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- ItemThermoelectric Characterization Platform for Electrochemically Deposited Materials(Weinheim : Wiley-VCH Verlag GmbH & Co. KG, 2020) Barati, Vida; Garcia Fernandez, Javier; Geishendorf, Kevin; Schnatmann, Lauritz Ule; Lammel, Michaela; Kunzmann, Alexander; Pérez, Nicolás; Li, Guodong; Schierning, Gabi; Nielsch, Kornelius; Reith, HeikoSuccessful optimization of the thermoelectric (TE) performance of materials, described by the figure of merit zT, is a key enabler for its application in energy harvesting or Peltier cooling devices. While the zT value of bulk materials is accessible by a variety of commercial measurement setups, precise determination of the zT value for thin and thick films remains a great challenge. This is particularly relevant for films synthesized by electrochemical deposition, where the TE material is deposited onto an electrically conductive seed layer causing an in-plane short circuit. Therefore, a platform for full in-plane zT characterization of electrochemically deposited TE materials is developed, eliminating the impact of the electrically conducting seed layer. The characterization is done using a suspended TE material within a transport device which was prepared by photolithography in combination with chemical etching steps. An analytical model to determine the thermal conductivity is developed and the results verified using finite element simulations. Taken together, the full in-plane zT characterization provides an inevitable milestone for material optimization under realistic conditions in TE devices. © 2020 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim
- ItemA multifunctional highway system incorporating superconductor levitated vehicles and liquefied hydrogen(Melville, NY : AIP Publishing, 2023) Vakaliuk, O.; Song, Shaowei; Floegel-Delor, U.; Werfel, F.; Nielsch, Kornelius; Ren, ZhifengMagnetic levitation for the transport of people and goods using bulk superconductors and electrical power transmission using superconductors have both been demonstrated, but neither has been developed for daily use due to technological deficiencies and high costs. We envision combining the transport of people and goods and energy transmission and storage in a single system. Such a system, built on existing highway infrastructure, incorporates a superconductor guideway, allowing for simultaneous levitation of vehicles with magnetized undercarriages for rapid transport without schedule limitations and lossless transmission and storage of electricity. Incorporating liquefied hydrogen additionally allows for simultaneous cooling of the superconductor guideway and sustainable energy transport and storage. Here, we report the successful demonstration of the primary technical prerequisite, levitating a magnet above a superconductor guideway.
- ItemSignatures of a Charge Density Wave Phase and the Chiral Anomaly in the Fermionic Material Cobalt Monosilicide CoSi(Weinheim : Wiley-VCH Verlag GmbH & Co. KG, 2020) Schnatmann, Lauritz; Geishendorf, Kevin; Lammel, Michaela; Damm, Christine; Novikov, Sergey; Thomas, Andy; Burkov, Alexander; Reith, Heiko; Nielsch, Kornelius; Schierning, GabiMaterials with topological electronic states have emerged as one of the most exciting discoveries of condensed quantum matter, hosting quasiparticles with extremely low effective mass and high mobility. Weyl materials contain such topological states in the bulk and additionally have a non-trivial chiral charge. However, despite known quantum effects caused by these chiral states, the interplay between chiral states, and a charge density wave phase, an ordering of the electrons to a correlated phase is not experimentally explored. Indications for the formation of a charge density wave phase in the Weyl material cobalt monosilicide CoSi are observed. Furthermore, the typical signatures of the charge density wave phase together with typical signatures of Weyl fermions in magnetic field dependent electrical transport characterization are investigated. The charge density wave and the chiral contribution to the electrical magneto-transport are separated as well as a suppression of the charge density wave phase is observed in magnetic fields. © 2019 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
- ItemDoping High-Mobility Donor : Acceptor Copolymer Semiconductors with an Organic Salt for High-Performance Thermoelectric Materials(Weinheim : Wiley-VCH Verlag GmbH & Co. KG, 2020) Guo, Jing; Li, Guodong; Reith, Heiko; Jiang, Lang; Wang, Ming; Li, Yuhao; Wang, Xinhao; Zeng, Zebing; Zhao, Huaizhou; Lu, Xinhui; Schierning, Gabi; Nielsch, Kornelius; Liao, Lei; Hu, YuanyuanOrganic semiconductors (OSCs) are attractive for fabrication of thermoelectric devices with low cost, large area, low toxicity, and high flexibility. In order to achieve high-performance organic thermoelectric devices (OTEs), it is essential to develop OSCs with high conductivity (σ), large Seebeck coefficient (S), and low thermal conductivity (κ). It is equally important to explore efficient dopants matching the need of thermoelectric devices. The thermoelectric performance of a high-mobility donor–acceptor (D–A) polymer semiconductor, which is doped by an organic salt, is studied. Both a high p-type electrical conductivity approaching 4 S cm−1 and an excellent power factor (PF) of 7 µW K−2 m−1 are obtained, which are among the highest reported values for polymer semiconductors. Temperature-dependent conductivity, Seebeck coefficient and power factor of the doped materials are systematically investigated. Detailed analysis on the results of thermoelectric measurements has revealed a hopping transport in the materials, which verifies the empirical relationship: S ∝ σ−1/4 and PF ∝ σ1/2. The results demonstrate that D–A copolymer semiconductors with proper combination of dopants have great potential for fabricating high-performance thermoelectric devices. © 2020 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim