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Beller, Matthias
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Kopf, Sara
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Neumann, Helfried
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benzaldehyde derivative
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Manganese-catalyzed selective C–H activation and deuteration by means of a catalytic transient directing group strategy
(
London : Royal Society of Chemistry (RSC),
2021
)
Kopf, Sara
;
Neumann, Helfried
;
Beller, Matthias
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A novel manganese-catalyzed C-H activation methodology for selective hydrogen isotope exchange of benzaldehydes is presented. Using D2O as a cheap and convenient source of deuterium, the reaction proceeds with excellent functional group tolerance. Highortho-selectivity is achieved in the presence of catalytic amounts of specific amines, whichin situform a transient directing group. © The Royal Society of Chemistry 2021.
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