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Author: Steglich, F. × Subject: Magnetic properties ×

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    Phase transition and anomalous low temperature ferromagnetic phase in Pr 0.6Sr 0.4MnO 3 single crystals
    (New York, NY : Springer Science + Business Media B.V., 2009) Rößler, S.; Harikrishnan, S.; Naveen Kumar, C.M.; Bhat, H.L.; Elizabeth, S.; Rößler, U.K.; Steglich, F.; Wirth, S.
    We report on the magnetic and electrical properties of Pr 0.6Sr 0.4MnO 3 single crystals. This compound undergoes a continuous paramagnetic-ferromagnetic transition with a Curie temperature T C301 K and a first-order structural transition at T S64 K. At T S, the magnetic susceptibility exhibits an abrupt jump, and a corresponding small hump is seen in the resistivity. The critical behavior of the static magnetization and the temperature dependence of the resistivity are consistent with the behavior expected for a nearly isotropic ferromagnet with short-range exchange belonging to the Heisenberg universality class. The magnetization (M-H) curves below T S are anomalous in that the virgin curve lies outside the subsequent M-H loops. The hysteretic structural transition at T S as well as the irreversible magnetization processes below T S can be explained by phase separation between a high-temperature orthorhombic and a low-temperature monoclinic ferromagnetic phase.
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    High-field phase diagram of the heavy-fermion metal YbRh2Si2
    (Milton Park : Taylor & Francis, 2006) Gegenwart, P.; Tokiwa, Y.; Westerkamp, T.; Weickert, F.; Custers, J.; Ferstl, J.; Krellner, C.; Geibel, C.; Kerschl, P.; Müller, K.-H.; Steglich, F.
    The tetragonal heavy-fermion (HF) metal YbRh2Si2 (Kondo temperature TK≈ 25 K) exhibits a magnetic field-induced quantum critical point related to the suppression of very weak antiferromagnetic (AF) ordering (TN = 70 mK) at a critical field of Bc = 0.06 T (B⊥ c). To understand the influence of magnetic fields on quantum criticality and the Kondo effect, we study the evolution of various thermodynamic and magnetic properties upon tuning the system by magnetic field. At B > Bc, the AF component of the quantum critical fluctuations becomes suppressed, and FM fluctuations dominate. Their polarization with magnetic field gives rise to a large increase of the magnetization. At B* = 10 T, the Zeeman energy becomes comparable to kB TK, and a steplike decrease of the quasi-particle mass deduced from the specific-heat coefficient indicates the suppression of HF behaviour. The magnetization M(B) shows a pronounced decrease in slope at B* without any signature of metamagnetism. The field dependence of the linear magnetostriction coefficient suggests an increase of the Yb-valency with field, reaching 3+ at high fields. A negative hydrostatic pressure dependence of B* is found, similar to that of the Kondo temperature. We also compare the magnetization behaviour in pulsed fields up to 50 T with that of the isoelectronic HF system YbIr2Si2, which, due to a larger unit-cell volume, has an enhanced TK of about 40 K.