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- ItemAerosol characteristics and particle production in the upper troposphere over the Amazon Basin(Katlenburg-Lindau : EGU, 2018) Andreae, Meinrat O.; Afchine, Armin; Albrecht, Rachel; Holanda, Bruna Amorim; Artaxo, Paulo; Barbosa, Henrique M. J.; Borrmann, Stephan; Cecchini, Micael A.; Costa, Anja; Dollner, Maximilian; Fütterer, Daniel; Järvinen, Emma; Jurkat, Tina; Klimach, Thomas; Konemann, Tobias; Knote, Christoph; Krämer, Martina; Krisna, Trismono; Machado, Luiz A. T.; Mertes, Stephan; Minikin, Andreas; Pöhlker, Christopher; Pöhlker, Mira L.; Pöschl, Ulrich; Rosenfeld, Daniel; Sauer, Daniel; Schlager, Hans; Schnaiter, Martin; Schneider, Johannes; Schulz, Christiane; Spanu, Antonio; Sperling, Vinicius B.; Voigt, Christiane; Walser, Adrian; Wang, Jian; Weinzierl, Bernadett; Wendisch, Manfred; Ziereis, HelmutAirborne observations over the Amazon Basin showed high aerosol particle concentrations in the upper troposphere (UT) between 8 and 15ĝ€km altitude, with number densities (normalized to standard temperature and pressure) often exceeding those in the planetary boundary layer (PBL) by 1 or 2 orders of magnitude. The measurements were made during the German–Brazilian cooperative aircraft campaign ACRIDICON–CHUVA, where ACRIDICON stands for
Aerosol, Cloud, Precipitation, and Radiation Interactions and Dynamics of Convective Cloud Systems
and CHUVA is the acronym forCloud Processes of the Main Precipitation Systems in Brazil: A Contribution to Cloud Resolving Modeling and to the GPM (global precipitation measurement)
, on the German High Altitude and Long Range Research Aircraft (HALO). The campaign took place in September–October 2014, with the objective of studying tropical deep convective clouds over the Amazon rainforest and their interactions with atmospheric trace gases, aerosol particles, and atmospheric radiation.
Aerosol enhancements were observed consistently on all flights during which the UT was probed, using several aerosol metrics, including condensation nuclei (CN) and cloud condensation nuclei (CCN) number concentrations and chemical species mass concentrations. The UT particles differed sharply in their chemical composition and size distribution from those in the PBL, ruling out convective transport of combustion-derived particles from the boundary layer (BL) as a source. The air in the immediate outflow of deep convective clouds was depleted of aerosol particles, whereas strongly enhanced number concentrations of small particles (< 90ĝ€nm diameter) were found in UT regions that had experienced outflow from deep convection in the preceding 5–72ĝ€h. We also found elevated concentrations of larger (> 90ĝ€nm) particles in the UT, which consisted mostly of organic matter and nitrate and were very effective CCN.
Our findings suggest a conceptual model, where production of new aerosol particles takes place in the continental UT from biogenic volatile organic material brought up by deep convection and converted to condensable species in the UT. Subsequently, downward mixing and transport of upper tropospheric aerosol can be a source of particles to the PBL, where they increase in size by the condensation of biogenic volatile organic compound (BVOC) oxidation products. This may be an important source of aerosol particles for the Amazonian PBL, where aerosol nucleation and new particle formation have not been observed. We propose that this may have been the dominant process supplying secondary aerosol particles in the pristine atmosphere, making clouds the dominant control of both removal and production of atmospheric particles. - ItemValidation of an improved batch model in a coupled combustion space/melt tank/batch melting glass fumace simulation(Offenbach : Verlag der Deutschen Glastechnischen Gesellschaft, 2000) Wang, Jian; Brewster, B. Scott; McQuay, Mardson Q.; Webb, Brent W.An improved coupled combustion space model, model for the transport processes in the melting tank, and batch blanket melting model has been developed which is capable of predicting the transport phenomena in a float glass furnace. Model predictions are compared with experimental furnace measurements reported previously. The batch blanket has been approximated as continuous and discrete (island) regions in an attempt to simulate the formation of discrete batch clumps ("logs") observed in real furnaces. Both the boundary location between the continuous blanket and batch island zones, and the batch coverage fraction in the batch island zone are specified as model inputs. The heat fluxes and temperatures at the interfaces between the combustion space, the batch coverage, and the glass tank are calculated in a coupled fashion rather than assumed as input boundary conditions as it must be done in traditional, uncoupled models. Α 455-metric-ton pull rate per day, air-fuel fired float-glass melting furnace was simulated. The 100 % batch blanket simulation (absence of batch islands) yields over-prediction of glass surface temperature, crown incident heat flux, and crown temperature. The assumption of 85 % batch coverage and 15 % free glass surface in the batch island zone agrees well with most experimental measurements. The batch island concept added to the batch melting model is a significant improvement over previous approaches for this case.
- ItemPredicted and measured glass surface temperatures in an industrial, regeneratively gas-fired flat glass furnace(Offenbach : Verlag der Deutschen Glastechnischen Gesellschaft, 1999) Hayes, R. Robert; Wang, Jian; McQuay, Mardson Q.; Webb, Brent W.; Huber, Aaron M.This study reports optically measured glass surface temperatures along the furnace center-line in the combustion space of a sideport, 455 (metric) t/d industrial, gas-fired flat glass furnace. The measurements were made using a water-cooled two-color pyrometer inserted through holes in the crown at six locations along the length of the furnace. Both average and time-resolved glass surface temperature measurements were performed during the approximately 20 s reversal period of the furnace. The measured glass surface temperature data are supplemented by observations of the batch location using a specially designed, water-cooled video probe. The average temperatures were found to rise from a low near 1700 Κ near the batch blanket to a peak of approximately 1900 K, then drop to a level of 1800 K. Evidence of batch Islands or "logs" is observed in the surface temperature data collected at the measurement location nearest the batch blanket. Large temperature excursions are seen here, indicative of measurement alternately of both the batch surface and the molten glass. Also reported in this study are results of a numerical model for the three-dimensional melt flow and heat transfer in the tank, coupled with a batch melting model. The radiant heat flux distribution incident on the melt and batch blanket surfaces is assumed. The melt tank model includes bubbling. The numerical predictions agree well with the timeaveraged glass surface temperature data collected experimentally The measurements and model predictions illustrate the complex transport phenomena in the melting section of the furnace.
- ItemPlastic Deformation Modes of CuZr/Cu Multilayers([London] : Macmillan Publishers Limited, part of Springer Nature, 2016) Cui, Yan; Abad, Oscar Torrents; Wang, Fei; Huang, Ping; Lu, Tian-Jian; Xu, Ke-Wei; Wang, JianWe synthesized CuZr/Cu multilayers and performed nanoindentation testing to explore the dependence of plastic deformation modes on the thickness of CuZr layers. The Cu layers were 18 nm thick and the CuZr layers varied in thickness from 4 nm to 100 nm. We observed continuous plastic co-deformation in the 4 nm and 10 nm CuZr − 18 nm Cu multilayers and plastic-induced shear instability in thick CuZr layers (>20 nm). The plastic co-deformation is ascribed to the nucleation and interaction of shear transformation zones in CuZr layers at the adjacent interfaces, while the shear instability is associated with the nucleation and propagation of shear bands in CuZr layers. Shear bands are initialized in the CuZr layers due to the accumulated glide dislocations along CuZr-Cu interfaces and propagate into adjacent Cu layers via slips on {111} plane non-parallel to the interface. Due to crystallographic constraint of the Cu layers, shear bands are approximately parallel to {111} plane in the Cu layer.