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Waveguide-Integrated Broadband Spectrometer Based on Tailored Disorder

2020, Hartmann, Wladick, Varytis, Paris, Gehring, Helge, Walter, Nicolai, Beutel, Fabian, Busch, Kurt, Pernice, Wolfram

Compact, on-chip spectrometers exploiting tailored disorder for broadband light scattering enable high-resolution signal analysis while maintaining a small device footprint. Due to multiple scattering events of light in the disordered medium, the effective path length of the device is significantly enhanced. Here, on-chip spectrometers are realized for visible and near-infrared wavelengths by combining an efficient broadband fiber-to-chip coupling approach with a scattering area in a broadband transparent silicon nitride waveguiding structure. Air holes etched into a structured silicon nitride slab terminated with multiple waveguides enable multipath light scattering in a diffusive regime. Spectral-to-spatial mapping is performed by determining the transmission matrix at the waveguide outputs, which is then used to reconstruct the probe signals. Direct comparison with theoretical analyses shows that such devices can be used for high-resolution spectroscopy from the visible up to the telecom wavelength regime. © 2020 The Authors. Published by WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim

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Needle beams: a review

2020, Grunwald R., Bock M.

Needle beams are highly attractive for applications which take advantage from a spatial and temporal localization of photons. High intensities, high resolution and extended depth of focus lead to fundamental advances in the optical system performance. Ultrashort, fringe-free, self-reconstructing nondiffracting pulses with undistorted temporal transfer are obtained by generating truncated Bessel beams under self-apodization conditions. Nondiffracting Talbot self-imaging of needle beam arrays enables to transfer near field information to the Fraunhofer zone. With addressable arrays of needle beams, reconfigurable time-wavefront sensors are built up. Moreover, spatial light modulators and flexible axicons are used to realize structured, highly localized wavepackets, accelerating beams and nondiffracting images. © 2020, © 2020 The Author(s). Published by Informa UK Limited, trading as Taylor & Francis Group.

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Delayed relaxation of highly excited naphthalene cations

2020, Reitsma, G., Hummert, J., Dura, J., Loriot, V., Vrakking, M.J.J., Lépine, F., Kornilov, O.

The efficiency of energy transfer in ultrafast electronic relaxation of molecules depends strongly on the complex interplay between electronic and nuclear motion. In this study we use wavelength-selected XUV pulses to induce relaxation dynamics of highly excited cationic states of naphthalene. Surprisingly, the observed relaxation lifetimes increase with the cationic excitation energy. We propose that this is a manifestation of a quantum mechanical population trapping that leads to delayed relaxation of molecules in the regions with a high density of excited states. © 2019 Published under licence by IOP Publishing Ltd.

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Generation of elliptically polarized soft x rays using high-order harmonic generation with orthogonal two-color laser fields

2020, Milošević, D.B., Becker, W.

High-order harmonic generation by orthogonally polarized two-color (OTC) laser fields is analysed using strong-field approximation and quantum-orbit theory. Results for the field components frequency ratio of 2:1 and 3:1 are presented and compared. We have shown that, depending on the relative phase between the field components, the shape of the high-harmonic spectrum can be very different from that obtained by a monochromatic linearly polarized laser field. It is also shown that it is possible to generate elliptically polarized high-order harmonics with very high photon energies using OTC laser field with the frequency ratio of 3:1 and a long fundamental wavelength. An effective relative phase control of the harmonic emission is demonstrated. The obtained results are explained using the quantum-orbit theory. © Published under licence by IOP Publishing Ltd.

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Tailored Disorder in Photonics: Learning from Nature

2021, Rothammer, Maximilian, Zollfrank, Cordt, Busch, Kurt, Freymann, Georg von

Disorder and photonics have long been seen as natural adversaries and designers of optical systems have often driven systems to perfection by minimizing deviations from the ideal design. Especially in the field of photonic crystals and metamaterials but also for optical circuits, disorder has been avoided as a nuisance for many years. However, starting from the very robust structural colors found in nature, scientists learn to analyze and tailor disorder to achieve functionalities beyond what is possible with perfectly ordered or ideal systems alone. This review article covers theoretical and materials aspects of tailored disorder as well as experimental results. Furthermore selected examples are highlighted in greater detail, for which the intentional use of disorder adds additional functionality or provides novel functionality impossible without disorder. © 2021 The Authors. Advanced Optical Materials published by Wiley-VCH GmbH

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Infrared emission bands and thermal effects for 440-nm-emitting GaN-based laser diodes

2020, Mao F., Hong J., Wang H., Chen Y., Jing C., Yang P., Tomm J.W., Chu J., Yue F.

Broad emission bands due to defects in (In,Ga,Al)N laser diodes operating at 440 nm are investigated using continuous-wave and pulsed currents. In addition to known yellow-green and short-wave infrared bands, defect emissions were observed even in the medium-wave infrared range. A separation from thermal radiation is possible. When using pulsed currents, a super-linearly increasing emission occurs at ∼1150 nm, which could be attributed to amplified spontaneous emission mainly due to the electroluminescence of deep defects in the optically active region. These results may be useful in interpreting the output power bottleneck of GaN-based lasers compared to mature GaAs-based lasers. © 2020 Author(s). All article content, except where otherwise noted, is licensed under a Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/). https://doi.org/10.1063/1.5143802

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Robust transverse structures in rescattered photoelectron wavepackets and their consequences

2020, Bredtmann, T., Patchkovskii, S.

Initial-state symmetry has been under-appreciated in strong-field spectroscopies, where laser fields dominate the dynamics. We demonstrate numerically that the transverse photoelectron phase structure, arising from the initial-state symmetry, is robust in strong-field rescattering, and has pronounced effects on strong-field photoelectron spectra. Interpretation of rescattering experiments need to take these symmetry effects into account. In turn, robust transverse photoelectron phase structures may enable attosecond sub-Ångström super-resolution imaging with structured electron beams.

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High-energy few-cycle pulses: post-compression techniques

2021, Nagy, Tamas, Simon, Peter, Veisz, Laszlo

Contemporary ultrafast science requires reliable sources of high-energy few-cycle light pulses. Currently two methods are capable of generating such pulses: post compression of short laser pulses and optical parametric chirped-pulse amplification (OPCPA). Here we give a comprehensive overview on the post-compression technology based on optical Kerr-effect or ionization, with particular emphasis on energy and power scaling. Relevant types of post compression techniques are discussed including free propagation in bulk materials, multiple-plate continuum generation, multi-pass cells, filaments, photonic-crystal fibers, hollow-core fibers and self-compression techniques. We provide a short theoretical overview of the physics as well as an in-depth description of existing experimental realizations of post compression, especially those that can provide few-cycle pulse duration with mJ-scale pulse energy. The achieved experimental performances of these methods are compared in terms of important figures of merit such as pulse energy, pulse duration, peak power and average power. We give some perspectives at the end to emphasize the expected future trends of this technology. © 2020 The Author(s). Published by Informa UK Limited, trading as Taylor & Francis Group.

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Nanostructured In3SbTe2 antennas enable switching from sharp dielectric to broad plasmonic resonances

2022, Heßler, Andreas, Wahl, Sophia, Kristensen, Philip Trøst, Wuttig, Matthias, Busch, Kurt, Taubner, Thomas

Phase-change materials (PCMs) allow for non-volatile resonance tuning of nanophotonic components. Upon switching, they offer a large dielectric contrast between their amorphous and crystalline phases. The recently introduced “plasmonic PCM” In3SbTe2 (IST) additionally features in its crystalline phase a sign change of its permittivity over a broad infrared spectral range. While optical resonance switching in unpatterned IST thin films has been investigated before, nanostructured IST antennas have not been studied, yet. Here, we present numerical and experimental investigations of nanostructured IST rod and disk antennas. By crystallizing the IST with microsecond laser pulses, we switched individual antennas from narrow dielectric to broad plasmonic resonances. For the rod antennas, we demonstrated a resonance shift of up to 1.2 µm (twice the resonance width), allowing on/off switching of plasmonic resonances with a contrast ratio of 2.7. With the disk antennas, we realized an increase of the resonance width by more than 800% from 0.24 µm to 1.98 µm while keeping the resonance wavelength constant. Further, we demonstrated intermediate switching states by tuning the crystallization depth within the resonators. Our work empowers future design concepts for nanophotonic applications like active spectral filters, tunable absorbers, and switchable flat optics.

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Strong-Field Ionization of Linear Molecules by a Bichromatic Elliptically Polarized Laser Field with Coplanar Counterrotating or Corotating Components of Different Frequencies

2020, Gazibegović-Busuladžić, A., Busuladžić, M., Čerkić, A., Hasović, E., Becker, W., Milošević, D.B.

We investigate strong-field ionization of linear molecules by a two-color laser field of frequencies rω and sω having coplanar counterrotating or corotating elliptically polarized components (ω is the fundamental laser field frequency and r and s are integers). Using the improved molecular strong-field approximation we analyze direct above-threshold ionization (ATI) and high-order ATI (HATI) spectra. More precisely, reflection and rotational symmetries of these spectra for linear molecules aligned in the laser-field polarization plane are considered. The reflection symmetries for particular molecular orientations, known to be valid for a bicircular field (this is the field with circularly polarized counterrotating components), are valid also for arbitrary component ellipticities. However, specific rotational symmetries that are satisfied for HATI by a bicircular field, are violated for an arbitrary elliptically polarized field with counterrotating components. For the corotating case and the N2 molecule we analyze molecular-orientation-dependent interferences and plateau structures for various ellipticities.