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GARRLiC and LIRIC: Strengths and limitations for the characterization of dust and marine particles along with their mixtures

2017, Tsekeri, Alexandra, Lopatin, Anton, Amiridis, Vassilis, Marinou, Eleni, Igloffstein, Julia, Siomos, Nikolaos, Solomos, Stavros, Kokkalis, Panagiotis, Engelmann, Ronny, Baars, Holger, Gratsea, Myrto, Raptis, Panagiotis I., Binietoglou, Ioannis, Mihalopoulos, Nikolaos, Kalivitis, Nikolaos, Kouvarakis, Giorgos, Bartsotas, Nikolaos, Kallos, George, Basart, Sara, Schuettemeyer, Dirk, Wandinger, Ulla, Ansmann, Albert, Chaikovsky, Anatoli P., Dubovik, Oleg

The Generalized Aerosol Retrieval from Radiometer and Lidar Combined data algorithm (GARRLiC) and the LIdar-Radiometer Inversion Code (LIRIC) provide the opportunity to study the aerosol vertical distribution by combining ground-based lidar and sun-photometric measurements. Here, we utilize the capabilities of both algorithms for the characterization of Saharan dust and marine particles, along with their mixtures, in the south-eastern Mediterranean during the CHARacterization of Aerosol mixtures of Dust and Marine origin Experiment (CHARADMExp). Three case studies are presented, focusing on dust-dominated, marinedominated and dust-marine mixing conditions. GARRLiC and LIRIC achieve a satisfactory characterization for the dust-dominated case in terms of particle microphysical properties and concentration profiles. The marine-dominated and the mixture cases are more challenging for both algorithms, although GARRLiC manages to provide more detailed microphysical retrievals compared to AERONET, while LIRIC effectively discriminates dust and marine particles in its concentration profile retrievals. The results are also compared with modelled dust and marine concentration profiles and surface in situ measurements.

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Extreme levels of Canadian wildfire smoke in the stratosphere over central Europe on 21-22 August 2017

2018, Ansmann, Albert, Baars, Holger, Chudnovsky, Alexandra, Mattis, Ina, Veselovskii, Igor, Haarig, Moritz, Seifert, Patric, Engelmann, Ronny, Wandinger, Ulla

Light extinction coefficients of 500 Mm1, about 20 times higher than after the Pinatubo volcanic eruptions in 1991, were observed by European Aerosol Research Lidar Network (EARLINET) lidars in the stratosphere over central Europe on 21-22 August 2017. Pronounced smoke layers with a 1-2 km vertical extent were found 2-5 km above the local tropopause. Optically dense layers of Canadian wildfire smoke reached central Europe 10 days after their injection into the upper troposphere and lower stratosphere which was caused by rather strong pyrocumulonimbus activity over western Canada. The smoke-related aerosol optical thickness (AOT) identified by lidar was close to 1.0 at 532 nm over Leipzig during the noon hours on 22 August 2017. Smoke particles were found throughout the free troposphere (AOT of 0.3) and in the pronounced 2 km thick stratospheric smoke layer at an altitude of 14-16 km (AOT of 0.6). The lidar observations indicated peak mass concentrations of 70-100 μgm-3 in the stratosphere. In addition to the lidar profiles, we analyzed Moderate Resolution Imaging Spectroradiometer (MODIS) fire radiative power (FRP) over Canada, and the distribution of MODIS AOT and Ozone Monitoring Instrument (OMI) aerosol index across the North Atlantic. These instruments showed a similar pattern and a clear link between the western Canadian fires and the aerosol load over Europe. In this paper, we also present Aerosol Robotic Network (AERONET) sun photometer observations, compare photometer and lidar-derived AOT, and discuss an obvious bias (the smoke AOT is too low) in the photometer observations. Finally, we compare the strength of this recordbreaking smoke event (in terms of the particle extinction coefficient and AOT) with major and moderate volcanic events observed over the northern midlatitudes.

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Earthcare atlid extinction and backscatter retrieval algorithms

2018, Donovan, David, van Zadelhoff, Gerd-Jan, Daou, David, Wandinger, Ulla, Nicolae, D., Makoto, A., Vassilis, A., Balis, D., Behrendt, A., Comeron, A., Gibert, F., Landulfo, E., McCormick, M.P., Senff, C., Veselovskii, I., Wandinger, U.

ATLID stands for "ATmospheric LIDar" and is the lidar to be flown on the Earth Clouds and Radiation Explorer (EarthCARE) platform in early 2019. ATLID is a High-Spectral Resolution (HSRL) system operating at 355nm. This presentation will introduce the ATLID level-2 retrieval algorithms being implemented in order to derive cloud and aerosol optical properties.

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Application of a multiple scattering model to estimate optical depth, lidar ratio and ice crystal effective radius of cirrus clouds observed with lidar.

2018, Gouveia, Diego, Baars, Holger, Seifert, Patric, Wandinger, Ulla, Barbosa, Henrique, Barja, Boris, Artaxo, Paulo, Lopes, Fabio, Landulfo, Eduardo, Ansmann, Albert, Nicolae, D., Makoto, A., Vassilis, A., Balis, D., Behrendt, A., Comeron, A., Gibert, F., Landulfo, E., McCormick, M.P., Senff, C., Veselovskii, I., Wandinger, U.

Lidar measurements of cirrus clouds are highly influenced by multiple scattering (MS). We therefore developed an iterative approach to correct elastic backscatter lidar signals for multiple scattering to obtain best estimates of single-scattering cloud optical depth and lidar ratio as well as of the ice crystal effective radius. The approach is based on the exploration of the effect of MS on the molecular backscatter signal returned from above cloud top.

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Target categorization of aerosol and clouds by continuous multiwavelength-polarization lidar measurements

2017, Baars, Holger, Seifert, Patric, Engelmann, Ronny, Wandinger, Ulla

Absolute calibrated signals at 532 and 1064 nm and the depolarization ratio from a multiwavelength lidar are used to categorize primary aerosol but also clouds in high temporal and spatial resolution. Automatically derived particle backscatter coefficient profiles in low temporal resolution (30 min) are applied to calibrate the lidar signals. From these calibrated lidar signals, new atmospheric parameters in temporally high resolution (quasi-particle-backscatter coefficients) are derived. By using thresholds obtained from multiyear, multisite EARLINET (European Aerosol Research Lidar Network) measurements, four aerosol classes (small; large, spherical; large, non-spherical; mixed, partly nonspherical) and several cloud classes (liquid, ice) are defined. Thus, particles are classified by their physical features (shape and size) instead of by source. The methodology is applied to 2 months of continuous observations (24 h a day, 7 days a week) with the multiwavelength-Raman-polarization lidar PollyXT during the High-Definition Clouds and Precipitation for advancing Climate Prediction (HD(CP)2) Observational Prototype Experiment (HOPE) in spring 2013. Cloudnet equipment was operated continuously directly next to the lidar and is used for comparison. By discussing three 24 h case studies, it is shown that the aerosol discrimination is very feasible and informative and gives a good complement to the Cloudnet target categorization. Performing the categorization for the 2-month data set of the entire HOPE campaign, almost 1 million pixel (5 min×30 m) could be analysed with the newly developed tool. We find that the majority of the aerosol trapped in the planetary boundary layer (PBL) was composed of small particles as expected for a heavily populated and industrialized area. Large, spherical aerosol was observed mostly at the top of the PBL and close to the identified cloud bases, indicating the importance of hygroscopic growth of the particles at high relative humidity. Interestingly, it is found that on several days non-spherical particles were dispersed from the ground into the atmosphere.

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EarthCARE Aerosol and Cloud Layer and Column Products

2018, Wandinger, Ulla, Hünerbein, Anja, Horn, Stefan, Schneider, Florian, Donovan, David, van Zadelhoff, Gerd-Jan, Daou, David, Docter, Nicole, Fischer, Jürgen, Filipitsch, Florian, Nicolae, D., Makoto, A., Vassilis, A., Balis, D., Behrendt, A., Comeron, A., Gibert, F., Landulfo, E., McCormick, M.P., Senff, C., Veselovskii, I., Wandinger, U.

We introduce the development of EarthCARE Level 2 layer products derived from profile measurements of the high-spectral-resolution lidar ATLID and column products obtained from combined information of ATLID and the Multi-Spectral Imager (MSI). Layer products include cloud top height as well as aerosol layer boundaries and mean optical properties along the satellite nadir track. Synergistic column products comprise cloud top height, Ångström exponent, and aerosol type both along-track and across the MSI swath.

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An automatic observation-based aerosol typing method for EARLINET

2018, Papagiannopoulos, Nikolaos, Mona, Lucia, Amodeo, Aldo, D'Amico, Giuseppe, Gumà Claramunt, Pilar, Pappalardo, Gelsomina, Alados-Arboledas, Lucas, Guerrero-Rascado, Juan Luís, Amiridis, Vassilis, Kokkalis, Panagiotis, Apituley, Arnoud, Baars, Holger, Schwarz, Anja, Wandinger, Ulla, Binietoglou, Ioannis, Nicolae, Doina, Bortoli, Daniele, Comerón, Adolfo, Rodríguez-Gómez, Alejandro, Sicard, Michaël, Papayannis, Alex, Wiegner, Matthias

We present an automatic aerosol classification method based solely on the European Aerosol Research Lidar Network (EARLINET) intensive optical parameters with the aim of building a network-wide classification tool that could provide near-real-time aerosol typing information. The presented method depends on a supervised learning technique and makes use of the Mahalanobis distance function that relates each unclassified measurement to a predefined aerosol type. As a first step (training phase), a reference dataset is set up consisting of already classified EARLINET data. Using this dataset, we defined 8 aerosol classes: clean continental, polluted continental, dust, mixed dust, polluted dust, mixed marine, smoke, and volcanic ash. The effect of the number of aerosol classes has been explored, as well as the optimal set of intensive parameters to separate different aerosol types. Furthermore, the algorithm is trained with literature particle linear depolarization ratio values. As a second step (testing phase), we apply the method to an already classified EARLINET dataset and analyze the results of the comparison to this classified dataset. The predictive accuracy of the automatic classification varies between 59% (minimum) and 90% (maximum) from 8 to 4 aerosol classes, respectively, when evaluated against pre-classified EARLINET lidar. This indicates the potential use of the automatic classification to all network lidar data. Furthermore, the training of the algorithm with particle linear depolarization values found in the literature further improves the accuracy with values for all the aerosol classes around 80%. Additionally, the algorithm has proven to be highly versatile as it adapts to changes in the size of the training dataset and the number of aerosol classes and classifying parameters. Finally, the low computational time and demand for resources make the algorithm extremely suitable for the implementation within the single calculus chain (SCC), the EARLINET centralized processing suite.

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Three-dimensional evolution of Saharan dust transport towards Europe based on a 9-year EARLINET-optimized CALIPSO dataset

2017, Marinou, Eleni, Amiridis, Vassilis, Binietoglou, Ioannis, Tsikerdekis, Athanasios, Solomos, Stavros, Proestakis, Emannouil, Konsta, Dimitra, Papagiannopoulos, Nikolaos, Tsekeri, Alexandra, Vlastou, Georgia, Zanis, Prodromos, Balis, Dimitrios, Wandinger, Ulla, Ansmann, Albert

In this study we use a new dust product developed using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) observations and EARLINET (European Aerosol Research Lidar Network) measurements and methods to provide a 3-D multiyear analysis on the evolution of Saharan dust over North Africa and Europe. The product uses a CALIPSO L2 backscatter product corrected with a depolarization-based method to separate pure dust in external aerosol mixtures and a Saharan dust lidar ratio (LR) based on long-term EARLINET measurements to calculate the dust extinction profiles. The methodology is applied on a 9-year CALIPSO dataset (2007-2015) and the results are analyzed here to reveal for the first time the 3-D dust evolution and the seasonal patterns of dust over its transportation paths from the Sahara towards the Mediterranean and Continental Europe. During spring, the spatial distribution of dust shows a uniform pattern over the Sahara desert. The dust transport over the Mediterranean Sea results in mean dust optical depth (DOD) values up to 0.1. During summer, the dust activity is mostly shifted to the western part of the desert where mean DOD near the source is up to 0.6. Elevated dust plumes with mean extinction values between 10 and 75 Mm-1 are observed throughout the year at various heights between 2 and 6 km, extending up to latitudes of 40° N. Dust advection is identified even at latitudes of about 60° N, but this is due to rare events of episodic nature. Dust plumes of high DOD are also observed above the Balkans during the winter period and above northwest Europe during autumn at heights between 2 and 4 km, reaching mean extinction values up to 50 Mm-1. The dataset is considered unique with respect to its potential applications, including the evaluation of dust transport models and the estimation of cloud condensation nuclei (CCN) and ice nuclei (IN) concentration profiles. Finally, the product can be used to study dust dynamics during transportation, since it is capable of revealing even fine dynamical features such as the particle uplifting and deposition on European mountainous ridges such as the Alps and Carpathian Mountains.

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Earlinet database: New design and new products for a wider use of aerosol lidar data

2018, Mona, Lucia, D’Amico, Giuseppe, Amato, Francesco, Linné, Holger, Baars, Holger, Wandinger, Ulla, Pappalardo, Gelsomina, Nicolae, D., Makoto, A., Vassilis, A., Balis, D., Behrendt, A., Comeron, A., Gibert, F., Landulfo, E., McCormick, M.P., Senff, C., Veselovskii, I., Wandinger, U.

The EARLINET database is facing a complete reshaping to meet the wide request for more intuitive products and to face the even wider request related to the new initiatives such as Copernicus, the European Earth observation programme. The new design has been carried out in continuity with the past, to take advantage from long-term database. In particular, the new structure will provide information suitable for synergy with other instruments, near real time (NRT) applications, validation and process studies and climate applications.

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Experimental techniques for the calibration of lidar depolarization channels in EARLINET

2018, Belegante, Livio, Bravo-Aranda, Juan Antonio, Freudenthaler, Volker, Nicolae, Doina, Nemuc, Anca, Ene, Dragos, Alados-Arboledas, Lucas, Amodeo, Aldo, Pappalardo, Gelsomina, D'Amico, Giuseppe, Amato, Francesco, Engelmann, Ronny, Baars, Holger, Wandinger, Ulla, Papayannis, Alexandros, Kokkalis, Panos, Pereira, Sérgio N.

Particle depolarization ratio retrieved from lidar measurements are commonly used for aerosol-typing studies, microphysical inversion, or mass concentration retrievals. The particle depolarization ratio is one of the primary parameters that can differentiate several major aerosol components but only if the measurements are accurate enough. The accuracy related to the retrieval of particle depolarization ratios is the driving factor for assessing and improving the uncertainties of the depolarization products. This paper presents different depolarization calibration procedures used to improve the quality of the depolarization data. The results illustrate a significant improvement of the depolarization lidar products for all the selected lidar stations that have implemented depolarization calibration procedures. The calibrated volume and particle depolarization profiles at 532-nm show values that fall within a range that is generally accepted in the literature.