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- ItemA phenomenology of new particle formation (NPF) at 13 European sites(Katlenburg-Lindau : European Geosciences Union, 2021) Bousiotis, Dimitrios; Pope, Francis D.; Beddows, David C. S.; Dall'Osto, Manuel; Massling, Andreas; Nøjgaard, Jakob Klenø; Nordstrøm, Claus; Niemi, Jarkko V.; Portin, Harri; Petäjä, Tuukka; Perez, Noemi; Alastuey, Andrés; Querol, Xavier; Kouvarakis, Giorgos; Mihalopoulos, Nikos; Vratolis, Stergios; Eleftheriadis, Konstantinos; Wiedensohler, Alfred; Weinhold, Kay; Merkel, Maik; Tuch, Thomas; Harrison, Roy M.New particle formation (NPF) events occur almost everywhere in the world and can play an important role as a particle source. The frequency and characteristics of NPF events vary spatially, and this variability is yet to be fully understood. In the present study, long-term particle size distribution datasets (minimum of 3 years) from 13 sites of various land uses and climates from across Europe were studied, and NPF events, deriving from secondary formation and not traffic-related nucleation, were extracted and analysed. The frequency of NPF events was consistently found to be higher at rural background sites, while the growth and formation rates of newly formed particles were higher at roadsides (though in many cases differences between the sites were small), underlining the importance of the abundance of condensable compounds of anthropogenic origin found there. The growth rate was higher in summer at all rural background sites studied. The urban background sites presented the highest uncertainty due to greater variability compared to the other two types of site. The origin of incoming air masses and the specific conditions associated with them greatly affect the characteristics of NPF events. In general, cleaner air masses present higher probability for NPF events, while the more polluted ones show higher growth rates. However, different patterns of NPF events were found, even at sites in close proximity (<ĝ€¯200ĝ€¯km), due to the different local conditions at each site. Region-wide events were also studied and were found to be associated with the same conditions as local events, although some variability was found which was associated with the different seasonality of the events at two neighbouring sites. NPF events were responsible for an increase in the number concentration of ultrafine particles of more than 400ĝ€¯% at rural background sites on the day of their occurrence. The degree of enhancement was less at urban sites due to the increased contribution of other sources within the urban environment. It is evident that, while some variables (such as solar radiation intensity, relative humidity, or the concentrations of specific pollutants) appear to have a similar influence on NPF events across all sites, it is impossible to predict the characteristics of NPF events at a site using just these variables, due to the crucial role of local conditions. © Author(s) 2021.
- ItemTerrestrial or marine – indications towards the origin of ice-nucleating particles during melt season in the European Arctic up to 83.7° N(Katlenburg-Lindau : European Geosciences Union, 2021) Hartmann, Markus; Gong, Xianda; Kecorius, Simonas; van Pinxteren, Manuela; Vogl, Teresa; Welti, André; Wex, Heike; Zeppenfeld, Sebastian; Herrmann, Hartmut; Wiedensohler, Alfred; Stratmann, FrankIce-nucleating particles (INPs) initiate the primary ice formation in clouds at temperatures above ca. -38gC and have an impact on precipitation formation, cloud optical properties, and cloud persistence. Despite their roles in both weather and climate, INPs are not well characterized, especially in remote regions such as the Arctic. We present results from a ship-based campaign to the European Arctic during May to July 2017. We deployed a filter sampler and a continuous-flow diffusion chamber for offline and online INP analyses, respectively. We also investigated the ice nucleation properties of samples from different environmental compartments, i.e., the sea surface microlayer (SML), the bulk seawater (BSW), and fog water. Concentrations of INPs (NINP) in the air vary between 2 to 3 orders of magnitudes at any particular temperature and are, except for the temperatures above -10gC and below -32gC, lower than in midlatitudes. In these temperature ranges, INP concentrations are the same or even higher than in the midlatitudes. By heating of the filter samples to 95gC for 1ĝ€¯h, we found a significant reduction in ice nucleation activity, i.e., indications that the INPs active at warmer temperatures are biogenic. At colder temperatures the INP population was likely dominated by mineral dust. The SML was found to be enriched in INPs compared to the BSW in almost all samples. The enrichment factor (EF) varied mostly between 1 and 10, but EFs as high as 94.97 were also observed. Filtration of the seawater samples with 0.2ĝ€¯μm syringe filters led to a significant reduction in ice activity, indicating the INPs are larger and/or are associated with particles larger than 0.2ĝ€¯μm. A closure study showed that aerosolization of SML and/or seawater alone cannot explain the observed airborne NINP unless significant enrichment of INP by a factor of 105 takes place during the transfer from the ocean surface to the atmosphere. In the fog water samples with -3.47gC, we observed the highest freezing onset of any sample. A closure study connecting NINP in fog water and the ambient NINP derived from the filter samples shows good agreement of the concentrations in both compartments, which indicates that INPs in the air are likely all activated into fog droplets during fog events. In a case study, we considered a situation during which the ship was located in the marginal sea ice zone and NINP levels in air and the SML were highest in the temperature range above -10gC. Chlorophyll a measurements by satellite remote sensing point towards the waters in the investigated region being biologically active. Similar slopes in the temperature spectra suggested a connection between the INP populations in the SML and the air. Air mass history had no influence on the observed airborne INP population. Therefore, we conclude that during the case study collected airborne INPs originated from a local biogenic probably marine source. © Author(s) 2021.
- ItemComparison of particle number size distribution trends in ground measurements and climate models(Katlenburg-Lindau : EGU, 2022) Leinonen, Ville; Kokkola, Harri; Yli-Juuti, Taina; Mielonen, Tero; Kühn, Thomas; Nieminen, Tuomo; Heikkinen, Simo; Miinalainen, Tuuli; Bergman, Tommi; Carslaw, Ken; Decesari, Stefano; Fiebig, Markus; Hussein, Tareq; Kivekäs, Niku; Krejci, Radovan; Kulmala, Markku; Leskinen, Ari; Massling, Andreas; Mihalopoulos, Nikos; Mulcahy, Jane P.; Noe, Steffen M.; van Noije, Twan; O'Connor, Fiona M.; O'Dowd, Colin; Olivie, Dirk; Pernov, Jakob B.; Petäjä, Tuukka; Seland, Øyvind; Schulz, Michael; Scott, Catherine E.; Skov, Henrik; Swietlicki, Erik; Tuch, Thomas; Wiedensohler, Alfred; Virtanen, Annele; Mikkonen, SanttuDespite a large number of studies, out of all drivers of radiative forcing, the effect of aerosols has the largest uncertainty in global climate model radiative forcing estimates. There have been studies of aerosol optical properties in climate models, but the effects of particle number size distribution need a more thorough inspection. We investigated the trends and seasonality of particle number concentrations in nucleation, Aitken, and accumulation modes at 21 measurement sites in Europe and the Arctic. For 13 of those sites, with longer measurement time series, we compared the field observations with the results from five climate models, namely EC-Earth3, ECHAM-M7, ECHAM-SALSA, NorESM1.2, and UKESM1. This is the first extensive comparison of detailed aerosol size distribution trends between in situ observations from Europe and five earth system models (ESMs). We found that the trends of particle number concentrations were mostly consistent and decreasing in both measurements and models. However, for many sites, climate models showed weaker decreasing trends than the measurements. Seasonal variability in measured number concentrations, quantified by the ratio between maximum and minimum monthly number concentration, was typically stronger at northern measurement sites compared to other locations. Models had large differences in their seasonal representation, and they can be roughly divided into two categories: for EC-Earth and NorESM, the seasonal cycle was relatively similar for all sites, and for other models the pattern of seasonality varied between northern and southern sites. In addition, the variability in concentrations across sites varied between models, some having relatively similar concentrations for all sites, whereas others showed clear differences in concentrations between remote and urban sites. To conclude, although all of the model simulations had identical input data to describe anthropogenic mass emissions, trends in differently sized particles vary among the models due to assumptions in emission sizes and differences in how models treat size-dependent aerosol processes. The inter-model variability was largest in the accumulation mode, i.e. sizes which have implications for aerosol-cloud interactions. Our analysis also indicates that between models there is a large variation in efficiency of long-range transportation of aerosols to remote locations. The differences in model results are most likely due to the more complex effect of different processes instead of one specific feature (e.g. the representation of aerosol or emission size distributions). Hence, a more detailed characterization of microphysical processes and deposition processes affecting the long-range transport is needed to understand the model variability.
- ItemClimate change impacts on European arable crop yields: Sensitivity to assumptions about rotations and residue management(Amsterdam [u.a.] : Elsevier, 2022) Faye, Babacar; Webber, Heidi; Gaiser, Thomas; Müller, Christoph; Zhang, Yinan; Stella, Tommaso; Latka, Catharina; Reckling, Moritz; Heckelei, Thomas; Helming, Katharina; Ewert, FrankMost large scale studies assessing climate change impacts on crops are performed with simulations of single crops and with annual re-initialization of the initial soil conditions. This is in contrast to the reality that crops are grown in rotations, often with sizable proportion of the preceding crop residue to be left in the fields and varying soil initial conditions from year to year. In this study, the sensitivity of climate change impacts on crop yield and soil organic carbon to assumptions about annual model re-initialization, specification of crop rotations and the amount of residue retained in fields was assessed for seven main crops across Europe. Simulations were conducted for a scenario period 2040–2065 relative to a baseline from 1980 to 2005 using the SIMPLACE1 framework. Results indicated across Europe positive climate change impacts on yield for C3 crops and negative impacts for maize. The consideration of simulating rotations did not have a benefit on yield variability but on relative yield change in response to climate change which slightly increased for C3 crops and decreased for C4 crops when rotation was considered. Soil organic carbon decreased under climate change in both simulations assuming a continuous monocrop and plausible rotations by between 1% and 2% depending on the residue management strategy.
- ItemOccupational health and safety in agriculture – a brief report on organization, legislation and support in selected European countries(Lublin : Institute of Agricultural Medicine, 2021) Jakob, Martina Carola; Santa, Dushica; Holte, Kari Anne; Sikkeland, Inger Johanne; Hilt, Bjorn; Lundqvist, PeterIntroduction and objective: Agriculture and forestry are among the most dangerous professions in Europe, with a high level of accidents affecting the sustainability and viability of the sector. International conventions, EU directives and national legislation build the fundamental basis for prevention. The aim of the study is to describe and categorize national mechanisms of occupational safety and health (OSH) for agricultural workers in Europe, to assess the extent of implementing safety regulation, the body in charge, and to give examples of health and safety initiatives. Material and methods: Results of a questionnaire-survey on basic safety regulations on farms sent by e-mail to the representatives of 30 participating European countries in the context of the Sacurima COST action network (CA 16123) are presented. Due to the complexity, only selected countries are described in this study highlighting the regulative bodies, occupational health services or specific training offers, as well as the complexity of the mechanisms. Results: One of the most serious issues and deficits of EU OSH regulation is the exclusion of self-employed farmers who compose nearly 90% of the farming population. This leads to serious under-reporting of accidents, and because one of the most common measures for the performance of health and safety initiatives are the injury and ill health statistics, better registration systems are urgently needed in almost all countries as a basis for preventive efforts. Conclusions: The results of the study provide a basis for raising awareness about the current OSH systems in Europe, and the importance of developing sector specific OSH strategies. The proposed activities should assist in tackling high accident rates and poor occupational health for self-employed farmers.
- ItemUncertainty of simulated groundwater recharge at different global warming levels: a global-scale multi-model ensemble study(Munich : EGU, 2021) Reinecke, Robert; Müller Schmied, Hannes; Trautmann, Tim; Andersen, Lauren Seaby; Burek, Peter; Flörke, Martina; Gosling, Simon N.; Grillakis, Manolis; Hanasaki, Naota; Koutroulis, Aristeidis; Pokhrel, Yadu; Thiery, Wim; Wada, Yoshihide; Yusuke, Satoh; Döll, PetraBillions of people rely on groundwater as being an accessible source of drinking water and for irrigation, especially in times of drought. Its importance will likely increase with a changing climate. It is still unclear, however, how climate change will impact groundwater systems globally and, thus, the availability of this vital resource. Groundwater recharge is an important indicator for groundwater availability, but it is a water flux that is difficult to estimate as uncertainties in the water balance accumulate, leading to possibly large errors in particular in dry regions. This study investigates uncertainties in groundwater recharge projections using a multi-model ensemble of eight global hydrological models (GHMs) that are driven by the bias-adjusted output of four global circulation models (GCMs). Pre-industrial and current groundwater recharge values are compared with recharge for different global warming (GW) levels as a result of three representative concentration pathways (RCPs). Results suggest that projected changes strongly vary among the different GHM–GCM combinations, and statistically significant changes are only computed for a few regions of the world. Statistically significant GWR increases are projected for northern Europe and some parts of the Arctic, East Africa, and India. Statistically significant decreases are simulated in southern Chile, parts of Brazil, central USA, the Mediterranean, and southeastern China. In some regions, reversals of groundwater recharge trends can be observed with global warming. Because most GHMs do not simulate the impact of changing atmospheric CO2 and climate on vegetation and, thus, evapotranspiration, we investigate how estimated changes in GWR are affected by the inclusion of these processes. In some regions, inclusion leads to differences in groundwater recharge changes of up to 100 mm per year. Most GHMs with active vegetation simulate less severe decreases in groundwater recharge than GHMs without active vegetation and, in some regions, even increases instead of decreases are simulated. However, in regions where GCMs predict decreases in precipitation and where groundwater availability is the most important, model agreement among GHMs with active vegetation is the lowest. Overall, large uncertainties in the model outcomes suggest that additional research on simulating groundwater processes in GHMs is necessary.
- ItemThe energy and carbon inequality corridor for a 1.5 °C compatible and just Europe(Bristol : IOP Publ., 2021-6-15) Jaccard, Ingram S; Pichler, Peter-Paul; Többen, Johannes; Weisz, HelgaThe call for a decent life for all within planetary limits poses a dual challenge: provide all people with the essential resources needed to live well and, collectively, not exceed the source and sink capacity of the biosphere to sustain human societies. We examine the corridor of possible distributions of household energy and carbon footprints that satisfy both minimum energy use for a decent life and available energy supply compatible with the 1.5 °C target in 2050. We estimated household energy and carbon footprints for expenditure deciles for 28 European countries in 2015 by combining data from national household budget surveys with the environmentally-extended multi-regional input–output model EXIOBASE. We found a top-to-bottom decile ratio (90:10) of 7.2 for expenditure, 3.1 for net energy and 2.6 for carbon. The lower inequality of energy and carbon footprints is largely attributable to inefficient energy and heating technologies in the lower deciles (mostly Eastern Europe). Adopting best technology across Europe would save 11 EJ of net energy annually, but increase environmental footprint inequality. With such inequality, both targets can only be met through the use of CCS, large efficiency improvements, and an extremely low minimum final energy use of 28 GJ per adult equivalent. Assuming a more realistic minimum energy use of about 55 GJ ae−1 and no CCS deployment, the 1.5 °C target can only be achieved at near full equality. We conclude that achieving both stated goals is an immense and widely underestimated challenge, the successful management of which requires far greater room for maneuver in monetary and fiscal terms than is reflected in the current European political discourse.
- ItemCRAAS: A European Cloud Regime dAtAset Based on the CLAAS-2.1 Climate Data Record(Basel : MDPI, 2022) Tzallas, Vasileios; Hünerbein, Anja; Stengel, Martin; Meirink, Jan Fokke; Benas, Nikos; Trentmann, Jörg; Macke, AndreasGiven the important role of clouds in our planet’s climate system, it is crucial to further improve our understanding of their governing processes as well as the resulting spatio-temporal variability of their properties. This co-variability of different cloud optical properties is adequately represented through the well-established concept of cloud regimes. The focus of the present study lies on the creation of a cloud regime dataset over Europe, named “Cloud Regime dAtAset based on the CLAAS-2.1 climate data record” (CRAAS), in order to analyze their variability and their changes at different spatio-temporal scales. In addition, co-occurrences between the cloud regimes and large-scale weather patterns are investigated. The CLoud property dAtAset using Spinning Enhanced Visible and Infrared (SEVIRI) edition 2.1 (CLAAS-2.1) data record, which is produced by the Satellite Application Facility on Climate Monitoring (CM SAF), was used as the basis for the derivation of the cloud regimes over Europe for a 14-year period (2004–2017). In particular, the cloud optical thickness (COT) and cloud top pressure (CTP) products of CLAAS-2.1 were used in order to compute 2D histograms. Then, the k-means clustering algorithm was applied to the generated 2D histograms in order to derive the cloud regimes. Eight cloud regimes were identified, which, along with the geographical distribution of their frequency of occurrence, assisted in providing a detailed description of the climate of the cloud properties over Europe. The annual and diurnal variabilities of the eight cloud regimes were studied, and trends in their frequency of occurrence were also examined. Larger changes in the frequency of occurrence of the produced cloud regimes were found for a regime associated to alto- and nimbo-type clouds and for a regime connected to shallow cumulus clouds and fog (−0.65% and +0.70% for the time period of the study, respectively).