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Retrieval of attosecond pulse ensembles from streaking experiments using mixed state time-domain ptychography

2020, Witting, Tobias, Furch, Federico J., Kornilov, Oleg, Osolodkov, Mikhail, Schulz, Claus P., Vrakking, Marc J.J.

The electric field of attosecond laser pulses can be retrieved from laser-dressed photoionisation measurements, where electron wavepackets that result from single-photon ionisation by the attosecond pulse in the presence of a dressing field are produced. In case of fluctuating dressing laser and/or attosecond pulses, e.g. due to pulse-to-pulse fluctuations of the carrier envelope phase of the infrared laser pulse, commonly applied retrieval algorithms result in the erroneous extraction of the pulse fields. We present a mixed state time-domain ptychography algorithm for the retrieval of pulse ensembles from attosecond streaking experiments. © 2020 The Author(s). Published by IOP Publishing Ltd.

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Generation and characterisation of few-pulse attosecond pulse trains at 100 kHz repetition rate

2020, Osolodkov, Mikhail, Furch, Federico J., Schell, Felix, Šušnjar, Peter, Cavalcante, Fabio, Menoni, Carmen S., Schulz, Claus P., Witting, Tobias, Vrakking, Marc J.J.

The development of attosecond pump-probe experiments at high repetition rate requires the development of novel attosecond sources maintaining a sufficient number of photons per pulse. We use 7 fs, 800 nm pulses from a non-collinear optical parametric chirped pulse amplification laser system to generate few-pulse attosecond pulse trains (APTs) with a flux of >106 photons per shot in the extreme ultraviolet at a repetition rate of 100 kHz. The pulse trains have been fully characterised by recording frequency-resolved optical gating for complete reconstruction of attosecond bursts (FROG-CRAB) traces with a velocity map imaging spectrometer. For the pulse retrieval from the FROG-CRAB trace a new ensemble retrieval algorithm has been employed that enables the reconstruction of the shape of the APTs in the presence of carrier envelope phase fluctuations of the few-cycle laser system. © 2020 The Author(s). Published by IOP Publishing Ltd.