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- ItemAtmospheric dust modeling from meso to global scales with the online NMMB/BSC-Dust model – Part 2: Experimental campaigns in Northern Africa(München : European Geopyhsical Union, 2012) Haustein, K.; Pérez, C.; Baldasano, J.M.; Jorba, O.; Basart, S.; Miller, R.L.; Janjic, Z.; Black, T.; Nickovic, S.; Todd, M.C.; Washington, R.; Müller, D.; Tesche, M.; Weinzierl, B.; Esselborn, M.; Schladitz, A.The new NMMB/BSC-Dust model is intended to provide short to medium-range weather and dust forecasts from regional to global scales. It is an online model in which the dust aerosol dynamics and physics are solved at each model time step. The companion paper (Pérez et al., 2011) develops the dust model parameterizations and provides daily to annual evaluations of the model for its global and regional configurations. Modeled aerosol optical depth (AOD) was evaluated against AERONET Sun photometers over Northern Africa, Middle East and Europe with correlations around 0.6–0.7 on average without dust data assimilation. In this paper we analyze in detail the behavior of the model using data from the Saharan Mineral dUst experiment (SAMUM-1) in 2006 and the Bodélé Dust Experiment (BoDEx) in 2005. AOD from satellites and Sun photometers, vertically resolved extinction coefficients from lidars and particle size distributions at the ground and in the troposphere are used, complemented by wind profile data and surface meteorological measurements. All simulations were performed at the regional scale for the Northern African domain at the expected operational horizontal resolution of 25 km. Model results for SAMUM-1 generally show good agreement with satellite data over the most active Saharan dust sources. The model reproduces the AOD from Sun photometers close to sources and after long-range transport, and the dust size spectra at different height levels. At this resolution, the model is not able to reproduce a large haboob that occurred during the campaign. Some deficiencies are found concerning the vertical dust distribution related to the representation of the mixing height in the atmospheric part of the model. For the BoDEx episode, we found the diurnal temperature cycle to be strongly dependant on the soil moisture, which is underestimated in the NCEP analysis used for model initialization. The low level jet (LLJ) and the dust AOD over the Bodélé are well reproduced. The remaining negative AOD bias (due to underestimated surface wind speeds) can be substantially reduced by decreasing the threshold friction velocity in the model.
- ItemOptimizing CALIPSO Saharan dust retrievals(München : European Geopyhsical Union, 2013) Amiridis, V.; Wandinger, U.; Marinou, E.; Giannakaki, E.; Tsekeri, A.; Basart, S.; Kazadzis, S.; Gkikas, A.; Taylor, M.; Baldasano, J.; Ansmann, A.We demonstrate improvements in CALIPSO (Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations) dust extinction retrievals over northern Africa and Europe when corrections are applied regarding the Saharan dust lidar ratio assumption, the separation of the dust portion in detected dust mixtures, and the averaging scheme introduced in the Level 3 CALIPSO product. First, a universal, spatially constant lidar ratio of 58 sr instead of 40 sr is applied to individual Level 2 dust-related backscatter products. The resulting aerosol optical depths show an improvement compared with synchronous and collocated AERONET (Aerosol Robotic Network) measurements. An absolute bias of the order of −0.03 has been found, improving on the statistically significant biases of the order of −0.10 reported in the literature for the original CALIPSO product. When compared with the MODIS (Moderate-Resolution Imaging Spectroradiometer) collocated aerosol optical depth (AOD) product, the CALIPSO negative bias is even less for the lidar ratio of 58 sr. After introducing the new lidar ratio for the domain studied, we examine potential improvements to the climatological CALIPSO Level 3 extinction product: (1) by introducing a new methodology for the calculation of pure dust extinction from dust mixtures and (2) by applying an averaging scheme that includes zero extinction values for the nondust aerosol types detected. The scheme is applied at a horizontal spatial resolution of 1° × 1° for ease of comparison with the instantaneous and collocated dust extinction profiles simulated by the BSC-DREAM8b dust model. Comparisons show that the extinction profiles retrieved with the proposed methodology reproduce the well-known model biases per subregion examined. The very good agreement of the proposed CALIPSO extinction product with respect to AERONET, MODIS and the BSC-DREAM8b dust model makes this dataset an ideal candidate for the provision of an accurate and robust multiyear dust climatology over northern Africa and Europe.
- ItemSaharan dust contribution to the Caribbean summertime boundary layer - A lidar study during SALTRACE(München : European Geopyhsical Union, 2016) Groß, Silke; Gasteiger, Josef; Freudenthaler, Volker; Müller, Thomas; Sauer, Daniel; Toledano, Carlos; Ansmann, AlbertDual-wavelength lidar measurements with the small lidar system POLIS of the Ludwig-Maximilians-Universität München were performed during the SALTRACE experiment at Barbados in June and July 2013. Based on high-accuracy measurements of the linear depolarization ratio down to about 200 m above ground level, the dust volume fraction and the dust mass concentration within the convective marine boundary layer can be derived. Additional information from radiosonde launches at the ground-based measurement site provide independent information on the convective marine boundary layer height and the meteorological situation within the convective marine boundary layer. We investigate the lidar-derived optical properties, the lidar ratio and the particle linear depolarization ratio at 355 and 532 nm and find mean values of 0.04 (SD 0.03) and 0.05 (SD 0.04) at 355 and 532 nm, respectively, for the particle linear depolarization ratio, and (26 ± 5) sr for the lidar ratio at 355 and 532 nm. For the concentration of dust in the convective marine boundary layer we find that most values were between 20 and 50 µgm−3. On most days the dust contribution to total aerosol volume was about 30–40 %. Comparing the dust contribution to the column-integrated sun-photometer measurements we see a correlation between high dust contribution, high total aerosol optical depth and a low Angström exponent, and of low dust contribution with low total aerosol optical depth.
- ItemOptical properties of long-range transported Saharan dust over Barbados as measured by dual-wavelength depolarization Raman lidar measurements(München : European Geopyhsical Union, 2015) Groß, S.; Freudenthaler, V.; Schepanski, K.; Toledano, C.; Schäfler, A.; Ansmann, A.; Weinzierl, B.Dual-wavelength Raman and depolarization lidar observations were performed during the Saharan Aerosol Long-range Transport and Aerosol-Cloud interaction Experiment in Barbados in June and July 2013 to characterize the optical properties and vertical distribution of long-range transported Saharan dust after transport across the Atlantic Ocean. Four major dust events were studied during the measurements from 15 June to 13 July 2013 with aerosol optical depths at 532 nm of up to 0.6. The vertical aerosol distribution was characterized by a three-layer structure consisting of the boundary layer, the entrainment or mixing layer and the pure Saharan dust layer. The upper boundary of the pure dust layer reached up to 4.5 km in height. The contribution of the pure dust layer was about half of the total aerosol optical depth at 532 nm. The total dust contribution was about 50–70 % of the total aerosol optical depth at 532 nm. The lidar ratio within the pure dust layer was found to be wavelength independent with mean values of 53 ± 5 sr at 355 nm and 56 ± 7 sr at 532 nm. For the particle linear depolarization ratio, wavelength-independent mean values of 0.26 ± 0.03 at 355 nm and 0.27 ± 0.01 at 532 nm have been found.
- ItemNew developments in the representation of Saharan dust sources in the aerosol-climate model ECHAM6-HAM2(München : European Geopyhsical Union, 2016) Heinold, Bernd; Tegen, Ina; Schepanski, Kerstin; Banks, Jamie R.In the aerosol-climate model ECHAM6-HAM2, dust source activation (DSA) observations from Meteosat Second Generation (MSG) satellite are proposed to replace the original source area parameterization over the Sahara Desert. The new setup is tested in nudged simulations for the period 2007 to 2008. The evaluation is based on comparisons to dust emission events inferred from MSG dust index imagery, Aerosol Robotic Network (AERONET) sun photometer observations, and satellite retrievals of aerosol optical thickness (AOT). The model results agree well with AERONET measurements especially in terms of seasonal variability, and a good spatial correlation was found between model results and MSG-SEVIRI (Spinning-Enhanced Visible and InfraRed Imager) dust AOT as well as Multi-angle Imaging SpectroRadiometer (MISR) AOT. ECHAM6-HAM2 computes a more realistic geographical distribution and up to 20 % higher annual Saharan dust emissions, using the MSG-based source map. The representation of dust AOT is partly improved in the southern Sahara and Sahel. In addition, the spatial variability is increased towards a better agreement with observations depending on the season. Thus, using the MSG DSA map can help to circumvent the issue of uncertain soil input parameters. An important issue remains the need to improve the model representation of moist convection and stable nighttime conditions. Compared to sub-daily DSA information from MSG-SEVIRI and results from a regional model, ECHAM6-HAM2 notably underestimates the important fraction of morning dust events by the breakdown of the nocturnal low-level jet, while a major contribution is from afternoon-to-evening emissions.
- ItemDesert dust aerosol air mass mapping in the western Sahara, using particle properties derived from space-based multi-angle imaging(Milton Park : Taylor & Francis, 2017) Kahn, Ralph; Petzold, Andreas; Wendisch, Manfred; Bierwirth, Eike; Dinter, Tilman; Esselborn, Michael; Fiebig, Marcus; Heese, Birgit; Knippertz, Peter; Müller, Detlef; Schladitz, Alexander; Von Hoyningen-HUENE, WolfgangCoincident observations made over the Moroccan desert during the Sahara mineral dust experiment (SAMUM) 2006 field campaign are used both to validate aerosol amount and type retrieved from multi-angle imaging spectroradiometer (MISR) observations, and to place the suborbital aerosol measurements into the satellite’s larger regional context. On three moderately dusty days during which coincident observations were made, MISR mid-visible aerosol optical thickness (AOT) agrees with field measurements point-by-point to within 0.05–0.1. This is about as well as can be expected given spatial sampling differences; the space-based observations capture AOT trends and variability over an extended region. The field data also validate MISR’s ability to distinguish and to map aerosol air masses, from the combination of retrieved constraints on particle size, shape and single-scattering albedo. For the three study days, the satellite observations (1) highlight regional gradients in the mix of dust and background spherical particles, (2) identify a dust plume most likely part of a density flow and (3) show an aerosol air mass containing a higher proportion of small, spherical particles than the surroundings, that appears to be aerosol pollution transported from several thousand kilometres away.
- ItemDepolarization ratio profiling at several wavelengths in pure Saharan dust during SAMUM 2006(Milton Park : Taylor & Francis, 2017) Freudenthaler, Volker; Esselborn, Michael; Wiegner, Matthias; Heese, Birgit; Tesche, Matthias; Ansmann, Albert; Müller, Detlef; Althausen, Dietrich; Wirth, Martin; Fix, Andreas; Ehret, Gerhard; Knippertz, Peter; Toledano, Carlos; Gasteiger, Josef; Garhammer, Markus; Seefeldner, MeinhardVertical profiles of the linear particle depolarization ratio of pure dust clouds were measured during the Saharan Mineral Dust Experiment (SAMUM) at Ouarzazate, Morocco (30.9◦N, –6.9◦E), close to source regions in May–June 2006, with four lidar systems at four wavelengths (355, 532, 710 and 1064 nm). The intercomparison of the lidar systems is accompanied by a discussion of the different calibration methods, including a new, advanced method, and a detailed error analysis. Over the whole SAMUM periode pure dust layers show a mean linear particle depolarization ratio at 532 nm of 0.31, in the range between 0.27 and 0.35, with a mean Ångström exponent (AE, 440–870 nm) of 0.18 (range 0.04–0.34) and still high mean linear particle depolarization ratio between 0.21 and 0.25 during periods with aerosol optical thickness less than 0.1, with a mean AE of 0.76 (range 0.65–1.00), which represents a negative correlation of the linear particle depolarization ratio with the AE. A slight decrease of the linear particle depolarization ratio with wavelength was found between 532 and 1064 nm from 0.31 ± 0.03 to 0.27 ± 0.04.
- ItemAirborne spectral radiation measurements to derive solar radiative forcing of Saharan dust mixed with biomass burning smoke particles(Milton Park : Taylor & Francis, 2017) Bauer, S.; Bierwirth, E.; Esselborn, M.; Petzold, A.; Macke, A.; Trautmann, T.; Wendisch, M.Airborne measurements of upward solar spectral irradiances were performed during the second Saharan Mineral dUst experiMent (SAMUM-2) campaign based on the Cape Verde Islands. Additionally, airborne high resolution lidar measurements of vertical profiles of particle extinction coefficients were collected in parallel to the radiation data. Aerosol layers of Saharan dust, partly mixed with biomass-burning smoke, were probed. With corresponding radiative transfer simulations the single scattering albedo and the asymmetry parameter of the aerosol particles were derived although with high uncertainty. The broad-band aerosol solar radiative forcing at the top of atmosphere was calculated and examined as a function of the aerosol types. However, due to uncertainties in both the measurements and the calculations the chemical composition cannot be identified. In addition, a mostly measurement-based method to derive the broad-band aerosol solar radiative forcing was used. This approach revealed clear differences of broad-band net irradiances as a function of the aerosol optical depth. The data were used to identify different aerosol types from different origins. Higher portions of biomass-burning smoke lead to larger broad-band net irradiances.
- ItemEvaluation of long-range transport and deposition of desert dust with the CTM MOCAGE(Milton Park : Taylor & Francis, 2017) Martet, M.; Peuch, V-H.; Laurent, B.; Marticorena, B.; Bergametti, G.Desert dust modelling and forecasting attract growing interest, due to the numerous impacts of dusts on climate, numerical weather prediction, health, ecosystems, transportation, as well as on many industrial activities. The validation of numerical tools is a very important activity in this context, and we present here an example of such an effort, combining in situ (horizontal visibility in SYNOP messages, IMPROVE database) and remote-sensing data (satellite imagery, AERONET aerosol optical thickness data). Interestingly, these measurements are available routinely, and not only in the context of dedicated measurements campaign; thus, they can be used in an operational context to monitor the performances of operational forecasting systems. MOCAGE is the chemistry-transport model of Météo-France, used operationally to forecast the three-dimensional transport of dusts and their deposition. Two very long-range transport episodes of dust have been studied: one case of Saharan dust transported to East America through Asia and Pacific observed in November 2004 and one case of Saharan dust transported from West Africa to Caribbean Islands in May 2007. Episodes of geographical extension had seldom been studied, and they provide a very selective reference to compare the modelled desert dusts with. The representation of dusts in MOCAGE appears to be realistic in these two very different cases. In turn, the model simulations are used to make the link between the complementary information provided by the different measurements tools, providing a fully consistent picture of the entire episodes. The evolution of the aerosol size distribution during the episodes has also been studied. With no surprise, our study underlines that deposition processes are very sensitive to the size of dust particles. If the atmospheric cycle, in terms of mass, is very much under the influence of larger particles (some micrometres and above), only the finer particles actually travel over thousands of kilometres. This illustrates the need for an accurate representation of size distributions for this aerosol component in numerical models and advocates for using a size-resolved (bin) approach as sinks, and particularly, deposition do not affect the emitted log-normal distributions symmetrically on both sides of the median diameter. Overall, the results presented in this study provide an evaluation of Météo-France operational dust forecasting system MOCAGE.
- ItemEARLINET observations of the 14-22-May long-range dust transport event during SAMUM 2006: Validation of results from dust transport modelling(Milton Park : Taylor & Francis, 2017) Müller, D.; Heinold, B.; Tesche, M.; Tegen, I.; Althausen, D.; Alados Arboledas, L.; Amiridis, V.; Amodeo, A.; Ansmann, A.; Balis, D.; Comeron, A.; D’mico, G.; Gerasopoulos, E.; Guerrero-Rascado, J.L.; Freudenthaler, V.; Giannakaki, E.; Heese, B.; Iarlori, M.; Knippertz, P.; Mamouri, R.E.; Mona, L.; Papayannis, A.; Pappalardo, G.; Perrone, R-M.; Pisani, G.; Rizi, V.; Sicard, M.; Spinelli, N.; Tafuro, A.; Wiegner, M.We observed a long-range transport event of mineral dust from North Africa to South Europe during the Saharan Mineral Dust Experiment (SAMUM) 2006. Geometrical and optical properties of that dust plume were determined with Sun photometer of the Aerosol Robotic Network (AERONET) and Raman lidar near the North African source region, and with Sun photometers of AERONET and lidars of the European Aerosol Research Lidar Network (EARLINET) in the far field in Europe. Extinction-to-backscatter ratios of the dust plume over Morocco and Southern Europe do not differ. Ångstr¨om exponents increase with distance from Morocco. We simulated the transport, and geometrical and optical properties of the dust plume with a dust transport model. The model results and the experimental data show similar times regarding the appearance of the dust plume over each EARLINET site. Dust optical depth from the model agrees in most cases to particle optical depth measured with the Sun photometers. The vertical distribution of the mineral dust could be satisfactorily reproduced, if we use as benchmark the extinction profiles measured with lidar. In some cases we find differences. We assume that insufficient vertical resolution of the dust plume in the model calculations is one reason for these deviations.