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    Particle hygroscopicity during atmospheric new particle formation events: Implications for the chemical species contributing to particle growth
    (Göttingen : Copernicus, 2013) Wu, Z.; Birmili, W.; Poulain, L.; Poulain, L.; Merkel, M.; Fahlbusch, B.; Van Pinxteren, D.; Herrmann, H.; Wiedensohler, A.
    This study examines the hygroscopicity of newly formed particles (diameters range 25-45 nm) during two atmospheric new particle formation (NPF) events in the German mid-level mountains during the Hill Cap Cloud Thuringia 2010 (HCCT-2010) field experiment. At the end of the NPF event involving clear particle growth, we measured an unusually high soluble particle fraction of 58.5% at 45 nm particle size. The particle growth rate contributed through sulfuric acid condensation only accounts for around 6.5% of the observed growth rate. Estimations showed that sulfuric acid condensation explained, however, only around 10% of that soluble particle fraction. Therefore, the formation of additional water-soluble matter appears imperative to explain the missing soluble fraction. Although direct evidence is missing, we consider water-soluble organics as candidates for this mechanism. For the case with clear growth process, the particle growth rate was determined by two alternative methods based on tracking the mode diameter of the nucleation mode. The mean particle growth rate obtained from the inter-site data comparison using Lagrangian consideration is 3.8 (± 2.6) nm h-1. During the same period, the growth rate calculated based on one site data is 5.0 nm h-1 using log-normal distribution function method. In light of the fact that considerable uncertainties could be involved in both methods, we consider both estimated growth rates consistent.
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    Modeling forest plantations for carbon uptake with the LPJmL dynamic global vegetation model
    (Göttingen : Copernicus Publ., 2019) Braakhekke, Maarten C.; Doelman, Jonathan C.; Baas, Peter; Müller, Christoph; Schaphoff, Sibyll; Stehfest, Elke; van Vuuren, Detlef P.
    We present an extension of the dynamic global vegetation model, Lund-Potsdam-Jena Managed Land (LPJmL), to simulate planted forests intended for carbon (C) sequestration. We implemented three functional types to simulate plantation trees in temperate, tropical, and boreal climates. The parameters of these functional types were optimized to fit target growth curves (TGCs). These curves represent the evolution of stemwood C over time in typical productive plantations and were derived by combining field observations and LPJmL estimates for equivalent natural forests. While the calibrated model underestimates stemwood C growth rates compared to the TGCs, it represents substantial improvement over using natural forests to represent afforestation. Based on a simulation experiment in which we compared global natural forest versus global forest plantation, we found that forest plantations allow for much larger C uptake rates on the timescale of 100 years, with a maximum difference of a factor of 1.9, around 54 years. In subsequent simulations for an ambitious but realistic scenario in which 650Mha (14% of global managed land, 4.5% of global land surface) are converted to forest over 85 years, we found that natural forests take up 37PgC versus 48PgC for forest plantations. Comparing these results to estimations of C sequestration required to achieve the 2°C climate target, we conclude that afforestation can offer a substantial contribution to climate mitigation. Full evaluation of afforestation as a climate change mitigation strategy requires an integrated assessment which considers all relevant aspects, including costs, biodiversity, and trade-offs with other land-use types. Our extended version of LPJmL can contribute to such an assessment by providing improved estimates of C uptake rates by forest plantations. © 2019 American Institute of Physics Inc.. All rights reserved.
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    Description and evaluation of the process-based forest model 4C v2.2 at four European forest sites
    (Katlenburg-Lindau : Copernicus, 2020) Lasch-Born, Petra; Suckow, Felicitas; Reyer, Christopher P. O.; Gutsch, Martin; Kollas, Chris; Badeck, Franz-Werner; Bugmann, Harald K. M.; Grote, Rüdiger; Fürstenau, Cornelia; Lindner, Marcus; Schaber, Jörg
    The process-based model 4C (FORESEE) has been developed over the past 20 years to study climate impacts on forests and is now freely available as an open-source tool. The objective of this paper is to provide a comprehensive description of this 4C version (v2.2) for scientific users of the model and to present an evaluation of 4C at four different forest sites across Europe. The evaluation focuses on forest growth as well as carbon (net ecosystem exchange, gross primary production), water (actual evapotranspiration, soil water content), and heat fluxes (soil temperature) using data from the PROFOUND database. We applied different evaluation metrics and compared the daily, monthly, and annual variability of observed and simulated values. The ability to reproduce forest growth (stem diameter and biomass) differs from site to site and is best for a pine stand in Germany (Peitz, model efficiency ME=0.98). 4C is able to reproduce soil temperature at different depths in Sorø and Hyytiälä with good accuracy (for all soil depths ME > 0.8). The dynamics in simulating carbon and water fluxes are well captured on daily and monthly timescales (0.51 < ME < 0.983) but less so on an annual timescale (ME < 0). This model–data mismatch is possibly due to the accumulation of errors because of processes that are missing or represented in a very general way in 4C but not with enough specific detail to cover strong, site-specific dependencies such as ground vegetation growth. These processes need to be further elaborated to improve the projections of climate change on forests. We conclude that, despite shortcomings, 4C is widely applicable, reliable, and therefore ready to be released to the scientific community to use and further develop the model.
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    Climate analogues suggest limited potential for intensification of production on current croplands under climate change
    (London : Nature Publishing Group, 2016) Pugh, T.A.M.; Müller, C.; Elliott, J.; Deryng, D.; Folberth, C.; Olin, S.; Schmid, E.; Arneth, A.