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Now showing 1 - 10 of 12
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    Properties of arctic haze aerosol from lidar observations during iarea 2015 campaign on spitsbergen
    (Les Ulis : EDP Sciences, 2018) Stachlewska, Iwona S.; Ritter, Christoph; Böckmann, Christine; Engelmann, Ronny; Nicolae, D.; Makoto, A.; Vassilis, A.; Balis, D.; Behrendt, A.; Comeron, A.; Gibert, F.; Landulfo, E.; McCormick, M.P.; Senff, C.; Veselovskii, I.; Wandinger, U.
    Arctic Haze event was observed on 5-8 April 2015 using simultaneously Near-range Aerosol Raman Lidar of IGFUW and Koldewey Aerosol Raman Lidar of AWI, both based at AWIPEV German-French station in Ny-Ålesund, Spitsbergen. The alterations in particle abundance and altitude of the aerosol load observed on following days of the event is analyzed. The daytime profiles of particle optical properties were obtained for both lidars, and then served as input for microphysical parameters inversion. The results indicate aerosol composition typical for the Arctic Haze. However, in some layers, a likely abundance of aqueous aerosol or black carbon originating in biomass burning over Siberia, changes measurably the Arctic Haze properties.
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    Lidar Measurements of Canadian Forest Fire Smoke Episode Observed in July 2013 over Warsaw, Poland
    (Les Ulis : EDP Sciences, 2016) Janicka, Lucja; Stachlewska, Iwona S.; Markowicz, Krzysztof M.; Baars, Holger; Engelmann, Ronny; Heese, Birgit; Gross, Barry; Moshary, F.; Arend, M.
    This paper presents a preliminary study of aerosol optical properties of air-mass advected on 10th July 2013 from Canada above Warsaw, Poland, during the forest fire event that occurred in Quebec at the beginning of July 2013. The observations were conducted with use of the modern version of 8-channel PollyXT lidar capable of measuring at 3β+2α+2δ+VW and interpreted with available information from the MACC model, the CALIPSO and MODIS satellite sensors, the AERONET data products and the data gathered within the Poland-AOD network.
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    Lidar derived properties of air-masses advected from Ukraine, Sahara and Carpathian mountains to Warsaw, Poland on 9 - 11 August 2015
    (Les Ulis : EDP Sciences, 2018) Janicka, Lucja; Szczepanik, Dominika; Borek, Karolina; Heese, Birgit; Stachlewska, Iwona S.; Nicolae, D.; Makoto, A.; Vassilis, A.; Balis, D.; Behrendt, A.; Comeron, A.; Gibert, F.; Landulfo, E.; McCormick, M.P.; Senff, C.; Veselovskii, I.; Wandinger, U.
    The aerosol layers of different origin, suspended in the atmosphere on 9-11 August 2015 were observed with the PollyXT-UW lidar in Warsaw, Poland. The HYSPLIT ensemble backward trajectories indicate that the observed air-masses attribute to a few different sources, among others, possible transport paths from Ukraine, Slovakia, and Africa. In this paper, we attempt to analyse and discuss the properties of aerosol particles of different origin that were suspended over Warsaw during this event.
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    The unprecedented 2017–2018 stratospheric smoke event: decay phase and aerosol properties observed with the EARLINET
    (Katlenburg-Lindau : EGU, 2019) Baars, Holger; Ansmann, Albert; Ohneiser, Kevin; Haarig, Moritz; Engelmann, Ronny; Althausen, Dietrich; Hanssen, Ingrid; Gausa, Michael; Pietruczuk, Aleksander; Szkop, Artur; Stachlewska, Iwona S.; Wang, Dongxiang; Reichardt, Jens; Skupin, Annett; Mattis, Ina; Trickl, Thomas; Vogelmann, Hannes; Navas-Guzmán, Francisco; Haefele, Alexander; Acheson, Karen; Ruth, Albert A.; Tatarov, Boyan; Müller, Detlef; Hu, Qiaoyun; Podvin, Thierry; Goloub, Philippe; Veselovskii, Igor; Pietras, Christophe; Haeffelin, Martial; Fréville, Patrick; Sicard, Michaël; Comerón, Adolfo; García, Alfonso Javier Fernández; Molero Menéndez, Francisco; Córdoba-Jabonero, Carmen; Guerrero-Rascado, Juan Luis; Alados-Arboledas, Lucas; Bortoli, Daniele; Costa, Maria João; Dionisi, Davide; Liberti, Gian Luigi; Wang, Xuan; Sannino, Alessia; Papagiannopoulos, Nikolaos; Boselli, Antonella; Mona, Lucia; D’Amico, Guiseppe; Romano, Salvatore; Perrone, Maria Rita; Belegante, Livio; Nicolae, Doina; Grigorov, Ivan; Gialitaki, Anna; Amiridis, Vassilis; Soupiona, Ourania; Papayannis, Alexandros; Mamouri, Rodanthi-Elisaveth; Nisantzi, Argyro; Heese, Birgit; Hofer, Julian; Schechner, Yoav Y.; Wandinger, Ulla; Pappalardo, Gelsomina
    Six months of stratospheric aerosol observations with the European Aerosol Research Lidar Network (EARLINET) from August 2017 to January 2018 are presented. The decay phase of an unprecedented, record-breaking stratospheric perturbation caused by wildfire smoke is reported and discussed in terms of geometrical, optical, and microphysical aerosol properties. Enormous amounts of smoke were injected into the upper troposphere and lower stratosphere over fire areas in western Canada on 12 August 2017 during strong thunderstorm–pyrocumulonimbus activity. The stratospheric fire plumes spread over the entire Northern Hemisphere in the following weeks and months. Twenty-eight European lidar stations from northern Norway to southern Portugal and the eastern Mediterranean monitored the strong stratospheric perturbation on a continental scale. The main smoke layer (over central, western, southern, and eastern Europe) was found at heights between 15 and 20 km since September 2017 (about 2 weeks after entering the stratosphere). Thin layers of smoke were detected at heights of up to 22–23 km. The stratospheric aerosol optical thickness at 532 nm decreased from values > 0.25 on 21–23 August 2017 to 0.005–0.03 until 5–10 September and was mainly 0.003–0.004 from October to December 2017 and thus was still significantly above the stratospheric background (0.001–0.002). Stratospheric particle extinction coefficients (532 nm) were as high as 50–200 Mm−1 until the beginning of September and on the order of 1 Mm−1 (0.5–5 Mm−1) from October 2017 until the end of January 2018. The corresponding layer mean particle mass concentration was on the order of 0.05–0.5 µg m−3 over these months. Soot particles (light-absorbing carbonaceous particles) are efficient ice-nucleating particles (INPs) at upper tropospheric (cirrus) temperatures and available to influence cirrus formation when entering the tropopause from above. We estimated INP concentrations of 50–500 L−1 until the first days in September and afterwards 5–50 L−1 until the end of the year 2017 in the lower stratosphere for typical cirrus formation temperatures of −55 ∘C and an ice supersaturation level of 1.15. The measured profiles of the particle linear depolarization ratio indicated a predominance of nonspherical smoke particles. The 532 nm depolarization ratio decreased slowly with time in the main smoke layer from values of 0.15–0.25 (August–September) to values of 0.05–0.10 (October–November) and < 0.05 (December–January). The decrease of the depolarization ratio is consistent with aging of the smoke particles, growing of a coating around the solid black carbon core (aggregates), and thus change of the shape towards a spherical form. We found ascending aerosol layer features over the most southern European stations, especially over the eastern Mediterranean at 32–35∘ N, that ascended from heights of about 18–19 to 22–23 km from the beginning of October to the beginning of December 2017 (about 2 km per month). We discuss several transport and lifting mechanisms that may have had an impact on the found aerosol layering structures.
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    Microphysical characterization of long-range transported biomass burning particles from North America at three EARLINET stations
    (Katlenburg-Lindau : EGU, 2017) Ortiz-Amezcua, Pablo; Guerrero-Rascado, Juan Luis; Granados-Muñoz, María José; Benavent-Oltra, José Antonio; Böckmann, Christine; Samaras, Stefanos; Stachlewska, Iwona S.; Janicka, Łucja; Baars, Holger; Bohlmann, Stephanie; Alados-Arboledas, Lucas
    Strong events of long-range transported biomass burning aerosol were detected during July 2013 at three EARLINET (European Aerosol Research Lidar Network) stations, namely Granada (Spain), Leipzig (Germany) and Warsaw (Poland). Satellite observations from MODIS (Moderate Resolution Imaging Spectroradiometer) and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) instruments, as well as modeling tools such as HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) and NAAPS (Navy Aerosol Analysis and Prediction System), have been used to estimate the sources and transport paths of those North American forest fire smoke particles. A multiwavelength Raman lidar technique was applied to obtain vertically resolved particle optical properties, and further inversion of those properties with a regularization algorithm allowed for retrieving microphysical information on the studied particles. The results highlight the presence of smoke layers of 1-2 km thickness, located at about 5 km a.s.l. altitude over Granada and Leipzig and around 2.5 km a.s.l. at Warsaw. These layers were intense, as they accounted for more than 30 % of the total AOD (aerosol optical depth) in all cases, and presented optical and microphysical features typical for different aging degrees: Color ratio of lidar ratios (LR532/LR355) around 2, α-related ängström exponents of less than 1, effective radii of 0.3 μm and large values of single scattering albedos (SSA), nearly spectrally independent. The intensive microphysical properties were compared with columnar retrievals form co-located AERONET (Aerosol Robotic Network) stations. The intensity of the layers was also characterized in terms of particle volume concentration, and then an experimental relationship between this magnitude and the particle extinction coefficient was established.
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    Earlinet validation of CATS L2 product
    (Les Ulis : EDP Sciences, 2018) Proestakis, Emmanouil; Amiridis, Vassilis; Kottas, Michael; Marinou, Eleni; Binietoglou, Ioannis; Ansmann, Albert; Wandinger, Ulla; Yorks, John; Nowottnick, Edward; Makhmudov, Abduvosit; Papayannis, Alexandros; Pietruczuk, Aleksander; Gialitaki, Anna; Apituley, Arnoud; Muñoz-Porcar, Constantino; Bortoli, Daniele; Dionisi, Davide; Althausen, Dietrich; Mamali, Dimitra; Balis, Dimitris; Nicolae, Doina; Tetoni, Eleni; Luigi Liberti, Gian; Baars, Holger; Stachlewska, Iwona S.; Voudouri, Kalliopi-Artemis; Mona, Lucia; Mylonaki, Maria; Rita Perrone, Maria; João Costa, Maria; Sicard, Michael; Papagiannopoulos, Nikolaos; Siomos, Nikolaos; Burlizzi, Pasquale; Engelmann, Ronny; Abdullaev, Sabur F.; Hofer, Julian; Pappalardo, Gelsomina; Nicolae, D.; Makoto, A.; Vassilis, A.; Balis, D.; Behrendt, A.; Comeron, A.; Gibert, F.; Landulfo, E.; McCormick, M.P.; Senff, C.; Veselovskii, I.; Wandinger, U.
    The Cloud-Aerosol Transport System (CATS) onboard the International Space Station (ISS), is a lidar system providing vertically resolved aerosol and cloud profiles since February 2015. In this study, the CATS aerosol product is validated against the aerosol profiles provided by the European Aerosol Research Lidar Network (EARLINET). This validation activity is based on collocated CATS-EARLINET measurements and the comparison of the particle backscatter coefficient at 1064nm.
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    Effect of heatwave conditions on aerosol optical properties derived from satellite and ground-based remote sensing over Poland
    (Basel : MDPI, 2017) Stachlewska, Iwona S.; Zawadzka, Olga; Engelmann, Ronny
    During an exceptionally warm September in 2016, unique and stable weather conditions contributed to a heat wave over Poland, allowing for observations of aerosol optical properties, using a variety of ground-based and satellite remote sensors. The data set collected during 11–16 September 2016 was analysed in terms of aerosol transport (HYbrid Single-Particle Lagrangian Integrated Trajectory model (HYSPLIT)), aerosol load model simulations (Copernicus Atmosphere Monitoring Service (CAMS), Navy Aerosol Analysis and Prediction System (NAAPS), Global Environmental Multiscale-Air Quality (GEM-AQ), columnar aerosol load measured at ground level (Aerosol Robotic NETwork (AERONET), Polish Aerosol Research Network (PolandAOD)) and from satellites (Spinning Enhanced Visible and Infrared Imager (SEVIRI), Moderate Resolution Imaging Spectroradiometer (MODIS)), as well as with 24/7 PollyXT Raman Lidar observations at the European Aerosol Research Lidar Network (EARLINET) site in Warsaw. Analyses revealed a single day of a relatively clean background aerosol related to an Arctic air-mass inflow, surrounded by a few days with a well increased aerosol load of differing origin: pollution transported from Germany and biomass burning from Ukraine. Such conditions proved excellent to test developed-in-house algorithms designed for near real-time aerosol optical depth (AOD) derivation from the SEVIRI sensor. The SEVIRI AOD maps derived over the territory of Poland, with an exceptionally high resolution (every 15 min; 5.5 × 5.5 km2), revealed on an hourly scale, very low aerosol variability due to heat wave conditions. Comparisons of SEVIRI with NAAPS and CAMS AOD maps show strong qualitative similarities; however, NAAPS underestimates AOD and CAMS tends to underestimate it on relatively clean days (<0.2), and overestimate it for a high aerosol load (>0.4). A slight underestimation of the SEVIRI AOD is reported for pixel-to-column comparisons with AODs of several radiometers (AERONET, PolandAOD) and Lidar (EARLINET) with high correlation coefficients (r2 of 0.8–0.91) and low root-mean-square error (RMSE of 0.03–0.05). A heat wave driven increase of the boundary layer height of 10% is accompanied with the AOD increase of 8–12% for an urban site dominated by anthropogenic pollution. Contrary trend, with an AOD decrease of around 4% for a rural site dominated by a long-range transported biomass burning aerosol is reported. There is a positive feedback of heat wave conditions on local and transported pollution and an extenuating effect on transported biomass burning aerosol. The daytime mean SEVIRI PM2.5 converted from the SEVIRI AODs at a pixel representative for Warsaw is in agreement with the daily mean PM2.5 surface measurements, whereby SEVIRI PM2.5 and Lidar-derived Ångström exponent are anti-correlated.
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    Variability of the boundary layer over an urban continental site based on 10 years of active remote sensing observations in Warsaw
    (Basel : MDPI, 2020) Wang, Dongxiang; Stachlewska, Iwona S.; Song, Xiaoquan; Heese, Birgit; Nemuc, Anca
    Atmospheric boundary layer height (ABLH) was observed by the CHM15k ceilometer (January 2008 to October 2013) and the PollyXT lidar (July 2013 to December 2018) over the European Aerosol Research LIdar NETwork to Establish an Aerosol Climatology (EARLINET) site at the Remote Sensing Laboratory (RS-Lab) in Warsaw, Poland. Out of a maximum number of 4017 observational days within this period, a subset of quasi-continuous measurements conducted with these instruments at the same wavelength (1064 nm) was carefully chosen. This provided a data sample of 1841 diurnal cycle ABLH observations. The ABLHs were derived from ceilometer and lidar signals using the wavelet covariance transform method (WCT), gradient method (GDT), and standard deviation method (STD). For comparisons, the rawinsondes of the World Meteorological Organization (WMO 12374 site in Legionowo, 25 km distance to the RS-Lab) were used. The ABLHs derived from rawinsondes by the skew-T-log-p method and the bulk Richardson (bulk-Ri) method had a linear correlation coefficient (R2) of 0.9 and standard deviation (SD) of 0.32 km. A comparison of the ABLHs obtained for different methods and instruments indicated a relatively good agreement. The ABLHs estimated from the rawinsondes with the bulk-Ri method had the highest correlations, R2 of 0.80 and 0.70 with the ABLHs determined using the WCT method on ceilometer and lidar signals, respectively. The three methods applied to the simultaneous, collocated lidar, and ceilometer observations (July to October 2013) showed good agreement, especially for the WCT method (R2 of 0.94, SD of 0.19 km). A scaling threshold-based algorithm was proposed to homogenize ceilometer and lidar datasets, which were applied on the lidar data, and significantly improved the coherence of the results (R2 of 0.98, SD of 0.11 km). The difference of ABLH between clear-sky and cloudy conditions was on average below 230 m for the ceilometer and below 70 m for the lidar retrievals. The statistical analysis of the long-term observations indicated that the monthly mean ABLHs varied throughout the year between 0.6 and 1.8 km. The seasonal mean ABLH was of 1.16 ± 0.16 km in spring, 1.34 ± 0.15 km in summer, 0.99 ± 0.11 km in autumn, and 0.73 ± 0.08 km in winter. In spring and summer, the daytime and nighttime ABLHs appeared mainly in a frequency distribution range of 0.6 to 1.0 km. In winter, the distribution was common between 0.2 and 0.6 km. In autumn, it was relatively balanced between 0.2 and 1.2 km. The annual mean ABLHs maintained between 0.77 and 1.16 km, whereby the mean heights of the well-mixed, residual, and nocturnal layer were 1.14 ± 0.11, 1.27 ± 0.09, and 0.71 ± 0.06 km, respectively (for clear-sky conditions). For the whole observation period, the ABLHs below 1 km constituted more than 60% of the retrievals. A strong seasonal change of the monthly mean ABLH diurnal cycle was evident; a mild weakly defined autumn diurnal cycle, followed by a somewhat flat winter diurnal cycle, then a sharp transition to a spring diurnal cycle, and a high bell-like summer diurnal cycle. A prolonged summertime was manifested by the September cycle being more similar to the summer than autumn cycles.
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    First Ever Observations of Mineral Dust in Wintertime over Warsaw, Poland
    (Basel : MDPI, 2022) Szczepanik, Dominika M.; Ortiz-Amezcua, Pablo; Heese, Birgit; D’Amico, Giuseppe; Stachlewska, Iwona S.
    The long-range transport of desert dust over the area of the temperate climate zone is associated with the influx of hot air masses due to the location of the sources of this aerosol in the tropical climate zone. Between 24–26 February 2021, such an aerosol outbreak took place and reached Central Europe. The mean temperature of +11.7 °C was recorded during the event. A comparison of this value to the 20-year (2000–2020) average February temperature for Warsaw (−0.2 °C) indicates the uniqueness of the meteorological conditions. It was the first wintertime inflow of Saharan dust over Warsaw, the presence of which was confirmed by lidar and sun-photometer measurements. The properties of the desert dust layers were obtained; the mean values of the particle depolarization for the fully developed mineral dust layer were 13 ± 3% and 22 ± 4% for 355 and 532 nm, respectively. The aerosol optical thickness was high with average values >0.36 for all wavelengths smaller than 500 nm. The three-modal, aerosol size distribution was dominated by coarse-mode particles, with a visible contribution of accumulation-mode particles. It suggests the possible presence of other aerosol types.
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    Modification of local urban aerosol properties by long-range transport of biomass burning aerosol
    (Basel : MDPI, 2018) Stachlewska, Iwona S.; Samson, Mateusz; Zawadzka, Olga; Harenda, Kamila M.; Janicka, Lucja; Poczta, Patryk; Szczepanik, Dominika; Heese, Birgit; Wang, Dongxiang; Borek, Karolina; Tetoni, Eleni; Proestakis, Emmanouil; Siomos, Nikolaos; Nemuc, Anca; Chojnicki, Bogdan H.; Markowicz, Krzysztof M.; Pietruczuk, Aleksander; Szkop, Artur; Althausen, Dietrich; Stebel, Kerstin; Schuettemeyer, Dirk; Zehner, Claus
    During August 2016, a quasi-stationary high-pressure system spreading over Central and North-Eastern Europe, caused weather conditions that allowed for 24/7 observations of aerosol optical properties by using a complex multi-wavelength PollyXT lidar system with Raman, polarization and water vapour capabilities, based at the European Aerosol Research Lidar Network (EARLINET network) urban site in Warsaw, Poland. During 24–30 August 2016, the lidar-derived products (boundary layer height, aerosol optical depth, Ångström exponent, lidar ratio, depolarization ratio) were analysed in terms of air mass transport (HYSPLIT model), aerosol load (CAMS data) and type (NAAPS model) and confronted with active and passive remote sensing at the ground level (PolandAOD, AERONET, WIOS-AQ networks) and aboard satellites (SEVIRI, MODIS, CATS sensors). Optical properties for less than a day-old fresh biomass burning aerosol, advected into Warsaw’s boundary layer from over Ukraine, were compared with the properties of long-range transported 3–5 day-old aged biomass burning aerosol detected in the free troposphere over Warsaw. Analyses of temporal changes of aerosol properties within the boundary layer, revealed an increase of aerosol optical depth and Ångström exponent accompanied by an increase of surface PM10 and PM2.5. Intrusions of advected biomass burning particles into the urban boundary layer seem to affect not only the optical properties observed but also the top height of the boundary layer, by moderating its increase.