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- ItemEnsemble analysis of complex network properties—an MCMC approach([London] : IOP, 2022) Pfeffer, Oskar; Molkenthin, Nora; Hellmann, FrankWhat do generic networks that have certain properties look like? We use relative canonical network ensembles as the ensembles that realize a property R while being as indistinguishable as possible from a background network ensemble. This allows us to study the most generic features of the networks giving rise to the property under investigation. To test the approach we apply it to study properties thought to characterize ‘small-world networks’. We consider two different defining properties, the ‘small-world-ness’ of Humphries and Gurney, as well as a geometric variant. Studying them in the context of Erdős-Rényi and Watts-Strogatz ensembles we find that all ensembles studied exhibit phase transitions to systems with large hubs and in some cases cliques. Such features are not present in common examples of small-world networks, indicating that these properties do not robustly capture the notion of small-world networks. We expect the overall approach to have wide applicability for understanding network properties of real world interest, such as optimal ride-sharing designs, the vulnerability of networks to cascades, the performance of communication topologies in coordinating fluctuation response or the ability of social distancing measures to suppress disease spreading.
- ItemDiffraction imaging of light induced dynamics in xenon-doped helium nanodroplets([London] : IOP, 2022-11-30) Langbehn, B.; Ovcharenko, Y.; Clark, A.; Coreno, M.; Cucini, R.; Demidovich, A.; Drabbels, M.; Finetti, P.; Di Fraia, M.; Giannessi, L.; Grazioli, C.; Iablonskyi, D.; LaForge, A.C.; Nishiyama, T.; Oliver Álvarez de Lara, V.; Peltz, C.; Piseri, P.; Plekan, O.; Sander, K.; Ueda, K.; Fennel, T.; Prince, K.C.; Stienkemeier, F.; Callegari, C.; Möller, T.; Rupp, D.We explore the light induced dynamics in superfluid helium nanodroplets with wide-angle scattering in a pump–probe measurement scheme. The droplets are doped with xenon atoms to facilitate the ignition of a nanoplasma through irradiation with near-infrared laser pulses. After a variable time delay of up to 800 ps, we image the subsequent dynamics using intense extreme ultraviolet pulses from the FERMI free-electron laser. The recorded scattering images exhibit complex intensity fluctuations that are categorized based on their characteristic features. Systematic simulations of wide-angle diffraction patterns are performed, which can qualitatively explain the observed features by employing model shapes with both randomly distributed as well as structured, symmetric distortions. This points to a connection between the dynamics and the positions of the dopants in the droplets. In particular, the structured fluctuations might be governed by an underlying array of quantized vortices in the superfluid droplet as has been observed in previous small-angle diffraction experiments. Our results provide a basis for further investigations of dopant–droplet interactions and associated heating mechanisms.
- ItemFemtosecond XUV–IR induced photodynamics in the methyl iodide cation([London] : IOP, 2021) Murillo-Sánchez, Marta L.; Reitsma, Geert; Poullain, Sonia Marggi; Fernández-Milán, Pedro; González-Vázquez, Jesús; de Nalda, Rebeca; Martín, Fernando; Vrakking, Marc J. J.; Kornilov, Oleg; Bañares, LuisThe time-resolved photodynamics of the methyl iodide cation (CH3I+) are investigated by means of femtosecond XUV-IR pump-probe spectroscopy. A time-delay-compensated XUV monochromator is employed to isolate a specific harmonic, the 9th harmonic of the fundamental 800 nm (13.95 eV, 88.89 nm), which is used as a pump pulse to prepare the cation in several electronic states. A time-delayed IR probe pulse is used to probe the dissociative dynamics on the first excited state potential energy surface. Photoelectrons and photofragment ions - and I+ - are detected by velocity map imaging. The experimental results are complemented with high level ab initio calculations for the potential energy curves of the electronic states of CH3I+ as well as with full dimension on-the-fly trajectory calculations on the first electronically excited state, considering the presence of the IR pulse. The and I+ pump-probe transients reflect the role of the IR pulse in controlling the photodynamics of CH3I+ in the state, mainly through the coupling to the ground state and to the excited state manifold. Oscillatory features are observed and attributed to a vibrational wave packet prepared in the state. The IR probe pulse induces a coupling between electronic states leading to a slow depletion of fragments after the cation is transferred to the ground states and an enhancement of I+ fragments by absorption of IR photons yielding dissociative photoionization. © 2021 The Author(s). Published by IOP Publishing Ltd on behalf of the Institute of Physics and Deutsche Physikalische Gesellschaft.
- ItemCorrigendum: Generation of high-quality GeV-class electron beams utilizing attosecond ionization injection (2021 New J. Phys. 23 043016)([London] : IOP, 2021) Lécz, Zsolt; Andreev, Alexander; Kamperidis, C.; Hafz, NasrAcceleration of electrons in laser-driven plasma wakefields has been extended up to the ∼8 GeV energy within a distance of tens of centimeters. However, in applications, requiring small energy spread within the electron bunch, only a small portion of the bunch can be used and often the low-energy electrons represent undesired background in the spectrum. We present a compact and tunable scheme providing clean and mono-energetic electron bunches with less than one percent energy spread and with central energy on the GeV level. It is a two-step process consisting of ionization injection with attosecond pulses and acceleration in a capillary plasma wave-guide. Semi-analytical theory and particle-in-cell simulations are used to accurately model the injection and acceleration steps.
- ItemImproved earthquake aftershocks forecasting model based on long-term memory([London] : IOP, 2021) Zhang, Yongwen; Zhou, Dong; Fan, Jingfang; Marzocchi, Warner; Ashkenazy, Yosef; Havlin, ShlomoA prominent feature of earthquakes is their empirical laws, including memory (clustering) in time and space. Several earthquake forecasting models, such as the epidemic-type aftershock sequence (ETAS) model, were developed based on these empirical laws. Yet, a recent study [1] showed that the ETAS model fails to reproduce the significant long-term memory characteristics found in real earthquake catalogs. Here we modify and generalize the ETAS model to include short- and long-term triggering mechanisms, to account for the short- and long-time memory (exponents) discovered in the data. Our generalized ETAS model accurately reproduces the short- and long-term/distance memory observed in the Italian and Southern Californian earthquake catalogs. The revised ETAS model is also found to improve earthquake forecasting after large shocks.
- ItemEfficient network immunization strategy based on generalized Herfindahl–Hirschman index([London] : IOP, 2021) Chen, Peng; Qi, Mingze; Lu, Xin; Duan, Xiaojun; Kurths, JürgenThe topic of finding effective strategies to restrain epidemic spreading in complex networks is of current interest. A widely used approach for epidemic containment is the fragmentation of the contact networks through immunization. However, due to the limitation of immune resources, we cannot always fragment the contact network completely. In this study, based on the size distribution of connected components for the network, we designed a risk indicator of epidemic outbreaks, the generalized Herfindahl–Hirschman index (GHI), which measures the upper bound of the expected infection's prevalence (the fraction of infected nodes) in random outbreaks. An immunization approach based on minimizing GHI is developed to reduce the infection risk for individuals in the network. Experimental results show that our immunization strategy could effectively decrease the infection's prevalence as compared to other existing strategies, especially against infectious diseases with higher infection rates or lower recovery rates. The findings provide an efficient and practicable strategy for immunization against epidemic diseases.
- ItemSpontaneous trail formation in populations of auto-chemotactic walkers([London] : IOP, 2022) Mokhtari, Zahra; Patterson, Robert I. A.; Höfling, FelixWe study the formation of trails in populations of self-propelled agents that make oriented deposits of pheromones and also sense such deposits to which they then respond with gradual changes of their direction of motion. Based on extensive off-lattice computer simulations aiming at the scale of insects, e.g. ants, we identify a number of emerging stationary patterns and obtain qualitatively the non-equilibrium state diagram of the model, spanned by the strength of the agent–pheromone interaction and the number density of the population. In particular, we demonstrate the spontaneous formation of persistent, macroscopic trails, and highlight some behaviour that is consistent with a dynamic phase transition. This includes a characterisation of the mass of system-spanning trails as a potential order parameter. We also propose a dynamic model for a few macroscopic observables, including the sub-population size of trail-following agents, which captures the early phase of trail formation.
- ItemNeural partial differential equations for chaotic systems([London] : IOP, 2021) Gelbrecht, Maximilian; Boers, Niklas; Kurths, JürgenWhen predicting complex systems one typically relies on differential equation which can often be incomplete, missing unknown influences or higher order effects. By augmenting the equations with artificial neural networks we can compensate these deficiencies. We show that this can be used to predict paradigmatic, high-dimensional chaotic partial differential equations even when only short and incomplete datasets are available. The forecast horizon for these high dimensional systems is about an order of magnitude larger than the length of the training data.
- ItemInterplay of charge density waves, disorder, and superconductivity in 2H-TaSe2 elucidated by NMR([London] : IOP, 2022) Baek, Seung-Ho; Sur, Yeahan; Kim, Kee Hoon; Vojta, Matthias; Büchner, BerndSingle crystals of pristine and 6% Pd-intercalated 2H‐TaSe2 have been studied by means of 77Se nuclear magnetic resonance. The temperature dependence of the 77Se spectrum, with an unexpected line narrowing upon Pd intercalation, unravels the presence of correlated local lattice distortions far above the transition temperature of the charge density wave (CDW) order, thereby supporting a strong-coupling CDW mechanism in 2H‐TaSe2. While, the Knight shift data suggest that the incommensurate CDW transition involves a partial Fermi surface gap opening. As for spin dynamics, the 77Se spin-lattice relaxation rate T1-1 as a function of temperature shows that a pseudogap behavior dominates the low-energy spin excitations even within the CDW phase, and gets stronger along with superconductivity in the Pd-6% sample. We discuss that CDW fluctuations may be responsible for the pseudogap as well as superconductivity, although the two phenomena are unlikely to be directly linked each other.
- ItemStrong surface termination dependence of the electronic structure of polar superconductor LaFeAsO revealed by nano-ARPES([London] : IOP, 2022) Jung, Sung Won; Rhodes, Luke C; Watson, Matthew D; Evtushinsky, Daniil V; Cacho, Cephise; Aswartham, Saicharan; Kappenberger, Rhea; Wurmehl, Sabine; Büchner, Bernd; Kim, Timur KThe electronic structures of the iron-based superconductors have been intensively studied by using angle-resolved photoemission spectroscopy (ARPES). A considerable amount of research has been focused on the LaFeAsO family, showing the highest transition temperatures, where previous ARPES studies have found much larger Fermi surfaces than bulk theoretical calculations would predict. The discrepancy has been attributed to the presence of termination-dependent surface states. Here, using photoemission spectroscopy with a sub-micron focused beam spot (nano-ARPES) we have successfully measured the electronic structures of both the LaO and FeAs terminations in LaFeAsO. Our data reveal very different band dispersions and core-level spectra for different surface terminations, showing that previous macro-focus ARPES measurements were incomplete. Our results give direct evidence for the surface-driven electronic structure reconstruction in LaFeAsO, including formation of the termination-dependent surface states at the Fermi level. This experimental technique, which we have shown to be very powerful when applied to this prototypical compound, can now be used to study various materials with different surface terminations.