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Author: Schell, Felix × Type: Text ×

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    Generation and characterisation of few-pulse attosecond pulse trains at 100 kHz repetition rate
    (Bristol : IOP Publ., 2020) Osolodkov, Mikhail; Furch, Federico J.; Schell, Felix; Šušnjar, Peter; Cavalcante, Fabio; Menoni, Carmen S.; Schulz, Claus P.; Witting, Tobias; Vrakking, Marc J.J.
    The development of attosecond pump-probe experiments at high repetition rate requires the development of novel attosecond sources maintaining a sufficient number of photons per pulse. We use 7 fs, 800 nm pulses from a non-collinear optical parametric chirped pulse amplification laser system to generate few-pulse attosecond pulse trains (APTs) with a flux of >106 photons per shot in the extreme ultraviolet at a repetition rate of 100 kHz. The pulse trains have been fully characterised by recording frequency-resolved optical gating for complete reconstruction of attosecond bursts (FROG-CRAB) traces with a velocity map imaging spectrometer. For the pulse retrieval from the FROG-CRAB trace a new ensemble retrieval algorithm has been employed that enables the reconstruction of the shape of the APTs in the presence of carrier envelope phase fluctuations of the few-cycle laser system. © 2020 The Author(s). Published by IOP Publishing Ltd.
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    Strong field ionization of small hydrocarbon chains with full 3D momentum analysis
    (Bristol : IOP Publ., 2015) Schulz, Claus Peter; Birkner, Sascha; Furch, Federico J.; Anderson, Alexandria; Mikosch, Jochen; Schell, Felix; Vrakking, Marc J. J.
    Strong field ionization of small hydrocarbon chains is studied in a kinematic complete experiment using a reaction microscope. By coincidence detection of ions and electrons different ionization continua populated during the ionization process are identified. In addition, photoelectron momentum distributions from laser-aligned molecules allow to characterize the electron wavepackets emerging from different Dyson orbitals.
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    Molecular orbital imprint in laser-driven electron recollision
    (Washington, DC [u.a.] : Assoc., 2018) Schell, Felix; Bredtmann, Timm; Schulz, Claus Peter; Patchkovskii, Serguei; Vrakking, Marc J. J.; Mikosch, Jochen
    Electrons released by strong-field ionization from atoms and molecules or in solids can be accelerated in the oscillating laser field and driven back to their ion core. The ensuing interaction, phase-locked to the optical cycle, initiates the central processes underlying attosecond science. A common assumption assigns a single, welldefined return direction to the recolliding electron. We study laser-induced electron rescattering associated with two different ionization continua in the same, spatially aligned, polyatomic molecule. We show by experiment and theory that the electron return probability is molecular frame-dependent and carries structural information on the ionized orbital. The returning wave packet structure has to be accounted for in analyzing strong-field spectroscopy experiments that critically depend on the interaction of the laser-driven continuum electron, such as laser-induced electron diffraction.