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Generation and characterization of isolated attosecond pulses for coincidence spectroscopy at 100 kHz repetition rate

2020, Witting, T., Furch, F., Osolodkov, M., Schell, F., Menoni, C., Schulz, C.P., Vrakking, M.J.J.

An attosecond pump-probe beamline with 100 kHz repetition rate for coincidence experiments has been developed. It is based on non-collinear optical parametric chirped pulse ampli-cation and delivers 100 µJ sub-4 fs to an high-harmonic generation source. Details on the generation and characterization of isolated attosecond pulses will be presented. © 2019 Published under licence by IOP Publishing Ltd.

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High power, high repetition rate laser-based sources for attosecond science

2022, Furch, F.J., Witting, T., Osolodkov, M., Schell, F., Schulz, C.P., Vrakking, M.J.

Within the last two decades attosecond science has been established as a novel research field providing insights into the ultrafast electron dynamics that follows a photoexcitation or photoionization process. Enabled by technological advances in ultrafast laser amplifiers, attosecond science has been in turn, a powerful engine driving the development of novel sources of intense ultrafast laser pulses. This article focuses on the development of high repetition rate laser-based sources delivering high energy pulses with a duration of only a few optical cycles, for applications in attosecond science. In particular, a high power, high repetition rate optical parametric chirped pulse amplification system is described, which was developed to drive an attosecond pump-probe beamline targeting photoionization experiments with electron-ion coincidence detection at high acquisition rates.