Search Results
Evaluating stratospheric ozone and water vapour changes in CMIP6 models from 1850 to 2100
2021, Keeble, James, Hassler, Birgit, Banerjee, Antara, Checa-Garcia, Ramiro, Chiodo, Gabriel, Davis, Sean, Eyring, Veronika, Griffiths, Paul T., Morgenstern, Olaf, Nowack, Peer, Zeng, Guang, Zhang, Jiankai, Bodeker, Greg, Burrows, Susannah, Cameron-Smith, Philip, Cugnet, David, Danek, Christopher, Deushi, Makoto, Horowitz, Larry W., Kubin, Anne, Li, Lijuan, Lohmann, Gerrit, Michou, Martine, Mills, Michael J., Nabat, Pierre, Olivié, Dirk, Park, Sungsu, Seland, Øyvind, Stoll, Jens, Wieners, Karl-Hermann, Wu, Tongwen
Stratospheric ozone and water vapour are key components of the Earth system, and past and future changes to both have important impacts on global and regional climate. Here, we evaluate long-term changes in these species from the pre-industrial period (1850) to the end of the 21st century in Coupled Model Intercomparison Project phase 6 (CMIP6) models under a range of future emissions scenarios. There is good agreement between the CMIP multi-model mean and observations for total column ozone (TCO), although there is substantial variation between the individual CMIP6 models. For the CMIP6 multi-model mean, global mean TCO has increased from ∼300 DU in 1850 to ∼ 305 DU in 1960, before rapidly declining in the 1970s and 1980s following the use and emission of halogenated ozone-depleting substances (ODSs). TCO is projected to return to 1960s values by the middle of the 21st century under the SSP2-4.5, SSP3-7.0, SSP4-3.4, SSP4-6.0, and SSP5-8.5 scenarios, and under the SSP3-7.0 and SSP5-8.5 scenarios TCO values are projected to be ∼ 10 DU higher than the 1960s values by 2100. However, under the SSP1-1.9 and SSP1-1.6 scenarios, TCO is not projected to return to the 1960s values despite reductions in halogenated ODSs due to decreases in tropospheric ozone mixing ratios. This global pattern is similar to regional patterns, except in the tropics where TCO under most scenarios is not projected to return to 1960s values, either through reductions in tropospheric ozone under SSP1-1.9 and SSP1-2.6, or through reductions in lower stratospheric ozone resulting from an acceleration of the Brewer-Dobson circulation under other Shared Socioeconomic Pathways (SSPs). In contrast to TCO, there is poorer agreement between the CMIP6 multi-model mean and observed lower stratospheric water vapour mixing ratios, with the CMIP6 multi-model mean underestimating observed water vapour mixing ratios by ∼ 0.5 ppmv at 70 hPa. CMIP6 multi-model mean stratospheric water vapour mixing ratios in the tropical lower stratosphere have increased by ∼ 0.5 ppmv from the pre-industrial to the present-day period and are projected to increase further by the end of the 21st century. The largest increases (∼ 2 ppmv) are simulated under the future scenarios with the highest assumed forcing pathway (e.g. SSP5-8.5). Tropical lower stratospheric water vapour, and to a lesser extent TCO, shows large variations following explosive volcanic eruptions. © Author(s) 2021.
VAHCOLI, a new concept for lidars: technical setup, science applications, and first measurements
2021, Lübken, Franz-Josef, Höffner, Josef
A new concept for a cluster of compact lidar systems named VAHCOLI (Vertical And Horizontal COverage by LIdars) is presented, which allows for the measurement of temperatures, winds, and aerosols in the middle atmosphere (10 110 km) with high temporal and vertical resolution of minutes and some tens of meters, respectively, simultaneously covering horizontal scales from a few hundred meters to several hundred kilometers ( four-dimensional coverage ). The individual lidars ( units ) being used in VAHCOLI are based on a diode-pumped alexandrite laser, which is currently designed to detect potassium (D 770 nm), and on sophisticated laser spectroscopy measuring all relevant frequencies (seeder laser, power laser, backscattered light) with high temporal resolution (2 ms) and high spectral resolution applying Doppler-free spectroscopy. The frequency of the lasers and the narrowband filter in the receiving system are stabilized to typically 10 100 kHz, which is a factor of roughly 105 smaller than the Doppler-broadened Rayleigh signal. Narrowband filtering allows for the measurement of Rayleigh and/or resonance scattering separately from the aerosol (Mie) signal during both night and day. Lidars used for VAHCOLI are compact (volume: 1m3) and multi-purpose systems which employ contemporary electronic, optical, and mechanical components. The units are designed to autonomously operate under harsh field conditions in remote locations. An error analysis with parameters of the anticipated system demonstrates that temperatures and line-of-sight winds can be measured from the lower stratosphere to the upper mesosphere with an accuracy of (0.1 5)K and (0.1 10)ms1, respectively, increasing with altitude. We demonstrate that some crucial dynamical processes in the middle atmosphere, such as gravity waves and stratified turbulence, can be covered by VAHCOLI with sufficient temporal, vertical, and horizontal sampling and resolution. The four-dimensional capabilities of VAHCOLI allow for the performance of time-dependent analysis of the flow field, for example by employing Helmholtz decomposition, and for carrying out statistical tests regarding, for example, intermittency and helicity. The first test measurements under field conditions with a prototype lidar were performed in January 2020. The lidar operated successfully during a 6-week period (night and day) without any adjustment. The observations covered a height range of 5 100 km and demonstrated the capability and applicability of this unit for the VAHCOLI concept.
Model simulations of chemical effects of sprites in relation with observed HO2 enhancements over sprite-producing thunderstorms
2021, Winkler, Holger, Yamada, Takayoshi, Kasai, Yasuko, Berger, Uwe, Notholt, Justus
Recently, measurements by the Superconducting Submillimeter-Wave Limb Emission Sounder (SMILES) satellite instrument have been presented which indicate an increase in mesospheric HO2 above sprite-producing thunderstorms. The aim of this paper is to compare these observations to model simulations of chemical sprite effects. A plasma chemistry model in combination with a vertical transport module was used to simulate the impact of a streamer discharge in the altitude range 70–80 km, corresponding to one of the observed sprite events. Additionally, a horizontal transport and dispersion model was used to simulate advection and expansion of the sprite air masses. The model simulations predict a production of hydrogen radicals mainly due to reactions of proton hydrates formed after the electrical discharge. The net effect is a conversion of water molecules into H+OH. This leads to increasing HO2 concentrations a few hours after the electric breakdown. Due to the modelled long-lasting increase in HO2 after a sprite discharge, an accumulation of HO2 produced by several sprites appears possible. However, the number of sprites needed to explain the observed HO2 enhancements is unrealistically large. At least for the lower measurement tangent heights, the production mechanism of HO2 predicted by the model might contribute to the observed enhancements.
Inherent Dissipation of Upwind‐Biased Potential Temperature Advection and its Feedback on Model Dynamics
2021, Gassmann, A.
Higher order upwind-biased advection schemes are often used for potential temperature advection in dynamical cores of atmospheric models. The inherent diffusive and antidiffusive fluxes are interpreted here as the effect of irreversible sub-gridscale dynamics. For those, total energy conservation and positive internal entropy production must be guaranteed. As a consequence of energy conservation, the pressure gradient term should be formulated in Exner pressure form. The presence of local antidiffusive fluxes in potential temperature advection schemes foils the validity of the second law of thermodynamics. Due to this failure, a spurious wind acceleration into the wrong direction is locally induced via the pressure gradient term. When correcting the advection scheme to be more entropically consistent, the spurious acceleration is avoided, but two side effects come to the fore: (i) the overall accuracy of the advection scheme decreases and (ii) the now purely diffusive fluxes become more discontinuous compared to the original ones, which leads to more sudden body forces in the momentum equation. Therefore, the amplitudes of excited gravity waves from jets and fronts increase compared to the original formulation with inherent local antidiffusive fluxes. The means used for supporting the argumentation line are theoretical arguments concerning total energy conservation and internal entropy production, pure advection tests, one-dimensional advection-dynamics interaction tests and evaluation of runs with a global atmospheric dry dynamical core.
Orographically induced spontaneous imbalance within the jet causing a large-scale gravity wave event
2021, Geldenhuys, Markus, Preusse, Peter, Krisch, Isabell, Zülicke, Christoph, Ungermann, Jörn, Ern, Manfred, Friedl-Vallon, Felix, Riese, Martin
To better understand the impact of gravity waves (GWs) on the middle atmosphere in the current and future climate, it is essential to understand their excitation mechanisms and to quantify their basic properties. Here a new process for GW excitation by orography-jet interaction is discussed. In a case study, we identify the source of a GW observed over Greenland on 10 March 2016 during the POLSTRACC (POLar STRAtosphere in a Changing Climate) aircraft campaign. Measurements were taken with the Gimballed Limb Observer for Radiance Imaging of the Atmosphere (GLORIA) instrument deployed on the High Altitude Long Range (HALO) German research aircraft. The measured infrared limb radiances are converted into a 3D observational temperature field through the use of inverse modelling and limited-angle tomography. We observe GWs along a transect through Greenland where the GW packet covers ≈1/3 of the Greenland mainland. GLORIA observations indicate GWs between 10 and 13km of altitude with a horizontal wavelength of 330km, a vertical wavelength of 2km and a large temperature amplitude of 4.5K. Slanted phase fronts indicate intrinsic propagation against the wind, while the ground-based propagation is with the wind. The GWs are arrested below a critical layer above the tropospheric jet. Compared to its intrinsic horizontal group velocity (25-72ms-1) the GW packet has a slow vertical group velocity of 0.05-0.2ms-1. This causes the GW packet to propagate long distances while spreading over a large area and remaining constrained to a narrow vertical layer. A plausible source is not only orography, but also out-of-balance winds in a jet exit region and wind shear. To identify the GW source, 3D GLORIA observations are combined with a gravity wave ray tracer, ERA5 reanalysis and high-resolution numerical experiments. In a numerical experiment with a smoothed orography, GW activity is quite weak, indicating that the GWs in the realistic orography experiment are due to orography. However, analysis shows that these GWs are not mountain waves. A favourable area for spontaneous GW emission is identified in the jet by the cross-stream ageostrophic wind, which indicates when the flow is out of geostrophic balance. Backwards ray-tracing experiments trace into the jet and regions where the Coriolis and the pressure gradient forces are out of balance. The difference between the full and a smooth-orography experiment is investigated to reveal the missing connection between orography and the out-of-balance jet. We find that this is flow over a broad area of elevated terrain which causes compression of air above Greenland. The orography modifies the wind flow over large horizontal and vertical scales, resulting in out-of-balance geostrophic components. The out-of-balance jet then excites GWs in order to bring the flow back into balance. This is the first observational evidence of GW generation by such an orography-jet mechanism.
Linear relationship between effective radius and precipitation water content near the top of convective clouds: measurement results from ACRIDICON–CHUVA campaign
2021, Braga, Ramon Campos, Rosenfeld, Daniel, Krüger, Ovid O., Ervens, Barbara, Holanda, Bruna A., Wendisch, Manfred, Krisna, Trismono, Pöschl, Ulrich, Andreae, Meinrat O., Voigt, Christiane, Pöhlker, Mira L.
Quantifying the precipitation within clouds is a crucial challenge to improve our current understanding of the Earth's hydrological cycle.We have investigated the relationship between the effective radius of droplets and ice particles (re) and precipitation water content (PWC) measured by cloud probes near the top of growing convective cumuli. The data for this study were collected during the ACRIDICON-CHUVA campaign on the HALO research aircraft in clean and polluted conditions over the Amazon Basin and over the western tropical Atlantic in September 2014. Our results indicate a threshold of re ∼ 13 μm for warm rain initiation in convective clouds, which is in agreement with previous studies. In clouds over the Atlantic Ocean, warm rain starts at smaller re, likely linked to the enhancement of coalescence of drops formed on giant cloud condensation nuclei. In cloud passes where precipitation starts as ice hydrometeors, the threshold of re is also shifted to values smaller than 13 μm when coalescence processes are suppressed and precipitating particles are formed by accretion. We found a statistically significant linear relationship between PWC and re for measurements at cloud tops, with a correlation coefficient of ∼ 0:94. The tight relationship between re and PWC was established only when particles with sizes large enough to precipitate (drizzle and raindrops) are included in calculating re. Our results emphasize for the first time that re is a key parameter to determine both initiation and amount of precipitation at the top of convective clouds. © Author(s) 2021.
Evidence for the In‐Situ Generation of Plasma Depletion Structures Over the Transition Region of Geomagnetic Low‐Mid Latitude
2021, Sivakandan, M., Mondal, S., Sarkhel, S., Chakrabarty, D., Sunil Krishna, M.V., Upadhayaya, A.K., Shinbori, A., Sori, T., Kannaujiya, S., Champati Ray, P.K.
On a geomagnetic quiet night of October 29, 2018, we captured an observational evidence of the onset of dark band structures within the field-of-view of an all-sky airglow imager operating at 630.0 nm over a geomagnetic low-mid latitude transition region, Hanle, Leh Ladakh. Simultaneous ionosonde observations over New Delhi shows the occurrence of spread-F in the ionograms. Additionally, virtual and peak height indicate vertical upliftment in the F layer altitude and reduction in the ionospheric peak frequency were also observed when the dark band pass through the ionosonde location. All these results confirmed that the observed depletions are indeed associated with ionospheric F region plasma irregularities. The rate of total electron content index (ROTI) indicates the absence of plasma bubble activities over the equatorial/low latitude region which confirms that the observed event is a mid-latitude plasma depletion. Our calculations reveal that the growth time of the plasma depletion is ∼2 h if one considers only the Perkins instability mechanism. This is not consistent with the present observations as the plasma depletion developed within ∼25 min. By invoking possible Es layer instabilities and associated E-F region coupling, we show that the growth rate increases roughly by an order of magnitude. This strongly suggests that the Cosgrove and Tsunoda mechanism may be simultaneously operational in this case. Furthermore, it is also suggested that reduced F region flux-tube integrated conductivity in the southern part of onset region created conducive background conditions for the growth of the plasma depletion on this night.
A novel rocket-borne ion mass spectrometer with large mass range: instrument description and first-flight results
2021, Stude, Joan, Aufmhoff, Heinfried, Schlager, Hans, Rapp, Markus, Arnold, Frank, Strelnikov, Boris
We present a novel rocket-borne ion mass spectrometer named ROMARA (ROcket-borne MAss spectrometer for Research in the Atmosphere) for measuring atmospheric positive and negative ions (atomic, molecular and cluster ions) and positively and negatively charged meteor smoke particles. Our ROMARA instrument has, compared to previous rocket-borne ion mass spectrometers, a markedly larger mass range of up to m=z 2000 and a larger sensitivity, particularly for meteor smoke particle detection. The major objectives of this first ROMARA flight included the following: a functional test of the ROMARA instrument, measurements between 55 and 121 km in the mass range of atmospheric positive and negative ions, a first attempt to conduct mass spectrometric measurements in the mass range of meteor smoke particles with mass-to-charge ratios up to m=z 2000, and measurements inside a polar mesospheric winter echo layer as detected by ground-based radar. Our ROMARA measurements took place on the Arctic island of Andøya, Norway, at around noon in April 2018 and represented an integral part of the polar mesospheric winter radar echo (PMWE) rocket campaign. During the rocket flight, ROMARA was operated in a measurement mode, offering maximum sensitivity and the ability to qualitatively detect total ion signatures even beyond its mass-resolving mass range. On this first ROMARA flight we were able to meet all of our objectives. We detected atmospheric species including positive atomic, molecular and cluster ions along with negative molecular ions up to about m=z 100. Above m=z 2000, ROMARA measured strong negative-ion signatures, which are likely due to negatively charged meteor smoke particles. © 2021 Author(s).
Mesospheric gravity wave activity estimated via airglow imagery, multistatic meteor radar, and SABER data taken during the SIMONe–2018 campaign
2021, Vargas, Fabio, Chau, Jorge L., Charuvil Asokan, Harikrishnan, Gerding, Michael
We describe in this study the analysis of small and large horizontal-scale gravity waves from datasets composed of images from multiple mesospheric airglow emissions as well as multistatic specular meteor radar (MSMR) winds collected in early November 2018, during the SIMONe-2018 (Spread-spectrum Interferometric Multi-static meteor radar Observing Network) campaign. These ground-based measurements are supported by temperature and neutral density profiles from TIMED/SABER (Thermosphere, Ionosphere, Mesosphere Energetics and Dynamics/Sounding of the Atmosphere using Broadband Emission Radiometry) satellite in orbits near Kühlungsborn, northern Germany (54.1 N, 11.8 E). The scientific goals here include the characterization of gravity waves and their interaction with the mean flow in the mesosphere and lower thermosphere and their relationship to dynamical conditions in the lower and upper atmosphere. We have obtained intrinsic parameters of small- and large-scale gravity waves and characterized their impact in the mesosphere via momentum flux (FM) and momentum flux divergence (FD) estimations. We have verified that a small percentage of the detected wave events is responsible for most of FM measured during the campaign from oscillations seen in the airglow brightness and MSMR winds taken over 45 h during four nights of clear-sky observations. From the analysis of small-scale gravity waves (λh < 725 km) seen in airglow images, we have found FM ranging from 0.04-24.74 m2 s-2 (1.62 ± 2.70 m2 s-2 on average). However, small-scale waves with FM > 3 m2 s-2 (11 % of the events) transport 50 % of the total measured FM. Likewise, wave events of FM > 10 m2 s-2 (2 % of the events) transport 20 % of the total. The examination of large-scale waves (λh > 725 km) seen simultaneously in airglow keograms and MSMR winds revealed amplitudes > 35 %, which translates into FM Combining double low line 21.2-29.6 m2 s-2. In terms of gravity-wave-mean-flow interactions, these large FM waves could cause decelerations of FD Combining double low line 22-41 m s-1 d-1 (small-scale waves) and FD Combining double low line 38-43 m s-1 d-1 (large-scale waves) if breaking or dissipating within short distances in the mesosphere and lower thermosphere region. © 2021 Fabio Vargas et al.
Multi‐Point Measurements of the Plasma Properties Inside an Aurora From the SPIDER Sounding Rocket
2021, Giono, Gabriel, Ivchenko, Nickolay, Sergienko, Tima, Brändström, Urban
The Small Payloads for Investigation of Disturbances in Electrojet by Rockets (SPIDER) sounding rocket was launched on February 2nd, 2016 (21:09 UT), deploying 10 free falling units (FFUs) inside a westward traveling auroral surge. Each FFUs deployed spherical electric field and Langmuir probes on wire-booms, providing in situ multi-point recordings of the electric field and plasma properties. The analytical retrieval of the plasma parameters, namely the electron density, electron temperature and plasma potential, from the Langmuir probe measurements was non-trivial due to sheath effects and detailed explanation are discussed in this article. An empirical assumption on the sheath thickness was required, which was confirmed by simulating the plasma environment around the FFU using the Spacecraft Plasma Interaction Software (SPIS). In addition, the retrieved electron density and temperature are also in agreement with the simultaneous incoherent scatter radar measurements from the EISCAT facility. These two independent confirmations provided a good level of confidence in the plasma parameters obtained from the FFUs, and events observed during the flight are discussed in more details. Hints of drift-wave instabilities and increased currents inside a region of enhanced density were observed by the FFUs.