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- ItemStudy of the tidal variations in mesospheric temperature at low and mid latitudes from WINDII and potassium lidar observations(Göttingen : Copernicus GmbH, 2004) Shepherd, M.; Fricke-Begemann, C.Zonal mean daytime temperatures from the Wind Imaging Interferometer (WINDII) on the Upper Atmosphere Research Satellite (UARS) and nightly temperatures from a potassium (K) lidar are employed in the study of the tidal variations in mesospheric temperature at low and mid latitudes in the Northern Hemisphere. The analysis is applied to observations at 89 km height for winter solstice, December to February (DJF), at 55° N, and for May and November at 28° N. The WINDII results are based on observations from 1991 to 1997. The K-lidar observations for DJF at Kühlungsborn (54° N) were from 1996-1999, while those for May and November at Tenerife 28° N were from 1999. To avoid possible effects from year-to-year variability in the temperatures observed, as well as differences due to instrument calibration and observation periods, the mean temperature field is removed from the respective data sets, assuming that only tidal and planetary scale perturbations remain in the temperature residuals. The latter are then binned in 0.5 h periods and the individual data sets are fitted in a least-mean square sense to 12-h and 8-h harmonics, to infer semidiurnal and terdiurnal tidal parameters. Both the K-lidar and WINDII independently observed a strong semidiurnal tide in November, with amplitudes of 13 K and 7.4 K, respectively. Good agreement was also found in the tidal parameters derived from the two data sets for DJF and May. It was recognized that insufficient local time coverage of the two separate data sets could lead to an overestimation of the semidiurnal tidal amplitude. A combined ground-based/satellite data set with full diurnal local time coverage was created which was fitted to 24 h+ 12 h+8 h harmonics and a novel method applied to account for possible differences between the daytime and nighttime means. The results still yielded a strong semidiurnal tide in November at 28° N with an amplitude of 8.8 K which is twice the SD amplitude in May and DJF. The diurnal tidal parameters were practically the same at 28° N and 55° N, in November and DJF, respectively, with an amplitude of 6.5 K and peaking at ∼9h. The diurnal and semidiurnal amplitudes in May were about the same, 4 K, and 4.6 K, while the terdiurnal tide had the same amplitudes and phases in May and November at 28° N. Good agreement is found with other experimental data while models tend to underestimate the amplitudes.
- ItemHuman alterations of the terrestrial water cycle through land management(Göttingen : Copernicus GmbH, 2008) Rost, S.; Gerten, D.; Heyder, U.This study quantifies current and potential future changes in transpiration, evaporation, interception loss and river discharge in response to land use change, irrigation and climate change, by performing several distinct simulations within the consistent hydrology and biosphere modeling framework LPJmL (Lund-Potsdam-Jena managed Land). We distinguished two irrigation simulations: a water limited one in which irrigation was restricted by local renewable water resources (ILIM), and a potential one in which no such limitation was assumed but withdrawals from deep groundwater or remote rivers allowed (IPOT). We found that the effect of historical land use change as compared to potential natural vegetation was pronounced, including a reduction in interception loss and transpiration by 25.9% and 10.6%, respectively, whereas river discharge increased by 6.6% (climate conditions of 1991-2000). Furthermore, we estimated that about 1170km3yr-1 of irrigation water could be withdrawn from local renewable water resources (in ILIM), which resulted in a reduction of river discharge by 1.5%. However, up to 1660km3yr-1 of water withdrawals were required in addition under the assumption that optimal growth of irrigated crops was sustained (IPOT), which resulted in a slight net increase in global river discharge by 2.0% due to return flows. Under the HadCM3 A2 climate and emission scenario, climate change alone will decrease total evapotranspiration by 1.5% and river discharge by 0.9% in 2046-2055 compared to 1991-2000 average due to changes in precipitation patterns, a decrease in global precipitation amount, and the net effect of CO2 fertilization. A doubling of agricultural land in 2046-2055 compared to 1991-2000 average as proposed by the IMAGE land use change scenario will result in a decrease in total evapotranspiration by 2.5% and in an increase in river discharge by 3.9%. That is, the effects of land use change in the future will be comparable in magnitude to the effects of climate change in this particular scenario. On present irrigated areas future water withdrawal will increase especially in regions where climate changes towards warmer and dryer conditions will be pronounced.
- ItemSmall-scale mixing processes enhancing troposphere-to-stratosphere transport by pyro-cumulonimbus storms(Göttingen : Copernicus GmbH, 2007) Luderer, G.; Trentmann, J.; Hungershöfer, K.; Herzog, M.; Fromm, M.; Andreae, M.O.Deep convection induced by large forest fires is an efficient mechanism for transport of aerosol particles and trace gases into the upper troposphere and lower stratosphere (UT/LS). For many pyro-cumulonimbus clouds (pyroCbs) as well as other cases of severe convection without fire forcing, radiometric observations of cloud tops in the thermal infrared (IR) reveal characteristic structures, featuring a region of relatively high brightness temperatures (warm center) surrounded by a U-shaped region of low brightness temperatures. We performed a numerical simulation of a specific case study of pyroCb using a non-hydrostatic cloud resolving model with a two-moment cloud microphysics parameterization and a prognostic turbulence scheme. The model is able to reproduce the thermal IR structure as observed from satellite radiometry. Our findings establish a close link between the observed temperature pattern and small-scale mixing processes atop and downwind of the overshooting dome of the pyroCb. Such small-scale mixing processes are strongly enhanced by the formation and breaking of a stationary gravity wave induced by the overshoot. They are found to increase the stratospheric penetration of the smoke by up to almost 30 K and thus are of major significance for irreversible transport of forest fire smoke into the lower stratosphere.
- ItemDiurnal variation of midlatitudinal NO3 column abundance over table mountain facility, California(Göttingen : Copernicus GmbH, 2011) Chen, C.M.; Cageao, R.P.; Lawrence, L.; Stutz, J.; Salawitch, R.J.; Jourdain, L.; Li, Q.; Sander, S.P.The column abundance of NO3 was measured over Table Mountain Facility, CA (34.4° 117.7° W) from May 2003 through September 2004, using lunar occultation near full moon with a grating spectrometer. The NO 3 column retrieval was performed with the differential optical absorption spectroscopy (DOAS) technique using both the 623 and 662 nm NO 3 absorption bands. Other spectral features such as Fraunhofer lines and absorption from water vapor and oxygen were removed using solar spectra obtained at different airmass factors. We observed a seasonal variation, with nocturnally averaged NO3 columns between 5-7 × 1013 molec cm-2 during October through March, and 5-22 × 10 13 molec cm-2 during April through September. A subset of the data, with diurnal variability vastly different from the temporal profile obtained from one-dimensional stratospheric model calculations, clearly has boundary layer contributions; this was confirmed by simultaneous long-path DOAS measurements. However, even the NO3 columns that did follow the modeled time evolution were often much larger than modeled stratospheric partial columns constrained by realistic temperatures and ozone concentrations. This discrepancy is attributed to substantial tropospheric NO3 in the free troposphere, which may have the same time dependence as stratospheric NO 3.
- ItemNear-ubiquity of ice-edge blooms in the Arctic(Göttingen : Copernicus GmbH, 2011) Perrette, M.; Yool, A.; Quartly, G.D.; Popova, E.E.Ice-edge blooms are significant features of Arctic primary production, yet have received relatively little attention. Here we combine satellite ocean colour and sea-ice data in a pan-Arctic study. Ice-edge blooms occur in all seasonally ice-covered areas and from spring to late summer, being observed in 77-89% of locations for which adequate data exist, and usually peaking within 20 days of ice retreat. They sometimes form long belts along the ice-edge (greater than 100 km), although smaller structures were also found. The bloom peak is on average more than 1 mg m-3, with major blooms more than 10 mg m -3, and is usually located close to the ice-edge, though not always. Some propagate behind the receding ice-edge over hundreds of kilometres and over several months, while others remain stationary. The strong connection between ice retreat and productivity suggests that the ongoing changes in Arctic sea-ice may have a significant impact on higher trophic levels and local fish stocks.
- ItemTemperature sensitivity of decomposition in relation to soil organic matter pools: Critique and outlook(Göttingen : Copernicus GmbH, 2005) Reichstein, M.; Kätterer, T.; Andrén, O.; Ciais, P.; Schulze, E.-D.; Cramer, W.; Papale, D.; Valentini, R.Knorr et al. (2005) concluded that soil organic carbon pools with longer turnover times are more sensitive to temperature. We show that this conclusion is equivocal, largely dependent on their specific selection of data and does not persist when the data set of Kätterer et al. (1998) is analysed in a more appropriate way. Further, we analyse how statistical properties of the model parameters may interfere with correlative analyses that relate the Q 10 of soil respiration with the basal rate, where the latter is taken as a proxy for soil organic matter quality. We demonstrate that negative parameter correlations between Qio-values and base respiration rates are statistically expected and not necessarily provide evidence for a higher temperature sensitivity of low quality soil organic matter. Consequently, we propose it is premature to conclude that stable soil carbon is more sensitive to temperature than labile carbon.
- ItemSensitivity of polar stratospheric ozone loss to uncertainties in chemical reaction kinetics(Göttingen : Copernicus GmbH, 2009) Kawa, S.R.; Stolarski, R.S.; Newman, P.A.; Douglass, A.R.; Rex, M.; Hofmann, D.J.; Santee, M.L.; Frieler, K.The impact and significance of uncertainties in model calculations of stratospheric ozone loss resulting from known uncertainty in chemical kinetics parameters is evaluated in trajectory chemistry simulations for the Antarctic and Arctic polar vortices. The uncertainty in modeled ozone loss is derived from Monte Carlo scenario simulations varying the kinetic (reaction and photolysis rate) parameters within their estimated uncertainty bounds. Simulations of a typical winter/spring Antarctic vortex scenario and Match scenarios in the Arctic produce large uncertainty in ozone loss rates and integrated seasonal loss. The simulations clearly indicate that the dominant source of model uncertainty in polar ozone loss is uncertainty in the Cl2O 2 photolysis reaction, which arises from uncertainty in laboratory-measured molecular cross sections at atmospherically important wavelengths. This estimated uncertainty in JCl 2O2 from laboratory measurements seriously hinders our ability to model polar ozone loss within useful quantitative error limits. Atmospheric observations, however, suggest that the Cl2O2 photolysis uncertainty may be less than that derived from the lab data. Comparisons to Match, South Pole ozonesonde, and Aura Microwave Limb Sounder (MLS) data all show that the nominal recommended rate simulations agree with data within uncertainties when the Cl2O2 photolysis error is reduced by a factor of two, in line with previous in situ ClOx measurements. Comparisons to simulations using recent cross sections from Pope et al. (2007) are outside the constrained error bounds in each case. Other reactions producing significant sensitivity in polar ozone loss include BrO + ClO and its branching ratios. These uncertainties challenge our confidence in modeling polar ozone depletion and projecting future changes in response to changing halogen emissions and climate. Further laboratory, theoretical, and possibly atmospheric studies are needed.
- ItemSolar and lunar tides in noctilucent clouds as determined by ground-based lidar(Göttingen : Copernicus GmbH, 2018) Fiedler, J.; Baumgarten, G.Noctilucent clouds (NLCs) occur during summer from midlatitudes to high latitudes. They consist of nanometer-sized ice particles in an altitude range from 80 to 90 km and are sensitive to ambient temperature and water vapor content, which makes them a suitable tracer for variability on all timescales. The data set acquired by the ALOMAR Rayleigh-Mie-Raman (RMR) lidar covers 21 years and is investigated regarding tidal signatures in NLCs. For the first time solar and lunar tidal parameters in NLCs were determined simultaneously from the same data. Several NLC parameters are subject to persistent mean variations throughout the solar day as well as the lunar day. Variations with lunar time are generally smaller compared to variations with solar time. NLC occurrence frequency shows the most robust imprint of the lunar semidiurnal tide. Its amplitude is about 50 % of the solar semidiurnal tide, which is surprisingly large. Phase progressions of NLC occurrence frequency indicate upward propagating solar tides. Below 84 km altitude the corresponding vertical wavelengths are between 20 and 30 km. For the lunar semidiurnal tide phase progressions vary symmetrically with respect to the maximum of the NLC layer. © Author(s) 2018.
- ItemCoal fly ash: Linking immersion freezing behavior and physicochemical particle properties(Göttingen : Copernicus GmbH, 2018) Grawe, S.; Augustin-Bauditz, S.; Clemen, H.-C.; Ebert, M.; Eriksen Hammer, S.; Lubitz, J.; Reicher, N.; Rudich, Y.; Schneider, J.; Staacke, R.; Stratmann, F.; Welti, A.; Wex, H.To date, only a few studies have investigated the potential of coal fly ash particles to trigger heterogeneous ice nucleation in cloud droplets. The presented measurements aim at expanding the sparse dataset and improving process understanding of how physicochemical particle properties can influence the freezing behavior of coal fly ash particles immersed in water. Firstly, immersion freezing measurements were performed with two single particle techniques, i.e., the Leipzig Aerosol Cloud Interaction Simulator (LACIS) and the SPectrometer for Ice Nuclei (SPIN). The effect of suspension time on the efficiency of the coal fly ash particles when immersed in a cloud droplet is analyzed based on the different residence times of the two instruments and employing both dry and wet particle generation. Secondly, two cold-stage setups, one using microliter sized droplets (Leipzig Ice Nucleation Array) and one using nanoliter sized droplets (WeIzmann Supercooled Droplets Observation on Microarray setup) were applied. We found that coal fly ash particles are comparable to mineral dust in their immersion freezing behavior when being dry generated. However, a significant decrease in immersion freezing efficiency was observed during experiments with wet-generated particles in LACIS and SPIN. The efficiency of wet-generated particles is in agreement with the cold-stage measurements. In order to understand the reason behind the deactivation, a series of chemical composition, morphology, and crystallography analyses (single particle mass spectrometry, scanning electron microscopy coupled with energy dispersive X-ray microanalysis, X-ray diffraction analysis) were performed with dry- and wet-generated particles. From these investigations, we conclude that anhydrous CaSO4 and CaO - which, if investigated in pure form, show the same qualitative immersion freezing behavior as observed for dry-generated coal fly ash particles - contribute to triggering heterogeneous ice nucleation at the particle-water interface. The observed deactivation in contact with water is related to changes in the particle surface properties which are potentially caused by hydration of CaSO4 and CaO. The contribution of coal fly ash to the ambient population of ice-nucleating particles therefore depends on whether and for how long particles are immersed in cloud droplets.
- ItemThe Smithsonian solar constant data revisited: No evidence for a strong effect of solar activity in ground-based insolation data(Göttingen : Copernicus GmbH, 2011) Feulner, G.Apparent evidence for a strong signature of solar activity in ground-based insolation data was recently reported. In particular, a strong increase of the irradiance of the direct solar beam with sunspot number as well as a decline of the brightness of the solar aureole and the measured precipitable water content of the atmosphere with solar activity were presented. The latter effect was interpreted as evidence for cosmic-ray-induced aerosol formation. Here I show that these spurious results are due to a failure to correct for seasonal variations and the effects of volcanic eruptions and local pollution in the data. After correcting for these biases, neither the atmospheric water content nor the brightness of the solar aureole show any significant change with solar activity, and the variations of the solar-beam irradiance with sunspot number are in agreement with previous estimates. Hence there is no evidence for the influence of solar activity on the climate being stronger than currently thought.