2022, Pilz, Christian, Düsing, Sebastian, Wehner, Birgit, Müller, Thomas, Siebert, Holger, Voigtländer, Jens, Lonardi, Michael

Airborne observations of vertical aerosol particle distributions are crucial for detailed process studies and model improvements. Tethered balloon systems represent a less expensive alternative to aircraft to probe shallow atmospheric boundary layers (ABLs). This study presents the newly developed cubic aerosol measurement platform (CAMP) for balloon-borne observations of aerosol particle microphysical properties. With an edge length of 35 cm and a weight of 9 kg, the cube is an environmentally robust instrument platform intended for measurements at low temperatures, with a particular focus on applications in cloudy Arctic ABLs. The aerosol instrumentation on board CAMP comprises two condensation particle counters with different lower detection limits, one optical particle size spectrometer, and a miniaturized absorption photometer. Comprehensive calibrations and characterizations of the instruments were performed in laboratory experiments. The first field study with a tethered balloon system took place at the Leibniz Institute for Tropospheric Research (TROPOS) station in Melpitz, Germany, in the winter of 2019. At ambient temperatures between-8 and 15 C, the platform was operated up to a 1.5 km height on 14 flights under both clear-sky and cloudy conditions. The continuous aerosol observations at the ground station served as a reference for evaluating the CAMP measurements. Exemplary profiles are discussed to elucidate the performance of the system and possible process studies. Based on the laboratory instrument characterizations and the observations during the field campaign, CAMP demonstrated the capability to provide comprehensive aerosol particle measurements in cold and cloudy ABLs.

2019, Karpińska, Katarzyna, Bodenschatz, Jonathan F.E., Malinowski, Szymon P., Nowak, Jakub L., Risius, Steffen, Schmeissner, Tina, Shaw, Raymond A., Siebert, Holger, Xi, Hengdong, Xu, Haitao, Bodenschatz, Eberhard

The phenomenon of "cloud voids", i.e., elongated volumes inside a cloud that are devoid of droplets, was observed with laser sheet photography in clouds at a mountain-top station. Two experimental cases, similar in turbulence conditions yet with diverse droplet size distributions and cloud void prevalence, are reported. A theoretical explanation is proposed based on the study of heavy inertial sedimenting particles inside a Burgers vortex. A general conclusion regarding void appearance is drawn from theoretical analysis. Numerical simulations of polydisperse droplet motion with realistic vortex parameters and Mie scattering visual effects accounted for can explain the presence of voids with sizes similar to that of the observed ones. Clustering and segregation effects in a vortex tube are discussed for reasonable cloud conditions. © Author(s) 2019.

2022, Lückerath, Janine, Held, Andreas, Siebert, Holger, Michalkow, Michel, Wehner, Birgit

Aerosol particles are important for radiation effects, cloud formation, and therefore the climate system. A detailed understanding of the spatial distribution of aerosol particles within the atmospheric boundary layer, which depends on sources and sinks, as well as long-range transport and vertical exchange, is important. Especially in marine regions, where the climate effect of clouds is comparably high, long-range transport with subsequent vertical mixing dominates over local aerosol sources. In this study, three different methods were applied to estimate the vertical aerosol particle flux in the marine boundary layer (MBL) and the vertical exchange between the MBL and the free troposphere (FT): eddy covariance (EC), flux–gradient similarity (K theory), and the mixed-layer gradient method (MLG). For the first time, MBL aerosol fluxes derived from these three methods were compared in the framework of the “Azores Stratocumulus Measurements of Radiation, Turbulence and Aerosols” (ACORES) field campaign in the Azores region in the northeastern Atlantic Ocean in July 2017. Meteorological parameters and aerosol and cloud properties were measured in the marine troposphere using the helicopter-borne measurement platform ACTOS (Airborne Cloud Turbulence Observation System). All three methods were applied to estimate the net particle exchange between MBL and FT. In many cases, the entrainment fluxes of the MLG method agreed within the range of uncertainty with the EC and K-theory flux estimates close to the top of the MBL, while the surface flux estimates of the different methods diverged. It was not possible to measure directly above the surface with the helicopter-borne payload, which might be a source of uncertainty in the surface fluxes. The observed particle fluxes at the top of the MBL ranged from 0 to 10×106 m−2 s−1 both in the upward and the downward direction, and the associated uncertainties were on the same order of magnitude. Even though the uncertainties of all three methods are considerable, the results of this study contribute to an improved understanding of the transport of particles between the MBL and FT and their distribution in the MBL.

2016, Wex, Heike, Dieckmann, Katrin, Roberts, Greg C., Conrath, Thomas, Izaguirre, Miguel A., Hartmann, Susan, Herenz, Paul, Schäfer, Michael, Ditas, Florian, Schmeissner, Tina, Henning, Silvia, Wehner, Birgit, Siebert, Holger, Stratmann, Frank

The marine aerosol arriving at Barbados (Ragged Point) was characterized during two 3-week long measurement periods in November 2010 and April 2011, in the context of the measurement campaign CARRIBA (Cloud, Aerosol, Radiation and tuRbulence in the trade wInd regime over BArbados). Through a comparison between ground-based and airborne measurements it was shown that the former are representative of the marine boundary layer at least up to cloud base. In general, total particle number concentrations (Ntotal) ranged from as low as 100  up to 800 cm−3, while number concentrations for cloud condensation nuclei (NCCN) at a supersaturation of 0.26 % ranged from some 10 to 600 cm−3. Ntotal and NCCN depended on the air mass origin. Three distinct types of air masses were found. One type showed elevated values for both Ntotal and NCCN and could be attributed to long-range transport from Africa, by which biomass burning particles from the Sahel region and/or mineral dust particles from the Sahara were advected. The second and third type both had values for NCCN below 200 cm−3 and a clear minimum in the particle number size distribution (NSD) around 70 to 80 nm (Hoppel minimum). While for one of these two types the accumulation mode was dominating (albeit less so than for air masses advected from Africa), the Aitken mode dominated the other and contributed more than 50 % of all particles. These Aitken mode particles likely were formed by new particle formation no more than 3 days prior to the measurements. Hygroscopicity of particles in the CCN size range was determined from CCN measurements to be κ  =  0.66 on average, which suggests that these particles contain mainly sulfate and do not show a strong influence from organic material, which might generally be the case for the months during which measurements were made. The average κ could be used to derive NCCN from measured number size distributions, showing that this is a valid approach to obtain NCCN. Although the total particulate mass sampled on filters was found to be dominated by Na+ and Cl−, this was found to be contributed by a small number of large particles ( >  500 nm, mostly even in the super-micron size range). Based on a three-modal fit, a sea spray mode observed in the NSDs was found to contribute 90 % to the total particulate mass but only 4 to 10 % to Ntotal and up to 15 % to NCCN. This is in accordance with finding no correlation between Ntotal and wind speed.

2016, Babkovskaia, Natalia, Rannik, Ullar, Phillips, Vaughan, Siebert, Holger, Wehner, Birgit, Boy, Michael

The purpose of this study is to investigate the interaction between small-scale turbulence and aerosol and cloud microphysical properties using direct numerical simulations (DNS). We consider the domain located at the height of about 2000 m from the sea level, experiencing transient high supersaturation due to atmospheric fluctuations of temperature and humidity. To study the effect of total number of particles (Ntot) on air temperature, activation and supersaturation, we vary Ntot. To investigate the effect of aerosol dynamics on small-scale turbulence and vertical air motion, we vary the intensity of turbulent fluctuations and the buoyant force. We find that even a small number of aerosol particles (55.5 cm−3), and therefore a small droplet number concentration, strongly affects the air temperature due to release of latent heat. The system comes to an equilibrium faster and the relative number of activated particles appears to be smaller for larger Ntot. We conclude that aerosol particles strongly affect the air motion. In a case of updraught coursed by buoyant force, the presence of aerosol particles results in acceleration of air motion in vertical direction and increase of turbulent fluctuations.

2018, Düsing, Sebastian, Wehner, Birgit, Seifert, Patric, Ansmann, Albert, Baars, Holger, Ditas, Florian, Henning, Silvia, Ma, Nan, Poulain, Laurent, Siebert, Holger, Wiedensohler, Alfred, Macke, Andreas

This paper examines the representativeness of ground-based in situ measurements for the planetary boundary layer (PBL) and conducts a closure study between airborne in situ and ground-based lidar measurements up to an altitude of 2300 m. The related measurements were carried out in a field campaign within the framework of the High-Definition Clouds and Precipitation for Advancing Climate Prediction (HD(CP)2) Observational Prototype Experiment (HOPE) in September 2013 in a rural background area of central Europe. The helicopter-borne probe ACTOS (Airborne Cloud and Turbulence Observation System) provided measurements of the aerosol particle number size distribution (PNSD), the aerosol particle number concentration (PNC), the number concentration of cloud condensation nuclei (CCN-NC), and meteorological atmospheric parameters (e.g., temperature and relative humidity). These measurements were supported by the ground-based 3+2 wavelength polarization lidar system PollyXT, which provided profiles of the particle backscatter coefficient (σbsc) for three wavelengths (355, 532, and 1064 nm). Particle extinction coefficient (σext) profiles were obtained by using a fixed backscatter-to-extinction ratio (also lidar ratio, LR). A new approach was used to determine profiles of CCN-NC for continental aerosol. The results of this new approach were consistent with the airborne in situ measurements within the uncertainties. In terms of representativeness, the PNSD measurements on the ground showed a good agreement with the measurements provided with ACTOS for lower altitudes. The ground-based measurements of PNC and CCN-NC are representative of the PBL when the PBL is well mixed. Locally isolated new particle formation events on the ground or at the top of the PBL led to vertical variability in the cases presented here and ground-based measurements are not entirely representative of the PBL. Based on Mie theory (Mie, 1908), optical aerosol properties under ambient conditions for different altitudes were determined using the airborne in situ measurements and were compared with the lidar measurements. The investigation of the optical properties shows that on average the airborne-based particle light backscatter coefficient is 50.1 % smaller for 1064 nm, 27.4 % smaller for 532 nm, and 29.5 % smaller for 355 nm than the measurements of the lidar system. These results are quite promising, since in situ measurement-based Mie calculations of the particle light backscattering are scarce and the modeling is quite challenging. In contrast, for the particle light extinction coefficient we found a good agreement. The airborne-based particle light extinction coefficient was just 8.2 % larger for 532 nm and 3 % smaller for 355 nm, for an assumed LR of 55 sr. The particle light extinction coefficient for 1064 nm was derived with a LR of 30 sr. For this wavelength, the airborne-based particle light extinction coefficient is 5.2 % smaller than the lidar measurements. For the first time, the lidar ratio of 30 sr for 1064 nm was determined on the basis of in situ measurements and the LR of 55 sr for 355 and 532 nm wavelength was reproduced for European continental aerosol on the basis of this comparison. Lidar observations and the in situ based aerosol optical properties agree within the uncertainties. However, our observations indicate that a determination of the PNSD for a large size range is important for a reliable modeling of aerosol particle backscattering.

2021, Nowak, Jakub L., Siebert, Holger, Szodry, Kai-Erik, Malinowski, Szymon P.

We compare turbulence properties in coupled and decoupled marine stratocumulus-topped boundary layers (STBLs) using high-resolution in situ measurements performed by the helicopter-borne Airborne Cloud Turbulence Observation System (ACTOS) platform in the region of the eastern North Atlantic. The thermodynamically well-mixed coupled STBL was characterized by a comparable latent heat flux at the surface and in the cloud-top region, and substantially smaller sensible heat flux in the entire depth. Turbulence kinetic energy (TKE) was efficiently generated by buoyancy in the cloud and at the surface, and dissipated with comparable rate across the entire depth. Structure functions and power spectra of velocity fluctuations in the inertial range were reasonably consistent with the predictions of Kolmogorov theory. The turbulence was close to isotropic. In the decoupled STBL, decoupling was most obvious in humidity profiles. Heat fluxes and buoyant TKE production at the surface were similar to the coupled case. Around the transition level, latent heat flux decreased to zero and TKE was consumed by weak stability. In the cloud-top region, heat fluxes almost vanished and buoyancy production was significantly smaller than for the coupled case. The TKE dissipation rate inside the decoupled STBL varied between its sublayers. Structure functions and power spectra in the inertial range deviated from Kolmogorov scaling. This was more pronounced in the cloud and subcloud layer in comparison to the surface mixed layer. The turbulence was more anisotropic than in the coupled STBL, with horizontal fluctuations dominating. The degree of anisotropy was largest in the cloud and subcloud layer of the decoupled STBL. Integral length scales, of the order of 100gm in both cases, indicate turbulent eddies smaller than the depth of the coupled STBL or of the sublayers of the decoupled STBL. We hypothesize that turbulence produced in the cloud or close to the surface is redistributed across the entire coupled STBL but rather only inside the sublayers where it was generated in the case of the decoupled STBL. Scattered cumulus convection, developed below the stratocumulus base, may play a role in transport between those sublayers. © 2021 Jakub L. Nowak et al.

2021, Egerer, Ulrike, Ehrlich, André, Gottschalk, Matthias, Griesche, Hannes, Neggers, Roel A.J., Siebert, Holger, Wendisch, Manfred

Specific humidity inversions (SHIs) above low-level cloud layers have been frequently observed in the Arctic. The formation of these SHIs is usually associated with large-scale advection of humid air masses. However, the potential coupling of SHIs with cloud layers by turbulent processes is not fully understood. In this study, we analyze a 3 d period of a persistent layer of increased specific humidity above a stratocumulus cloud observed during an Arctic field campaign in June 2017. The tethered balloon system BELUGA (Balloon-bornE moduLar Utility for profilinG the lower Atmosphere) recorded vertical profile data of meteorological, turbulence, and radiation parameters in the atmospheric boundary layer. An in-depth discussion of the problems associated with humidity measurements in cloudy environments leads to the conclusion that the observed SHIs do not result from measurement artifacts. We analyze two different scenarios for the SHI in relation to the cloud top capped by a temperature inversion: (i) the SHI coincides with the cloud top, and (ii) the SHI is vertically separated from the lowered cloud top. In the first case, the SHI and the cloud layer are coupled by turbulence that extends over the cloud top and connects the two layers by turbulent mixing. Several profiles reveal downward virtual sensible and latent heat fluxes at the cloud top, indicating entrainment of humid air supplied by the SHI into the cloud layer. For the second case, a downward moisture transport at the base of the SHI and an upward moisture flux at the cloud top is observed. Therefore, the area between the cloud top and SHI is supplied with moisture from both sides. Finally, large-eddy simulations (LESs) complement the observations by modeling a case of the first scenario. The simulations reproduce the observed downward turbulent fluxes of heat and moisture at the cloud top. The LES realizations suggest that in the presence of a SHI, the cloud layer remains thicker and the temperature inversion height is elevated.

2017, Macke, Andreas, Seifert, Patric, Baars, Holger, Barthlott, Christian, Beekmans, Christoph, Behrendt, Andreas, Bohn, Birger, Brueck, Matthias, Bühl, Johannes, Crewell, Susanne, Damian, Thomas, Deneke, Hartwig, Düsing, Sebastian, Foth, Andreas, Di Girolamo, Paolo, Hammann, Eva, Heinze, Rieke, Hirsikko, Anne, Kalisch, John, Kalthoff, Norbert, Kinne, Stefan, Kohler, Martin, Löhnert, Ulrich, Madhavan, Bomidi Lakshmi, Maurer, Vera, Muppa, Shravan Kumar, Schween, Jan, Serikov, Ilya, Siebert, Holger, Simmer, Clemens, Späth, Florian, Steinke, Sandra, Träumner, Katja, Trömel, Silke, Wehner, Birgit, Wieser, Andreas, Wulfmeyer, Volker, Xie, Xinxin

The HD(CP)2 Observational Prototype Experiment (HOPE) was performed as a major 2-month field experiment in Jülich, Germany, in April and May 2013, followed by a smaller campaign in Melpitz, Germany, in September 2013. HOPE has been designed to provide an observational dataset for a critical evaluation of the new German community atmospheric icosahedral non-hydrostatic (ICON) model at the scale of the model simulations and further to provide information on land-surface-atmospheric boundary layer exchange, cloud and precipitation processes, as well as sub-grid variability and microphysical properties that are subject to parameterizations. HOPE focuses on the onset of clouds and precipitation in the convective atmospheric boundary layer. This paper summarizes the instrument set-ups, the intensive observation periods, and example results from both campaigns.

HOPE-Jülich instrumentation included a radio sounding station, 4 Doppler lidars, 4 Raman lidars (3 of them provide temperature, 3 of them water vapour, and all of them particle backscatter data), 1 water vapour differential absorption lidar, 3 cloud radars, 5 microwave radiometers, 3 rain radars, 6 sky imagers, 99 pyranometers, and 5 sun photometers operated at different sites, some of them in synergy. The HOPE-Melpitz campaign combined ground-based remote sensing of aerosols and clouds with helicopter- and balloon-based in situ observations in the atmospheric column and at the surface.

HOPE provided an unprecedented collection of atmospheric dynamical, thermodynamical, and micro- and macrophysical properties of aerosols, clouds, and precipitation with high spatial and temporal resolution within a cube of approximately 10 × 10 × 10km3. HOPE data will significantly contribute to our understanding of boundary layer dynamics and the formation of clouds and precipitation. The datasets have been made available through a dedicated data portal.

First applications of HOPE data for model evaluation have shown a general agreement between observed and modelled boundary layer height, turbulence characteristics, and cloud coverage, but they also point to significant differences that deserve further investigations from both the observational and the modelling perspective.

2014, Hoffmann, Fabian, Siebert, Holger, Schumacher, Jörg, Riechelmann, Theres, Katzwinkel, Jeannine, Kumar, Bipin, Götzfried, Paul, Raasch, Siegfried

This study combines observations, large-eddy simulations (LES), and direct numerical simulations (DNS) in order to analyze entrainment and mixing in shallow cumulus clouds at all relevant spatial scales and, additionally, to verify the results by the multiple methods used. The observations are based on three flights of the CARRIBA campaign which are similar to the classical BOMEX case used for LES. Virtual flights in the LES data are used to validate the observational method of line measurements. It is shown that line measurements overrepresent the cloud core, and it is quantified how derived statistics depend on small perturbations of the flight track, which has to be taken in account for the interpretation of airborne observations. A linear relation between fluctuations of temperature and liquid water content has been found in both LES and observations in a good quantitative agreement. However, the constant of proportionality deviates from purely adiabatic estimates, which can be attributed to cloud edge mixing. The cloud edge is compared in detail in observations and LES, which agree qualitatively although the LES cloud edge is smoother due to the model's resolution. The resulting typical amplitudes of the turbulence fields from this comparison are compared with the large-scale forcing model which is used in a series of DNS which study the mixing below the meter scale, which show that LES does not resolve the intermittency of small-scale turbulence.