on the vacuum-propagated on-axis pulse shapes for a femtosecond filament in argon. The effects can be minimized by transmitting the filament into the far-field by a laser-drilled pinhole setup. Using this method, we can monitor the pulse compression dynamics along the entire longitudinal extension of the filament, including the ionization-induced plasma channel.
- ItemNon-instantaneous polarization dynamics in dielectric media(Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2014) Hofmann, Michael; Hyyti, Janne; Birkholz, Simon; Bock, Martin; Das, Susanta K.; Grunwald, Rüdiger; Hoffmann, Mathias; Nagy, Tamas; Demircan, Ayhan; Jupé, Marco; Ristau, Detlev; Morgner, Uwe; Brée, Carsten; Woerner, Michael; Elsaesser, Thomas; Steinmeyer, GünterThird-order optical nonlinearities play a vital role for generation1,2 and characterization 3-5 of some of the shortest optical pulses to date, for optical switching applications6,7, and for spectroscopy8,9. In many cases, nonlinear optical effects are used far off resonance, and then an instantaneous temporal response is expected. Here, we show for the first time resonant frequency-resolved optical gating measurements1012 that indicate substantial nonlinear polarization relaxation times up to 6.5 fs in dielectric media, i.e., significantly beyond the shortest pulses directly available from commercial lasers. These effects are among the fastest effects observed in ultrafast spectroscopy. Numerical solutions of the time-dependent Schrödinger equation13,14 are in excellent agreement with experimental observations. The simulations indicate that pulse generation and characterization in the ultraviolet may be severely affected by this previously unreported effect. Moreover, our approach opens an avenue for application of frequency-resolved optical gating as a highly selective spectroscopic probe in high-field physics.