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- ItemCloud radar with hybrid mode towards estimation of shape and orientation of ice crystals(München : European Geopyhsical Union, 2016) Myagkov, A.; Seifert, P.; Bauer-Pfundstein, M.; Wandinger, U.This paper is devoted to the experimental quantitative characterization of the shape and orientation distribution of ice particles in clouds. The characterization is based on measured and modeled elevation dependencies of the polarimetric parameters differential reflectivity and correlation coefficient. The polarimetric data are obtained using a newly developed 35 GHz cloud radar MIRA-35 with hybrid polarimetric configuration and scanning capabilities. The full procedure chain of the technical implementation and the realization of the setup of the hybrid-mode cloud radar for the shape determination are presented. This includes the description of phase adjustments in the transmitting paths, the introduction of the general data processing scheme, correction of the data for the differences of amplifications and electrical path lengths in the transmitting and receiving channels, the rotation of the polarization basis by 45°, the correction of antenna effects on polarimetric measurements, the determination of spectral polarimetric variables, and the formulation of a scheme to increase the signal-to-noise ratio. Modeling of the polarimetric variables is based on existing back-scattering models assuming the spheroidal representation of cloud scatterers. The parameters retrieved from the model are polarizability ratio and degree of orientation, which can be assigned to certain particle orientations and shapes. The developed algorithm is applied to a measurement of the hybrid-mode cloud radar taken on 20 October 2014 in Cabauw, the Netherlands, in the framework of the ACCEPT (Analysis of the Composition of Clouds with Extended Polarization Techniques) campaign. The case study shows the retrieved polarizability ratio and degree of orientation of ice particles for a cloud system of three cloud layers at different heights. Retrieved polarizability ratios are 0.43, 0.85, and 1.5 which correspond to oblate, quasi-spherical, and columnar ice particles, respectively. It is shown that the polarizability ratio is useful for the detection of aggregation/riming processes. The orientation of oblate and prolate particles is estimated to be close to horizontal while quasi-spherical particles were found to be more randomly oriented.
- ItemProfiling of fine and coarse particle mass: Case studies of Saharan dust and Eyjafjallajökull/Grimsvötn volcanic plumes(München : European Geopyhsical Union, 2012) Ansmann, A.; Seifert, P.; Tesche, M.; Wandinger, U.The polarization lidar photometer networking (POLIPHON) method introduced to separate coarse-mode and fine-mode particle properties of Eyjafjallajökull volcanic aerosols in 2010 is extended to cover Saharan dust events as well. Furthermore, new volcanic dust observations performed after the Grimsvötn volcanic eruptions in 2011 are presented. The retrieval of particle mass concentrations requires mass-specific extinction coefficients. Therefore, a review of recently published mass-specific extinction coefficients for Saharan dust and volcanic dust is given. Case studies of four different scenarios corroborate the applicability of the profiling technique: (a) Saharan dust outbreak to central Europe, (b) Saharan dust plume mixed with biomass-burning smoke over Cape Verde, and volcanic aerosol layers originating from (c) the Eyjafjallajökull eruptions in 2010 and (d) the Grimsvötn eruptions in 2011. Strong differences in the vertical aerosol layering, aerosol mixing, and optical properties are observed for the different volcanic events.
- ItemFour-dimensional distribution of the 2010 Eyjafjallajökull volcanic cloud over Europe observed by EARLINET(München : European Geopyhsical Union, 2013) Pappalardo, G.; Mona, L.; D'Amico, G.; Wandinger, U.; Adam, M.; Amodeo, A.; Ansmann, A.; Apituley, A.; Alados Arboledas, L.; Balis, D.; Boselli, A.; Bravo-Aranda, J.A.; Chaikovsky, A.; Comeron, A.; Cuesta, J.; De Tomasi, F.; Freudenthaler, V.; Gausa, M.; Giannakaki, E.; Giehl, H.; Giunta, A.; Grigorov, I.; Groß, S.; Haeffelin, M.; Hiebsch, A.; Iarlori, M.; Lange, D.; Linné, H.; Madonna, F.; Mattis, I.; Mamouri, R.-E.; McAuliffe, M.A.P.; Mitev, V.; Molero, F.; Navas-Guzman, F.; Nicolae, D.; Papayannis, A.; Perrone, M.R.; Pietras, C.; Pietruczuk, A.; Pisani, G.; Preißler, J.; Pujadas, M.; Rizi, V.; Ruth, A.A.; Schmidt, J.; Schnell, F.; Seifert, P.; Serikov, I.; Sicard, M.; Simeonov, V.; Spinelli, N.; Stebel, K.; Tesche, M.; Trickl, T.; Wang, X.; Wagner, F.; Wiegner, M.; Wilson, K.M.The eruption of the Icelandic volcano Eyjafjallajökull in April–May 2010 represents a "natural experiment" to study the impact of volcanic emissions on a continental scale. For the first time, quantitative data about the presence, altitude, and layering of the volcanic cloud, in conjunction with optical information, are available for most parts of Europe derived from the observations by the European Aerosol Research Lidar NETwork (EARLINET). Based on multi-wavelength Raman lidar systems, EARLINET is the only instrument worldwide that is able to provide dense time series of high-quality optical data to be used for aerosol typing and for the retrieval of particle microphysical properties as a function of altitude. In this work we show the four-dimensional (4-D) distribution of the Eyjafjallajökull volcanic cloud in the troposphere over Europe as observed by EARLINET during the entire volcanic event (15 April–26 May 2010). All optical properties directly measured (backscatter, extinction, and particle linear depolarization ratio) are stored in the EARLINET database available at http://www.earlinet.org. A specific relational database providing the volcanic mask over Europe, realized ad hoc for this specific event, has been developed and is available on request at http://www.earlinet.org. During the first days after the eruption, volcanic particles were detected over Central Europe within a wide range of altitudes, from the upper troposphere down to the local planetary boundary layer (PBL). After 19 April 2010, volcanic particles were detected over southern and south-eastern Europe. During the first half of May (5–15 May), material emitted by the Eyjafjallajökull volcano was detected over Spain and Portugal and then over the Mediterranean and the Balkans. The last observations of the event were recorded until 25 May in Central Europe and in the Eastern Mediterranean area. The 4-D distribution of volcanic aerosol layering and optical properties on European scale reported here provides an unprecedented data set for evaluating satellite data and aerosol dispersion models for this kind of volcanic events.
- ItemThe Pagami Creek smoke plume after long-range transport to the upper troposphere over Europe – Aerosol properties and black carbon mixing state(München : European Geopyhsical Union, 2014) Dahlkötter, F.; Gysel, M.; Sauer, D.; Minikin, A.; Baumann, R.; Seifert, P.; Ansmann, A.; Fromm, M.; Voigt, C.; Weinzierl, B.During the CONCERT 2011 field experiment with the DLR research aircraft Falcon, an enhanced aerosol layer with particle linear depolarization ratios of 6–8% at 532 nm was observed at altitudes above 10 km over northeast Germany on 16 September 2011. Dispersion simulations with HYSPILT suggest that the elevated aerosol layer originated from the Pagami Creek forest fire in Minnesota, USA, which caused pyro-convective uplift of particles and gases. The 3–4 day-old smoke plume had high total refractory black carbon (rBC) mass concentrations of 0.03–0.35 μg m−3 at standard temperature and pressure (STP) with rBC mass equivalent diameter predominantly smaller than 130 nm. Assuming a core-shell particle structure, the BC cores exhibit very thick (median: 105–136 nm) BC-free coatings. A large fraction of the BC-containing particles disintegrated into a BC-free fragment and a BC fragment while passing through the laser beam of the Single Particle Soot Photometer (SP2). In this study, the disintegration is a result of very thick coatings around the BC cores. This is in contrast to a previous study in a forest-fire plume, where it was hypothesized to be a result of BC cores being attached to a BC-free particle. For the high-altitude forest-fire aerosol layer observed in this study, increased mass specific light-absorption cross sections of BC can be expected due to the very thick coatings around the BC cores, while this would not be the case for the attached-type morphology. We estimate the BC mass import from the Pagami Creek forest fire into the upper troposphere/lower stratosphere (UTLS) region (best estimate: 25 Mg rBC). A comparison to black carbon emission rates from aviation underlines the importance of pyro-convection on the BC load in the UTLS region. Our study provides detailed information on the microphysics and the mixing state of BC in the forest-fire aerosol layer in the upper troposphere that can be used to better understand and investigate the radiative impact of such upper tropospheric aerosol layers.
- ItemPeakTree: A framework for structure-preserving radar Doppler spectra analysis(Göttingen : Copernicus GmbH, 2019) Radenz, M.; Bühl, J.; Seifert, P.; Griesche, H.; Engelmann, R.Clouds are frequently composed of more than one particle population even at the smallest scales. Cloud radar observations frequently contain information on multiple particle species in the observation volume when there are distinct peaks in the Doppler spectrum. Multi-peaked situations are not taken into account by established algorithms, which only use moments of the Doppler spectrum. In this study, we propose a new algorithm that recursively represents the subpeaks as nodes in a binary tree. Using this tree data structure to represent the peaks of a Doppler spectrum, it is possible to drop all a priori assumptions on the number and arrangement of subpeaks. The approach is rigid, unambiguous and can provide a basis for advanced analysis methods. The applicability is briefly demonstrated in two case studies, in which the tree structure was used to investigate particle populations in Arctic multilayered mixed-phase clouds, which were observed during the research vessel Polarstern expedition PS106 and the Atmospheric Radiation Measurement Program BAECC campaign.
- ItemSurface matters: Limitations of CALIPSO V3 aerosol typing in coastal regions(München : European Geopyhsical Union, 2014) Kanitz, T.; Ansmann, A.; Foth, A.; Seifert, P.; Wandinger, U.; Engelmann, R.; Baars, H.; Althausen, D.; Casiccia, C.; Zamorano, F.In the CALIPSO data analysis, surface type (land/ocean) is used to augment the aerosol characterization. However, this surface-dependent aerosol typing prohibits a correct classification of marine aerosol over land that is advected from ocean to land. This might result in a systematic overestimation of the particle extinction coefficient and of the aerosol optical thickness (AOT) of up to a factor of 3.5 over land in coastal areas. We present a long-term comparison of CALIPSO and ground-based lidar observations of the aerosol conditions in the coastal environment of southern South America (Punta Arenas, Chile, 53° S), performed in December 2009–April 2010. Punta Arenas is almost entirely influenced by marine particles throughout the year, indicated by a rather low AOT of 0.02–0.04. However, we found an unexpectedly high fraction of continental aerosol in the aerosol types inferred by means of CALIOP observations and, correspondingly, too high values of particle extinction. Similar features of the CALIOP data analysis are presented for four other coastal areas around the world. Since CALIOP data serve as important input for global climate models, the influence of this systematic error was estimated by means of simplified radiative-transfer calculations.
- ItemObservations of turbulence-induced new particle formation in the residual layer(München : European Geopyhsical Union, 2010) Wehner, B.; Siebert, H.; Ansmann, A.; Ditas, F.; Seifert, P.; Stratmann, F.; Wiedensohler, A.; Apituley, A.; Shaw, R.A.; Manninen, H.E.; Kulmala, M.Aerosol particle measurements in the atmospheric boundary layer performed by a helicopter-borne measurement payload and by a lidar system from a case study during the IMPACT field campaign in Cabauw (NL) are presented. Layers of increased number concentrations of ultrafine particles were observed in the residual layer, indicating relatively recent new-particle formation. These layers were characterized by a sub-critical Richardson number and concomitant increased turbulence. Turbulent mixing is likely to lead to local supersaturation of possible precursor gases which are essential for new particle formation. Observed peaks in the number concentrations of ultrafine particles at ground level are connected to the new particle formation in the residual layer by boundary layer development and vertical mixing.
- ItemRadiative effect of aerosols above the northern and southern Atlantic Ocean as determined from shipborne lidar observations(Hoboken, NJ : Wiley, 2013) Kanitz, T.; Ansmann, Albert; Seifert, P.; Engelmann, R.; Althausen, D.The direct solar radiative effect of aerosols over the Atlantic Ocean was investigated on the basis of aerosol Raman/polarization lidar observations aboard the research vessel Polarsternbetween Germany (50°N) and either South America (50°S) or South Africa (40°S) in 2009 and 2010. First, a case study of complex aerosol conditions with marine aerosol, dust, and smoke particles in the boundary layer and free troposphere is presented to demonstrate that detailed knowledge of aerosol layering (boundary layer, free troposphere) and aerosol mixing state is required for an accurate determination of the resulting radiative effects. A statistical analysis based on all lidar observations revealed the highest daily mean radiative effect (−43±59 W m−2at the surface, −14±18 W m−2at top of atmosphere) in the latitudinal belt from 0°N–15°N in the Saharan dust outflow region. Mean aerosol radiative effects of the polluted northern and clean southern midlatitudes were contrasted. In the northern midlatitudes, the averaged aerosol radiative effect of all simulations was −24±33 W m−2at the surface which is a factor of 1.6 higher than at similar southern hemispheric latitudes. The simulations based on the lidar observations are in good agreement with colocated pyranometer measurements.
- ItemLocal and Remote Controls on Arctic Mixed-Layer Evolution(Malden MA: Wiley-Blackwell, 2020) Neggers, R.A.J.; Chylik, J.; Egerer, U.; Griesche, H.; Schemann, V.; Seifert, P.; Siebert, H.; Macke, A.In this study Lagrangian large-eddy simulation of cloudy mixed layers in evolving warm air masses in the Arctic is constrained by in situ observations from the recent PASCAL field campaign. A key novelty is that time dependence is maintained in the large-scale forcings. An iterative procedure featuring large-eddy simulation on microgrids is explored to calibrate the case setup, inspired by and making use of the typically long memory of Arctic air masses for upstream conditions. The simulated mixed-phase clouds are part of a turbulent mixed layer that is weakly coupled to the surface and is occasionally capped by a shallow humidity layer. All eight simulated mixed layers exhibit a strong time evolution across a range of time scales, including diurnal but also synoptic fingerprints. A few cases experience rapid cloud collapse, coinciding with a rapid decrease in mixed-layer depth. To gain insight, composite budget analyses are performed. In the mixed-layer interior the heat and moisture budgets are dominated by turbulent transport, radiative cooling, and precipitation. However, near the thermal inversion the large-scale vertical advection also contributes significantly, showing a distinct difference between subsidence and upsidence conditions. A bulk mass budget analysis reveals that entrainment deepening behaves almost time-constantly, as long as clouds are present. In contrast, large-scale subsidence fluctuates much more strongly and can both counteract and boost boundary-layer deepening resulting from entrainment. Strong and sudden subsidence events following prolonged deepening periods are found to cause the cloud collapses, associated with a substantial reduction in the surface downward longwave radiative flux. ©2019. The Authors.
- ItemInvestigation of the adiabatic assumption for estimating cloud micro- and macrophysical properties from satellite and ground observations(München : European Geopyhsical Union, 2016) Merk, D.; Deneke, H.; Pospichal, B.; Seifert, P.Cloud properties from both ground-based as well as from geostationary passive satellite observations have been used previously for diagnosing aerosol–cloud interactions. In this investigation, a 2-year data set together with four selected case studies are analyzed with the aim of evaluating the consistency and limitations of current ground-based and satellite-retrieved cloud property data sets. The typically applied adiabatic cloud profile is modified using a sub-adiabatic factor to account for entrainment within the cloud. Based on the adiabatic factor obtained from the combination of ground-based cloud radar, ceilometer and microwave radiometer, we demonstrate that neither the assumption of a completely adiabatic cloud nor the assumption of a constant sub-adiabatic factor is fulfilled (mean adiabatic factor 0.63 ± 0.22). As cloud adiabaticity is required to estimate the cloud droplet number concentration but is not available from passive satellite observations, an independent method to estimate the adiabatic factor, and thus the influence of mixing, would be highly desirable for global-scale analyses. Considering the radiative effect of a cloud described by the sub-adiabatic model, we focus on cloud optical depth and its sensitivities. Ground-based estimates are here compared vs. cloud optical depth retrieved from the Meteosat SEVIRI satellite instrument resulting in a bias of −4 and a root mean square difference of 16. While a synergistic approach based on the combination of ceilometer, cloud radar and microwave radiometer enables an estimate of the cloud droplet concentration, it is highly sensitive to radar calibration and to assumptions about the moments of the droplet size distribution. Similarly, satellite-based estimates of cloud droplet concentration are uncertain. We conclude that neither the ground-based nor satellite-based cloud retrievals applied here allow a robust estimate of cloud droplet concentration, which complicates its use for the study of aerosol–cloud interactions.