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Now showing 1 - 5 of 5
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    Kramers-Kronig relations and high order nonlinear susceptibilities
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2011) Brée, Carsten; Demircan, Ayhan; Steinmeyer, Günter
    As previous theoretical results recently revealed, a Kramers-Kronig transform of multiphoton absorption rates allows for a precise prediction on the dispersion of the nonlinear refractive index $n_2$ in the near IR. It was shown that this method allows to reproduce recent experimental results on the importance of the higher-order Kerr effect. Extending these results, the current manuscript provides the dispersion of $n_2$ for all noble gases in excellent agreement with reference data. It is furthermore established that the saturation and inversion of the nonlinear refractive index is highly dispersive with wavelength, which indicates the existence of different filamentation regimes. While shorter laser wavelengths favor the well-established plasma clamping regime, the influence of the higher-order Kerr effect dominates in the long wavelength regime.
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    Filamentary pulse self-compression : the impact of the cell windows
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2011) Brée, Carsten; Demircan, Ayhan; Bethge, Jens; Nibbering, Erik T.J.; Skupin, Stefan; Bergé, Luc; Steinmeyer, Günter
    Self-compression of multi-millijoule laser pulses during filamentary propagation is usually explained by the interplay of self-focusing and defocusing effects, causing a substantial concentration of energy on the axis of the propagating optical pulse. Recently, it has been argued that cell windows may play a decisive role in the self-compression mechanism. As such windows have to be used for media other than air their presence is often unavoidable, yet they present a sudden non-adiabatic change in dispersion and nonlinearity that should lead to a destruction of the temporal and spatial integrity of the light bullets generated in the self-compression mechanism. We now experimentally prove that there is in fact a self-healing mechanism that helps to overcome the potentially destructive consequences of the cell windows. We show in two carefully conducted experiments that the cell window position decisively influences activation or inhibition of the self-healing mechanism. A comparison with a windowless cell shows that presence of this mechanism is an important prerequisite for the exploitation of self-compression effects in windowed cells filled with inert gases.
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    Non-instantaneous polarization dynamics in dielectric media
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2014) Hofmann, Michael; Hyyti, Janne; Birkholz, Simon; Bock, Martin; Das, Susanta K.; Grunwald, Rüdiger; Hoffmann, Mathias; Nagy, Tamas; Demircan, Ayhan; Jupé, Marco; Ristau, Detlev; Morgner, Uwe; Brée, Carsten; Woerner, Michael; Elsaesser, Thomas; Steinmeyer, Günter
    Third-order optical nonlinearities play a vital role for generation1,2 and characterization 3-5 of some of the shortest optical pulses to date, for optical switching applications6,7, and for spectroscopy8,9. In many cases, nonlinear optical effects are used far off resonance, and then an instantaneous temporal response is expected. Here, we show for the first time resonant frequency-resolved optical gating measurements1012 that indicate substantial nonlinear polarization relaxation times up to 6.5 fs in dielectric media, i.e., significantly beyond the shortest pulses directly available from commercial lasers. These effects are among the fastest effects observed in ultrafast spectroscopy. Numerical solutions of the time-dependent Schrödinger equation13,14 are in excellent agreement with experimental observations. The simulations indicate that pulse generation and characterization in the ultraviolet may be severely affected by this previously unreported effect. Moreover, our approach opens an avenue for application of frequency-resolved optical gating as a highly selective spectroscopic probe in high-field physics.
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    Adjustable pulse compression scheme for generation of few-cycle pulses in the mid-infrared
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2014) Demircan, Ayhan; Amiranashvili, Shalva; Brée, Carsten; Morgner, Uwe; Steinmeyer, Günter
    An novel adjustable adiabatic soliton compression scheme is presented, enabling a coherent pulse source with pedestal-free few-cycle pulses in the infrared or mid-infrared regime. This scheme relies on interaction of a dispersive wave and a soliton copropagating at nearly identical group velocities in a fiber with enhanced infrared transmission. The compression is achieved directly in one stage, without necessity of an external compensation scheme. Numerical simulations are employed to demonstrate this scheme for silica and fluoride fibers, indicating ultimate limitations as well as the possibility of compression down to the single-cycle regime. Such output pulses appear ideally suited as seed sources for parametric amplification schemes in the mid-infrared.
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    Rogue wave formation by accelerated solitons at an optical event horizon
    (Berlin : Weierstraß-Institut für Angewandte Analysis und Stochastik, 2013) Demircan, Ayhan; Amiranashvili, Shalva; Brée, Carsten; Mahnke, Christoph; Mitschke, Fedor; Steinmeyer, Günter
    Rogue waves, by definition, are rare events of extreme amplitude, but at the same time they are frequent in the sense that they can exist in a wide range of physical contexts. While many mechanisms have been demonstrated to explain the appearance of rogue waves in various specific systems, there is no known generic mechanism or general set of criteria shown to rule their appearance. Presupposing only the existence of a nonlinear Schrödinger-type equation together with a concave dispersion profile around a zero dispersion wavelength we demonstrate that solitons may experience acceleration and strong reshaping due to the interaction with continuum radiation, giving rise to extreme-value phenomena. The mechanism is independent of the optical Raman effect. A strong increase of the peak power is accompanied by a mild increase of the pulse energy and carrier frequency, whereas the photon number of the soliton remains practically constant. This reshaping mechanism is particularly robust and is naturally given in optics in the supercontinuum generation process.