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Rotational quantum beat lasing without inversion

2020, Richter, Maria, Lytova, Marianna, Morales, Felipe, Haessler, Stefan, Smirnova, Olga, Spanner, Michael, Ivanov, Misha

In standard lasers, light amplification requires population inversion between an upper and a lower state to break the reciprocity between absorption and stimulated emission. However, in a medium prepared in a specific superposition state, quantum interference may fully suppress absorption while leaving stimulated emission intact, opening the possibility of lasing without inversion. Here we show that lasing without inversion arises naturally during propagation of intense femtosecond laser pulses in air. It is triggered by the combination of molecular ionization and molecular alignment, both unavoidable in intense light fields. The effect could enable inversionless amplification of broadband radiation in many molecular gases, opening unusual opportunities for remote sensing. © 2020 Optical Society of America

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In situ temporal measurement of ultrashort laser pulses at full power during high-intensity laser–matter interactions

2020, Crespo, Helder M., Witting, Tobias, Canhota, Miguel, Miranda, Miguel, Tisch, John W.G

In laser-matter interaction experiments, it is of paramount importance to characterize the laser pulse on target (in situ) and at full power. This allows pulse optimization and meaningful comparison with theory, and it can shed fundamental new light on pulse distortions occurring in or on the target.Here we introduce and demonstrate a new technique based on dispersion-scan using the concurrent third harmonic emission from the target that permits the full (amplitude and phase), in situ, in-parallel characterization of ultrashort laser pulses in a gas or solid target over a very wide intensity range encompassing the 1013-1015Wcm-2regime of high harmonic generation and other important strong-field phenomena, with possible extension to relativistic intensities presently inaccessible to other diagnostics. © 2020 OSA - The Optical Society. All rights reserved.