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The automated multiwavelength Raman polarization and water-vapor lidar PollyXT: The neXT generation

2016, Engelmann, Ronny, Kanitz, Thomas, Baars, Holger, Heese, Birgit, Althausen, Dietrich, Skupin, Annett, Wandinger, Ulla, Komppula, Mika, Stachlewska, Iwona S., Amiridis, Vassilis, Marinou, Eleni, Mattis, Ina, Linné, Holger, Ansmann, Albert

The atmospheric science community demands autonomous and quality-assured vertically resolved measurements of aerosol and cloud properties. For this purpose, a portable lidar called Polly was developed at TROPOS in 2003. The lidar system was continuously improved with gained experience from the EARLINET community, involvement in worldwide field campaigns, and international institute collaborations within the last 10 years. Here we present recent changes of the setup of the portable multiwavelength Raman and polarization lidar PollyXT and discuss the improved capabilities of the system by means of a case study. The latest system developments include an additional near-range receiver unit for Raman measurements of the backscatter and extinction coefficient down to 120 m above ground, a water-vapor channel, and channels for simultaneous measurements of the particle linear depolarization ratio at 355 and 532 nm. Quality improvements were achieved by systematically following the EARLINET guidelines and the international PollyNET quality assurance developments. A modified ship radar ensures measurements in agreement with air-traffic safety regulations and allows for 24∕7 monitoring of the atmospheric state with PollyXT.

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Technical Note: One year of Raman-lidar measurements in Gual Pahari EUCAARI site close to New Delhi in India – Seasonal characteristics of the aerosol vertical structure

2012, Komppula, M., Mielonen, T., Arola, A., Korhonen, K., Lihavainen, H., Hyvärinen, A.-P., Baars, H., Engelmann, R., Althausen, D., Ansmann, A., Müller, D., Panwar, T.S., Hooda, R.K., Sharma, V.P., Kerminen, V.-M., Lehtinen, K.E.J., Viisanen, Y.

One year of multi-wavelength (3 backscatter + 2 extinction + 1 depolarization) Raman lidar measurements at Gual Pahari, close to New Delhi, were analysed. The data was split into four seasons: spring (March–May), summer (June–August), autumn (September–November) and winter (December–February). The vertical profiles of backscatter, extinction, and lidar ratio and their variability during each season are presented. The measurements revealed that, on average, the aerosol layer was at its highest in spring (5.5 km). In summer, the vertically averaged (between 1–3 km) backscatter and extinction coefficients had the highest averages (3.3 Mm−1 sr−1 and 142 Mm−1 at 532 nm, respectively). Aerosol concentrations were slightly higher in summer compared to other seasons, and particles were larger in size. The autumn showed the highest lidar ratio and high extinction-related Ångström exponents (AEext), indicating the presence of smaller probably absorbing particles. The winter had the lowest backscatter and extinction coefficients, but AEext was the highest, suggesting still a large amount of small particles.

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Potential of polarization/Raman lidar to separate fine dust, coarse dust, maritime, and anthropogenic aerosol profiles

2017, Mamouri, Rodanthi-Elisavet, Ansmann, Albert

We applied the recently introduced polarization lidar–photometer networking (POLIPHON) technique for the first time to triple-wavelength polarization lidar measurements at 355, 532, and 1064 nm. The lidar observations were performed at Barbados during the Saharan Aerosol Long-Range Transport and Aerosol-Cloud-Interaction Experiment (SALTRACE) in the summer of 2014. The POLIPHON method comprises the traditional lidar technique to separate mineral dust and non-dust backscatter contributions and the new, extended approach to separate even the fine and coarse dust backscatter fractions. We show that the traditional and the advanced method are compatible and lead to a consistent set of dust and non-dust profiles at simplified, less complex aerosol layering and mixing conditions as is the case over the remote tropical Atlantic. To derive dust mass concentration profiles from the lidar observations, trustworthy extinction-to-volume conversion factors for fine, coarse, and total dust are needed and obtained from an updated, extended Aerosol Robotic Network sun photometer data analysis of the correlation between the fine, coarse and total dust volume concentration and the respective fine, coarse, and total dust extinction coefficient for all three laser wavelengths. Conversion factors (total volume to extinction) for pure marine aerosol conditions and continental anthropogenic aerosol situations are presented in addition. As a new feature of the POLIPHON data analysis, the Raman lidar method for particle extinction profiling is used to identify the aerosol type (marine or anthropogenic) of the non-dust aerosol fraction. The full POLIPHON methodology was successfully applied to a SALTRACE case and the results are discussed. We conclude that the 532 nm polarization lidar technique has many advantages in comparison to 355 and 1064 nm polarization lidar approaches and leads to the most robust and accurate POLIPHON products.

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Optical and microphysical properties of smoke over Cape Verde inferred from multiwavelength lidar measurements

2017, Tesche, Matthias, Müller, Detlef, Gross, Silke, Ansmann, Albert, Althausen, Dietrich, Freudenthaler, Volker, Weinzierl, Bernadett, Veira, Andreas, Petzold, Andreas

Lidar measurements of mixed dust/smoke plumes over the tropical Atlantic ocean were carried out during the winter campaign of SAMUM-2 at Cape Verde. Profiles of backscatter and extinction coefficients, lidar ratios, and Ångstr¨om exponents related to pure biomass-burning aerosol from southern West Africa were extracted from these observations. Furthermore, these findings were used as input for an inversion algorithm to retrieve microphysical properties of pure smoke. Seven measurement days were found suitable for the procedure of aerosol-type separation and successive inversion of optical data that describe biomass-burning smoke. We inferred high smoke lidar ratios of 87 ± 17 sr at 355 nm and 79 ± 17 sr at 532 nm. Smoke lidar ratios and Ångstr¨om exponents are higher compared to the ones for the dust/smoke mixture. These numbers indicate higher absorption and smaller sizes for pure smoke particles compared to the dust/smoke mixture. Inversion of the smoke data set results in mean effective radii of 0.22 ± 0.08 μm with individual results varying between 0.10 and 0.36 μm. The single-scattering albedo for pure biomass-burning smoke was found to vary between 0.63 and 0.89 with a very low mean value of 0.75 ± 0.07. This is in good agreement with findings of airborne in situ measurements which showed values of 0.77 ± 0.03. Effective radii from the inversion were similar to the ones found for the fine mode of the in situ size distributions.

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EARLINET Single Calculus Chain – overview on methodology and strategy

2015, D'Amico, Giuseppe, Amodeo, A., Baars, H., Binietoglou, I., Freudenthaler, V., Mattis, I., Wandinger, U., Pappalardo, G.

In this paper we describe the EARLINET Single Calculus Chain (SCC), a tool for the automatic analysis of lidar measurements. The development of this tool started in the framework of EARLINET-ASOS (European Aerosol Research Lidar Network – Advanced Sustainable Observation System); it was extended within ACTRIS (Aerosol, Clouds and Trace gases Research InfraStructure Network), and it is continuing within ACTRIS-2. The main idea was to develop a data processing chain that allows all EARLINET stations to retrieve, in a fully automatic way, the aerosol backscatter and extinction profiles starting from the raw lidar data of the lidar systems they operate. The calculus subsystem of the SCC is composed of two modules: a pre-processor module which handles the raw lidar data and corrects them for instrumental effects and an optical processing module for the retrieval of aerosol optical products from the pre-processed data. All input parameters needed to perform the lidar analysis are stored in a database to keep track of all changes which may occur for any EARLINET lidar system over the time. The two calculus modules are coordinated and synchronized by an additional module (daemon) which makes the whole analysis process fully automatic. The end user can interact with the SCC via a user-friendly web interface. All SCC modules are developed using open-source and freely available software packages. The final products retrieved by the SCC fulfill all requirements of the EARLINET quality assurance programs on both instrumental and algorithm levels. Moreover, the manpower needed to provide aerosol optical products is greatly reduced and thus the near-real-time availability of lidar data is improved. The high-quality of the SCC products is proven by the good agreement between the SCC analysis, and the corresponding independent manual retrievals. Finally, the ability of the SCC to provide high-quality aerosol optical products is demonstrated for an EARLINET intense observation period.

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Studying the vertical aerosol extinction coefficient by comparing in situ airborne data and elastic backscatter lidar

2016, Rosati, Bernadette, Herrmann, Erik, Bucci, Silvia, Fierli, Federico, Cairo, Francesco, Gysel, Martin, Tillmann, Ralf, Größ, Johannes, Gobbi, Gian Paolo, Liberto, Luca Di, Di Donfrancesco, Guido, Wiedensohler, Alfred, Weingartner, Ernest, Virtanen, Annele, Mentel, Thomas F., Baltensperger, Urs

Vertical profiles of aerosol particle optical properties were explored in a case study near the San Pietro Capofiume (SPC) ground station during the PEGASOS Po Valley campaign in the summer of 2012. A Zeppelin NT airship was employed to investigate the effect of the dynamics of the planetary boundary layer at altitudes between ∼  50 and 800 m above ground. Determined properties included the aerosol particle size distribution, the hygroscopic growth factor, the effective index of refraction and the light absorption coefficient. The first three parameters were used to retrieve the light scattering coefficient. Simultaneously, direct measurements of both the scattering and absorption coefficient were carried out at the SPC ground station. Additionally, a single wavelength polarization diversity elastic lidar system provided estimates of aerosol extinction coefficients using the Klett method to accomplish the inversion of the signal, for a vertically resolved comparison between in situ and remote-sensing results. Note, however, that the comparison was for the most part done in the altitude range where the overlap function is incomplete and accordingly uncertainties are larger. First, the airborne results at low altitudes were validated with the ground measurements. Agreement within approximately ±25 and ±20 % was found for the dry scattering and absorption coefficient, respectively. The single scattering albedo, ranged between 0.83 and 0.95, indicating the importance of the absorbing particles in the Po Valley region. A clear layering of the atmosphere was observed during the beginning of the flight (until ∼  10:00 LT – local time) before the mixing layer (ML) was fully developed. Highest extinction coefficients were found at low altitudes, in the new ML, while values in the residual layer, which could be probed at the beginning of the flight at elevated altitudes, were lower. At the end of the flight (after ∼  12:00 LT) the ML was fully developed, resulting in constant extinction coefficients at all altitudes measured on the Zeppelin NT. Lidar estimates captured these dynamic features well and good agreement was found for the extinction coefficients compared to the in situ results, using fixed lidar ratios (LR) between 30 and 70 sr for the altitudes probed with the Zeppelin. These LR are consistent with values for continental aerosol particles that can be expected in this region.

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Simultaneous and co-located wind measurements in the middle atmosphere by lidar and rocket-borne techniques

2016, Lübken, Franz-Josef, Baumgarten, Gerd, Hildebrand, Jens, Schmidlin, Francis J.

We present the first comparison of a new lidar technique to measure winds in the middle atmosphere, called DoRIS (Doppler Rayleigh Iodine Spectrometer), with a rocket-borne in situ method, which relies on measuring the horizontal drift of a target (“starute”) by a tracking radar. The launches took place from the Andøya Space Center (ASC), very close to the ALOMAR observatory (Arctic Lidar Observatory for Middle Atmosphere Research) at 69° N. DoRIS is part of a steerable twin lidar system installed at ALOMAR. The observations were made simultaneously and with a horizontal distance between the two lidar beams and the starute trajectories of typically 0–40 km only. DoRIS measured winds from 14 March 2015, 17:00 UTC, to 15 March 2015, 11:30 UTC. A total of eight starute flights were launched successfully from 14 March, 19:00 UTC, to 15 March, 00:19 UTC. In general there is excellent agreement between DoRIS and the in situ measurements, considering the combined range of uncertainties. This concerns not only the general height structures of zonal and meridional winds and their temporal developments, but also some wavy structures. Considering the comparison between all starute flights and all DoRIS observations in a time period of ±20 min around each individual starute flight, we arrive at mean differences of typically ±5–10 m s−1 for both wind components. Part of the remaining differences are most likely due to the detection of different wave fronts of gravity waves. There is no systematic difference between DoRIS and the in situ observations above 30 km. Below ∼ 30 km, winds from DoRIS are systematically too large by up to 10–20 m s−1, which can be explained by the presence of aerosols. This is proven by deriving the backscatter ratios at two different wavelengths. These ratios are larger than unity, which is an indication of the presence of aerosols.

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EARLINET instrument intercomparison campaigns: Overview on strategy and results

2016, Wandinger, Ulla, Freudenthaler, Volker, Baars, Holger, Amodeo, Aldo, Engelmann, Ronny, Mattis, Ina, Groß, Silke, Pappalardo, Gelsomina, Giunta, Aldo, D'Amico, Giuseppe, Chaikovsky, Anatoli, Osipenko, Fiodor, Slesar, Alexander, Nicolae, Doina, Belegante, Livio, Talianu, Camelia, Serikov, Ilya, Linné, Holger, Jansen, Friedhelm, Apituley, Arnoud, Wilson, Keith M., de Graaf, Martin, Trickl, Thomas, Giehl, Helmut, Adam, Mariana, Comerón, Adolfo, Muñoz-Porcar, Constantino, Rocadenbosch, Francesc, Sicard, Michaël, Tomás, Sergio, Lange, Diego, Kumar, Dhiraj, Pujadas, Manuel, Molero, Francisco, Fernández, Alfonso J., Alados-Arboledas, Lucas, Bravo-Aranda, Juan Antonio, Navas-Guzmán, Francisco, Guerrero-Rascado, Juan Luis, Granados-Muñoz, María José, Preißler, Jana, Wagner, Frank, Gausa, Michael, Grigorov, Ivan, Stoyanov, Dimitar, Iarlori, Marco, Rizi, Vincenco, Spinelli, Nicola, Boselli, Antonella, Wang, Xuan, Feudo, Teresa Lo, Perrone, Maria Rita, De Tomas, Ferdinando, Burlizzi, Pasquale

This paper introduces the recent European Aerosol Research Lidar Network (EARLINET) quality-assurance efforts at instrument level. Within two dedicated campaigns and five single-site intercomparison activities, 21 EARLINET systems from 18 EARLINET stations were intercompared between 2009 and 2013. A comprehensive strategy for campaign setup and data evaluation has been established. Eleven systems from nine EARLINET stations participated in the EARLINET Lidar Intercomparison 2009 (EARLI09). In this campaign, three reference systems were qualified which served as traveling standards thereafter. EARLINET systems from nine other stations have been compared against these reference systems since 2009. We present and discuss comparisons at signal and at product level from all campaigns for more than 100 individual measurement channels at the wavelengths of 355, 387, 532, and 607 nm. It is shown that in most cases, a very good agreement of the compared systems with the respective reference is obtained. Mean signal deviations in predefined height ranges are typically below ±2 %. Particle backscatter and extinction coefficients agree within ±2  ×  10−4 km−1 sr−1 and ± 0.01 km−1, respectively, in most cases. For systems or channels that showed larger discrepancies, an in-depth analysis of deficiencies was performed and technical solutions and upgrades were proposed and realized. The intercomparisons have reinforced confidence in the EARLINET data quality and allowed us to draw conclusions on necessary system improvements for some instruments and to identify major challenges that need to be tackled in the future.

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Fine and coarse dust separation with polarization lidar

2014, Mamouri, R.E., Ansmann, A.

The polarization-lidar photometer networking (POLIPHON) method for separating dust and non-dust aerosol backscatter and extinction, volume, and mass concentration is extended to allow for a height-resolved separation of fine-mode and coarse-mode dust properties in addition. The method is applied to a period with complex aerosol layering of fine-mode background dust from Turkey and Arabian desert dust from Syria. The observation was performed at the combined European Aerosol Research Lidar Network (EARLINET) and Aerosol Robotic Network (AERONET) site of Limassol (34.7° N, 33° E), Cyprus, in September 2011. The dust profiling methodology and case studies are presented. Consistency between the column-integrated optical properties obtained with sun/sky photometer and the respective results derived by means of the new lidar-based method corroborate the applicability of the extended POLIPHON version.

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Vertically resolved dust optical properties during SAMUM: Tinfou compared to Ouarzazate

2017, Heese, Birgit, Althausen, Dietrich, Dinter, Tilman, Esselborn, Michael, Müller, Thomas, Tesche, Matthias, Wiegner, Matthias

Vertical profiles of dust key optical properties are presented from measurements during the Saharan Mineral Dust Experiment (SAMUM) by Raman and depolarization lidar at two ground-based sites and by airborne high spectral resolution lidar. One of the sites, Tinfou, is located close to the border of the Sahara in Southern Morocco and was the main in situ site during SAMUM. The other site was Ouarzazate airport, the main lidar site. From the lidar measurements the spatial distribution of the dust between Tinfou and Ouarzazate was derived for 1 d. The retrieved profiles of backscatter and extinction coefficients and particle depolarization ratios show comparable dust optical properties, a similar vertical structure of the dust layer, and a height of about 4 km asl at both sites. The airborne cross-section of the extinction coefficient at the two sites confirms the low variability in dust properties. Although the general picture of the dust layer was similar, the lidar measurements reveal a higher dust load closer to the dust source. Nevertheless, the observed intensive optical properties were the same. These results indicate that the lidar measurements at two sites close to the dust source are both representative for the SAMUM dust conditions.