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- ItemRobust changes in tropical rainy season length at 1.5 °C and 2 °C(Bristol : IOP Publ., 2018) Saeed, Fahad; Bethke, Ingo; Fischer, Erich; Legutke, Stephanie; Shiogama, Hideo; Stone, Dáithí A.; Schleussner, Carl-FriedrichChanges in the hydrological cycle are among the aspects of climate change most relevant for human systems and ecosystems. Besides trends in overall wetting or drying, changes in temporal characteristics of wetting and drying are of crucial importance in determining the climate hazard posed by such changes. This is particularly the case for tropical regions, where most precipitation occurs during the rainy season and changes in rainy season onset and length have substantial consequences. Here we present projections for changes in tropical rainy season lengths for mean temperature increase of 1.5 °C and 2 °C above pre-industrial levels. Based on multi-ensemble quasi-stationary simulations at these warming levels, our analysis indicates robust changes in rainy season characteristics in large parts of the tropics despite substantial natural variability. Specifically, we report a robust shortening of the rainy season for all of tropical Africa as well as north-east Brazil. About 27% of West Africa is projected to experience robust changes in the rainy season length with a mean shortening of about 7 days under 1.5 °C. We find that changes in the temporal characteristics are largely unrelated to changes in overall precipitation, highlighting the importance of investigating both separately.
- ItemInfluence of annealing on microstructure and mechanical properties of ultrafine-grained Ti45Nb(Amsterdam [u.a.] : Elsevier Science, 2019) Völker, B.; Maier-Kiener, V.; Werbach, K.; Müller, T.; Pilz, S.; Calin, M.; Eckert, J.; Hohenwarter, A.Beta-Ti alloys have been intensively investigated in the last years because of their favorable low Young's moduli, biocompatibility and bio-inertness, making these alloys interesting candidates for implant materials. Due to their low mechanical strength, efforts are currently devoted to increasing it. A promising way to improve the strength is to tailor the microstructure using severe plastic deformation (SPD). In this investigation high pressure torsion was used to refine the microstructure of a Ti-45wt.%Nb alloy inducing a grain size of ~50 nm. The main focus of the subsequent investigations was devoted to the thermal stability of the microstructure. Isochronal heat-treatments performed for 30 min in a temperature range up to 500 °C caused an increase of hardness with a peak value at 300 °C before the hardness decreased at higher temperatures. Simultaneously, a distinct temperature-dependent variation of the Young's modulus was also measured. Tensile tests revealed an increase in strength after annealing compared to the SPD-state. Microstructural investigations showed that annealing causes the formation of α-Ti. The findings suggest that the combination of severe plastic deformation with subsequent heat treatment provides a feasible way to improve the mechanical properties of SPD-deformed β-Ti alloys making them suitable for higher strength applications.
- ItemInfluence of substrate dimensionality on the growth mode of epitaxial 3D-bonded GeTe thin films: From 3D to 2D growth(Amsterdam [u.a.] : Elsevier Science, 2019) Hilmi, Isom; Lotnyk, Andriy; Gerlach, Jürgen W.; Schumacher, Philipp; Rauschenbach, BerndThe pseudo-binary line of Sb2Te3-GeTe contains alloys featuring different crystalline characteristics from two-dimensionally (2D-) bonded Sb2Te3 to three-dimensionally (3D-) bonded GeTe. Here, the growth scenario of 3D-bonded GeTe is investigated by depositing epitaxial GeTe thin films on Si(111) and Sb2Te3-buffered Si(111) substrates using pulsed laser deposition (PLD). GeTe thin films were grown in trigonal structure within a temperature window for epitaxial growth of 210–270 °C on unbuffered Si(111) substrates. An unconventional growth onset was characterized by the formation of a thin amorphous GeTe layer. Nonetheless, the as-grown film is found to be crystalline. Furthermore, by employing a 2D-bonded Sb2Te3 thin film as a seeding layer on Si(111), a 2D growth of GeTe is harnessed. The epitaxial window can substantially be extended especially towards lower temperatures down to 145 °C. Additionally, the surface quality is significantly improved. The inspection of the local structure of the epitaxial films reveals the presence of a superposition of twinned domains, which is assumed to be an intrinsic feature of such thin films. This work might open a way for an improvement of an epitaxy of a 3D-bonded material on a highly-mismatched substrate (e.g. Si (111)) by employing a 2D-bonded seeding layer (e.g. Sb2Te3).
- ItemOptically stimulated luminescence dating of young fluvial deposits of the Middle Elbe River Flood Plains using different age models(Warsaw : De Gruyter, 2014) Kunz, Alexander; Pflanz, Dorthe; Weniger, Tobias; Urban, Brigitte; Krüger, Frank; Chen, Yue-GauIn the last few decades optically stimulated luminescence (OSL) dating has become an im-portant tool in geochronological studies. The great advantage of the method, i.e. dating the deposi-tional age of sediments directly, can be impaired by incomplete bleaching of grains. This can result in a scattered distribution of equivalent doses (DE), leading to incorrect estimation of the depositional age. Thoroughly tested protocols as well as good data analysis with adequate statistical methods are important to overcome this problem. In this study, samples from young fluvial sand and flood plain deposits from the Elbe River in northern Germany were investigated to compare its depositional ages from different age models with well-known historical dates. Coarse grain quartz (100-200 μm and 150-250 μm) and polymineral fine grains (4-11 μm) were dated using the single aliquot regenerative (SAR) dose protocol. The paleodose (DP) was calculated from the DE data set using different ap-proaches. Results were compared with the development of the Elbe River, which is well-documented by historical records and maps covering the last 1,000 years. Depending on the statistical approach it can be demonstrated that depositional ages significantly differ from the most likely depositional age. For the investigated coarse grain quartz samples all ages calculated from the MAM-3UL, including their uncertainties, are within the historical documented age. Results of the polymineral fine grain samples are overestimating the historically documented depositional age, indicating undetectable in-complete bleaching. This study shows the importance of using an adequate statistical approach to cal-culate reliable OSL ages from fluvial sediments. © 2013 Silesian University of Technology, Gliwice, Poland. All rights reserved.
- ItemThe mutual dependence of negative emission technologies and energy systems(Cambridge : RSC Publ., 2019) Creutzig, Felix; Breyer, Christian; Hilaire, Jérôme; Minx, Jan; Peters, Glen P.; Socolow, RobertWhile a rapid decommissioning of fossil fuel technologies deserves priority, most climate stabilization scenarios suggest that negative emission technologies (NETs) are required to keep global warming well below 2 °C. Yet, current discussions on NETs are lacking a distinct energy perspective. Prominent NETs, such as bioenergy with carbon capture and storage (BECCS) and direct air carbon capture and storage (DACCS), will integrate differently into the future energy system, requiring a concerted research effort to determine adequate means of deployment. In this perspective, we discuss the importance of energy per carbon metrics, factors of future cost development, and the dynamic response of NETs in intermittent energy systems. The energy implications of NETs deployed at scale are massive, and NETs may conceivably impact future energy systems substantially. DACCS outperform BECCS in terms of primary energy required per ton of carbon sequestered. For different assumptions, DACCS displays a sequestration efficiency of 75–100%, whereas BECCS displays a sequestration efficiency of 50–90% or less if indirect land use change is included. Carbon dioxide removal costs of DACCS are considerably higher than BECCS, but if DACCS modularity and granularity helps to foster technological learning to <100$ per tCO2, DACCS may remove CO2 at gigaton scale. DACCS also requires two magnitudes less land than BECCS. Designing NET systems that match intermittent renewable energies will be key for stringent climate change mitigation. Our results contribute to an emerging understanding of NETs that is notably different to that derived from scenario modelling.
- ItemLuminescence dating of volcanogenic outburst flood sediments from Aso volcano and tephric loess deposits, southwest Japan(Warsaw : De Gruyter, 2013) Tsukamoto, Sumiko; Kataoka, Kyoko; Miyabuchi, YasuoLuminescence dating has been applied to volcanogenic outburst flood sediments (Takuma gravel bed) from Aso volcano, Japan, and tephric loess deposits overlying the gravel bed. The poly-mineral fine grains (4-11 μm) from loess deposits were measured with pulsed optically stimulated luminescence (pulsed OSL) and post-IR infrared stimulated luminescence (pIRIR) methods, whereas the Takuma gravel bed containing no quartz, was measured with IRSL and pIRIR methods using sand sized (150-200 μm) plagioclase. The loess deposits date back at least to ∼50 ka by consistent IRSL, pIRIR and pulsed OSL ages from the lowermost part of the loess deposits from one section. The ages obtained from the bottom part of the other loess section are not consistent each other. However, we consider that the pIRIR age (72±6 ka) which showed negligible anomalous fading is most reliable, and regard as a preliminary minimum age of the Takuma gravel bed. The equivalent doses (De) for the plagioclase from the Takuma gravel bed have a narrow distribution and the weighted mean of the three samples yield an age of 89±3 ka. This age is in agreement with the last caldera-forming eruption of Aso volcano (∼87 ka) and it is likely that the pIRIR signal has not been bleached before the deposi-tion. IRSL dating without applying pIRIR using small aliquots was also conducted, however, the IRSL signal shows no clear evidence of an additional bleaching during the event of outburst flood from the caldera lake. © 2013 Silesian University of Technology, Gliwice, Poland. All rights reserved.
- ItemGeothermal potential of the Buntsandstein and Keuper aquifers in NE Bavaria with a focus on deep thermal aquifer storage(Berlin ; Heidelberg : Springer, 2019-9-26) Kunkel, Cindy; Agemar, Thorsten; Stober, IngridIntermediate and deep geothermal resources of Germany are limited to medium and low enthalpy resources. These resources are predominantly used for balneological applications, space and district heating and for power production at nine separate sites. This study focuses on confined aquifers in northeast Bavaria, which can be used for balneology as well as energy storage. Data from pumping tests and production data were interpreted to map the hydraulic conductivity of the main Keuper and Buntsandstein aquifers with a large spatial distribution for geothermal applications deeper than 100 m. Furthermore, temperature estimates as well as the depth of the two aquifers (Keuper 100 to 650 m, Buntsandstein 100 to 1400 m) are incorporated. The results will be visualized in the form of spatial distribution maps of the hydraulic conductivity and temperature, and will be integrated into the geothermal information system GeotIS (https://www.geotis.de). Altogether, about 80% of all 243 sampling sites show hydraulic conductivity values sufficient for geothermal energy utilization. For the Keuper aquifer, even 90% of all 155 sampling sites show transmissivities sufficient for geothermal energy utilization. However, these maps do not replace a feasibility study for specific geothermal projects because detailed geological site assessment is essential when planning a subsurface geothermal system.
- ItemTargeting microplastic particles in the void of diluted suspensions(Amsterdam [u.a.] : Elsevier Science, 2019) Islam, Shohana; Apitius, Lina; Jakob, Felix; Schwaneberg, UlrichAccumulation of microplastic in the environment and food chain will be a grand challenge for our society. Polyurethanes are widely used synthetic polymers in medical (e.g. catheters) and industrial products (especially as foams). Polyurethane is not abundant in nature and only a few microbial strains (fungi and bacteria) and enzymes (polyurethaneases and cutinases) have been reported to efficiently degrade polyurethane. Notably, in nature a long period of time (from 50 to >100 years depending on the literature) is required for degradation of plastics. Material binding peptides (e.g. anchor peptides) bind strongly to polymers such as polypropylene, polyethylene terephthalate, and polyurethane and can target specifically polymers. In this study we report the fusion of the anchor peptide Tachystatin A2 to the bacterial cutinase Tcur1278 which accelerated the degradation of polyester-polyurethane nanoparticles by a factor of 6.6 in comparison to wild-type Tcur1278. Additionally, degradation half-lives of polyester-polyurethane nanoparticles were reduced from 41.8 h to 6.2 h (6.7-fold) in a diluted polyester-polyurethane suspension (0.04% w/v).
- ItemTargeted policies can compensate most of the increased sustainability risks in 1.5 °C mitigation scenarios(Bristol : IOP Publ., 2018) Bertram, Christoph; Luderer, Gunnar; Popp, Alexander; Minx, Jan Christoph; Lamb, William F; Stevanović, Miodrag; Humpenöder, Florian; Giannousakis, Anastasis; Kriegler, ElmarMeeting the 1.5 °C goal will require a rapid scale-up of zero-carbon energy supply, fuel switching to electricity, efficiency and demand-reduction in all sectors, and the replenishment of natural carbon sinks. These transformations will have immediate impacts on various of the sustainable development goals. As goals such as affordable and clean energy and zero hunger are more immediate to great parts of global population, these impacts are central for societal acceptability of climate policies. Yet, little is known about how the achievement of other social and environmental sustainability objectives can be directly managed through emission reduction policies. In addition, the integrated assessment literature has so far emphasized a single, global (cost-minimizing) carbon price as the optimal mechanism to achieve emissions reductions. In this paper we introduce a broader suite of policies—including direct sector-level regulation, early mitigation action, and lifestyle changes—into the integrated energy-economy-land-use modeling system REMIND-MAgPIE. We examine their impact on non-climate sustainability issues when mean warming is to be kept well below 2 °C or 1.5 °C. We find that a combination of these policies can alleviate air pollution, water extraction, uranium extraction, food and energy price hikes, and dependence on negative emissions technologies, thus resulting in substantially reduced sustainability risks associated with mitigating climate change. Importantly, we find that these targeted policies can more than compensate for most sustainability risks of increasing climate ambition from 2 °C to 1.5 °C.
- ItemFreshwater requirements of large-scale bioenergy plantations for limiting global warming to 1.5 °C(Bristol : IOP Publ., 2019) Stenzel, Fabian; Gerten, Dieter; Werner, Constanze; Jägermeyr, JonasLimiting mean global warming to well below 2 °C will probably require substantial negative emissions (NEs) within the 21st century. To achieve these, bioenergy plantations with subsequent carbon capture and storage (BECCS) may have to be implemented at a large scale. Irrigation of these plantations might be necessary to increase the yield, which is likely to put further pressure on already stressed freshwater systems. Conversely, the potential of bioenergy plantations (BPs) dedicated to achieving NEs through CO2 assimilation may be limited in regions with low freshwater availability. This paper provides a first-order quantification of the biophysical potentials of BECCS as a negative emission technology contribution to reaching the 1.5 °C warming target, as constrained by associated water availabilities and requirements. Using a global biosphere model, we analyze the availability of freshwater for irrigation of BPs designed to meet the projected NEs to fulfill the 1.5 °C target, spatially explicitly on areas not reserved for ecosystem conservation or agriculture. We take account of the simultaneous water demands for agriculture, industries, and households and also account for environmental flow requirements (EFRs) needed to safeguard aquatic ecosystems. Furthermore, we assess to what extent different forms of improved water management on the suggested BPs and on cropland may help to reduce the freshwater abstractions. Results indicate that global water withdrawals for irrigation of BPs range between ∼400 and ∼3000 km3 yr−1, depending on the scenario and the conversion efficiency of the carbon capture and storage process. Consideration of EFRs reduces the NE potential significantly, but can partly be compensated for by improved on-field water management.